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Dissociation Energy of Molecular Hydrogen Isotopologues

Chemical Physics 2019-10-02 v1

Abstract

The nonrelativistic energy together with relativistic and quantum electrodynamic corrections for all the molecular hydrogen isotopologues (D2_2, T2_2, HD, HT, DT) were evaluated without expansion in the electron-nucleus mass ratio. The obtained results significantly improve the uncertainty of theoretical predictions, reaching a value below 1 MHz for the total dissociation energy. We observe good agreement with the experimental value for D2_2 and 3σ3\,\sigma discrepancy for the HD molecule, while no experimental values for the dissociation energy of molecules involving tritium have yet been obtained.

Keywords

Cite

@article{arxiv.1909.01985,
  title  = {Dissociation Energy of Molecular Hydrogen Isotopologues},
  author = {Mariusz Puchalski and Jacek Komasa and Anna Spyszkiewicz and Krzysztof Pachucki},
  journal= {arXiv preprint arXiv:1909.01985},
  year   = {2019}
}

Comments

7 pages. arXiv admin note: text overlap with arXiv:1812.02980