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The toolbox for imaging molecules is well-equipped today. Some techniques visualize the geometrical structure, others the electron density or electron orbitals. Molecules are many-body systems for which the correlation between the…

We present an experimental study of the dissociative excitation in the collision of helium ions with nitrogen and oxygen molecules for collision energy of $0.7-10$ keV. Absolute emission cross sections are measured and reported for most…

Atomic Physics · Physics 2024-01-30 M. Gochitashvili , R. Lomsadze , R. Ya. Kezerashvili , I. Noselidze , M. Schulz

Using a merged beams apparatus we have measured the associative detachment (AD) reaction of ${\rm H}^- + {\rm H} \to {\rm H}_2 + e^-$ for relative collision energies up to \textit{E}$_{\rm{r}} \leq 4.83$ eV. These data extend above the 1 eV…

Atomic Physics · Physics 2015-05-30 K. A. Miller , H. Bruhns , J. Eliášek , M. Čížek , H. Kreckel , X. Urbain , D. W. Savin

The nonrelativistic energy together with relativistic and quantum electrodynamic corrections for all the molecular hydrogen isotopologues (D$_2$, T$_2$, HD, HT, DT) were evaluated without expansion in the electron-nucleus mass ratio. The…

Chemical Physics · Physics 2019-10-02 Mariusz Puchalski , Jacek Komasa , Anna Spyszkiewicz , Krzysztof Pachucki

R-matrix calculations combined with the adiabatic-nuclei-rotation and Coulomb-Born approximations are used to compute electron-impact rotational rate coefficients for two open-shell diatomic cations of astrophysical interest: the hydoxyl…

Solar and Stellar Astrophysics · Physics 2018-03-14 James R Hamilton , Alexandre Faure , Jonathan Tennyson

Cross sections and thermal rate coefficients are computed for electron-impact dissociative recombination and vibrational excitation/de-excitation of the N$^+_2$ molecular ion in its lowest six vibrational levels, for collision…

The polarization properties of the elastic electron scattering on H-like ions are investigated within the framework of the relativistic QED theory. The polarization properties are determined by a combination of relativistic effects and spin…

Atomic Physics · Physics 2021-11-24 D. M. Vasileva , K. N. Lyashchenko , A. B. Voitkiv , D. Yu , O. Yu. Andreev

The distribution function of electrons and phonons interacting with electrons in semiconductors and semimetals in high electric and quantizing magnetic fields as a result of the solution of the coupled system of equations for the density…

Condensed Matter · Physics 2007-05-23 T. M. Gassym

We report measurements on the H$^{+}$ + H$^{+}$ fragmentation channel following direct single-photon double ionization of neutral NH$_{3}$ at 61.5 eV, where the two photoelectrons and two protons are measured in coincidence using 3-D…

Soft x-ray radiation from the sun is responsible for the production of high energy photoelectrons in the D and E regions of the ionosphere, where they deposit most of their ionization energy. The photoelectrons created by this process are…

Chemical Physics · Physics 2022-11-21 Srimoyee Samaddar , Karthik Venkataramani , Justin Yonker , Scott. M. Bailey

In this work we consider a numerically solvable model of a two-electron diatomic molecule to study a recently proposed approximation based on the density-functional theory of so-called strictly correlated electrons (SCE). We map out the…

Strongly Correlated Electrons · Physics 2019-02-13 Luis Cort , Soeren Ersbak Bang Nielsen , Robert van Leeuwen

The low-energy electron-impact dissociation of molecular hydrogen has been a source of disagreement between various calculations and measurements for decades. Excitation of the ground state of H$_2$ into the dissociative $b ^3\Sigma_u^+$…

Plasma Physics · Physics 2021-02-24 Liam H. Scarlett , Dmitry V. Fursa , Jack Knol , Mark C. Zammit , Igor Bray

We present velocity map imaging data on intramolecular ion-pair dissociation (IPD) of carbonyl sulfide (OCS) induced by electron impact over the 20 eV to 45 eV energy range. Two distinct IPD pathways were resolved: CO+ + S- (threshold 14.8…

Atomic and Molecular Clusters · Physics 2026-04-21 Narayan Kundu , Soumya Ghosh , Dhananjay Nandi

Stereo-dynamics of dissociative electron attachments to CO_2 is investigated by the O^- anion velocity imaging experiments combined with the R-matrix calculations. ^2{\Pi}_g as a Feshbach resonant state of CO_2^- is confirmed to play roles…

Chemical Physics · Physics 2011-10-31 Bin Wu , Lei Xia , Yong-Feng Wang , Hong-Kai Li , Xian-Jin Zeng , Shan Xi Tian

We present first-principles calculations of the dI/dV characteristics of an H2 molecule sandwiched between Au and Pt electrodes in the presence of electron-phonon interactions. The conductance is found to decrease by a few percentage at…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 I. S. Kristensen , M. Paulsson , K. S. Thygesen , K. W. Jacobsen

Dissociative electron attachment (DEA) is one of the processes that shows a strong coupling between the nuclear and electronic degrees of freedom in a molecule. This coupling results in an efficient transformation of the kinetic energy of…

Chemical Physics · Physics 2024-04-17 Suvasis Swain , Akshay Kumar , E. Krishnakumar , Vaibhav S. Prabhudesai

On a dense energy grid reaching up to 75 meV electron collision energy the fragmentation angle and the kinetic energy release of neutral dissociative recombination fragments have been studied in a twin merged beam experiment. The anisotropy…

The two-photon decay in hydrogen-like ions is investigated within the framework of second order perturbation theory and Dirac's relativistic equation. Special attention is paid to the angular correlation of the emitted photons as well as to…

Atomic Physics · Physics 2014-10-23 P. Amaro , F. Fratini , S. Fritzsche , P. Indelicato , J. P. Santos , A. Surzhykov

The development of intense high-energy radiation sources and the improvement of techniques for detecting charged fragments have made possible experiments on multiple ionization of a molecule with registration of the momentum and charge of…

We study the electron-impact induced ionization of O$_{2}$ from threshold to 120 eV using the electron spectroscopy method. Our approach is simple in concept and embodies the ion source with a collision chamber and a mass spectrometer with…

Atomic Physics · Physics 2021-04-23 R. A. Lomsadze , M. R. Gochitashvili , R. Ya. Kezerashvili , M. Schulz