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Finite-range numerical atomic orbitals are the basis functions of choice for several first principles methods, due to their flexibility and scalability. Generating and testing such basis sets, however, remains a significant challenge for…

Chemical Physics · Physics 2013-11-12 Fabiano Corsetti , M. -V. Fernández-Serra , José M. Soler , Emilio Artacho

New sets of functions with arbitrary large finite cardinality are constructed for two-electron atoms. Functions from these sets exactly satisfy the Kato's cusp conditions. The new functions are special linear combinations of Hylleraas-…

Atomic Physics · Physics 2020-01-08 A. T. Kruppa , J. Kovács , I. Hornyak

A detailed comparison of Faddeev and variational wave functions for $^3$H, calculated with realistic nuclear forces, has been made to study the form of three-body correlations in few-body nuclei. Three new three-body correlations for use in…

Nuclear Theory · Physics 2008-11-26 A. Arriaga , V. R. Pandharipande , R. B. Wiringa

Hyperspherical partial wave theory has been applied here in a new way in the calculation of the triple differential cross sections for the ionization of hydrogen atoms by electron impact at low energies for various equal-energy-sharing…

Atomic Physics · Physics 2009-11-07 J. N. Das , S. Paul , K. Chakrabarti

The form of the wave function at three-electron coalescence points is examined for several spin states using an alternative method to the usual Fock expansion. We find that, in two- and three-dimensional systems, the non-analytical nature…

Chemical Physics · Physics 2016-01-18 Pierre-François Loos , Nathaniel J. Bloomfield , Peter M. W. Gill

It is shown that the geometry of multi-electron threshold ionization in atoms depends on the initial configuration of bound electrons. The reason for this behavior is found in the stability properties of the classical fixed point of the…

Atomic Physics · Physics 2009-11-13 Agapi Emmanouilidou , Peijie Wang , Jan Michael Rost

The electron spectrum in a uniform nanowire with a hexagonal cross-section is calculated by means of a numerical diagonalization of the effective-mass Hamiltonian. Two basis sets are utilized. The wave-functions of low-lying states are…

Mesoscale and Nanoscale Physics · Physics 2021-01-19 I. A. Kokurin

Universal low-energy properties are studied for three identical bosons confined in two dimensions. The short-range pair-wise interaction in the low-energy limit is described by means of the boundary condition model. The wave function is…

Atomic Physics · Physics 2009-11-11 O. I. Kartavtsev , A. V. Malykh

On the basis of perturbation theory in fine structure constant alpha and the ratio of electron to muon masses we calculate one-loop vacuum polarization, electron vertex corrections, nuclear structure and recoil corrections to hyperfine…

High Energy Physics - Phenomenology · Physics 2015-09-01 A. P. Martynenko , A. A. Ulybin

A study of fermion nodes for spin-polarized states of a few-electron ions and molecules with $s,p,d$ one-particle orbitals is presented. We find exact nodes for some cases of two electron atomic and molecular states and also the first exact…

Other Condensed Matter · Physics 2009-11-10 Michal Bajdich , Lubos Mitas , Gabriel Drobný , Lucas K. Wagner

The three-body Schr\"odinger equation of the H$_2^+$ hydrogen molecular ion with Coulomb potentials is solved in perimetric coordinates using the Lagrange-mesh method. The Lagrange-mesh method is an approximate variational calculation with…

Quantum Physics · Physics 2015-06-16 Horacio Olivares Pilón , Daniel Baye

The hyperspherical harmonics (HH) provide a complete basis for the expansion of atomic wave functions, but even for two particles the number of harmonics for a given order is not trivial and, as the number of electrons increases, this…

Atomic Physics · Physics 2016-09-08 Anthony D. Klemm , Michel Fabre de la Ripelle , Sigurd Yves Larsen

A systematic method is presented for constructing effective Hamiltonians for general phonon-related structural transitions. The key feature is the application of group theoretical methods to identify the subspace in which the effective…

mtrl-th · Physics 2009-10-28 K. M. Rabe , U. V. Waghmare

The possibility to construct and parametrize the nonbonded interactions in atomistic force fields based on the valence electron structure of molecules is explored in this paper. Three different charge distribution models using simple…

Chemical Physics · Physics 2016-06-22 Nuria Plattner

We introduce a new type of Gutzwiller variational wavefunction for correlated electrons coupled to phonons, able to treat on equal footing electronic and lattice degrees of freedom. We benchmark the wavefunction in the infinite-$U$…

Strongly Correlated Electrons · Physics 2007-07-24 P. Barone , R. Raimondi , M. Capone , C. Castellani , M. Fabrizio

We present a basis-set-free approach to the variational quantum eigensolver using an adaptive representation of the spatial part of molecular wavefunctions. Our approach directly determines system-specific representations of qubit…

Quantum Physics · Physics 2021-01-05 Jakob S. Kottmann , Philipp Schleich , Teresa Tamayo-Mendoza , Alán Aspuru-Guzik

On the basis of variational method we study energy levels of pionic helium $(\pi-e-He)$ and kaonic helium $(K-e-He)$ with an electron in ground state and a meson in excited state with principal and orbital quantum numbers $n\sim l+1\sim…

High Energy Physics - Phenomenology · Physics 2023-11-21 V. I. Korobov , A. V. Eskin , A. P. Martynenko , F. A. Martynenko

Variational, nonrelativisitic energies have been calculated for the ground state ($^3P_g$) and the lowest quintuplet state ($^5S_u$) of the carbon atom, with wavefunctions expressed in the basis of symmetry-projected, explicitly correlated…

Chemical Physics · Physics 2020-09-21 Krzysztof Strasburger

Energy levels, wavelengths, magnetic-dipole and electric-quadrupole transition rates between the low-lying states are evaluated for W$^{51+}$ to W$^{54+}$ ions with $3d^n$ (n = 2 to 5) electronic configurations using an approach combining…

Atomic Physics · Physics 2018-01-10 M. S. Safronova , U. I. Safronova , S. G. Porsev , M. G. Kozlov , Yu. Ralchenko

The complex scaling method permits calculations of few-body resonances with the correct asymptotic behaviour using a simple box boundary condition at a sufficiently large distance. This is also valid for systems involving more than one…

Nuclear Theory · Physics 2008-11-26 E. Garrido , D. V. Fedorov , A. S. Jensen
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