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Spin-1/2 chains with alternating antiferromagnetic (AF) and ferromagnetic (FM) couplings exhibit quantum entanglement like the integer-spin Haldane chains and might be similarly utilized for quantum computations. Such alternating AF-FM…

Strongly Correlated Electrons · Physics 2020-12-09 Shang Gao , Ling-Fang Lin , Andrew F. May , Binod K. Rai , Qiang Zhang , Elbio Dagotto , Andrew D. Christianson , Matthew B. Stone

Recent theoretical and experimental work suggest that the honeycomb cobaltates, initially proposed as candidate Kitaev quantum magnets, are in fact described by a pseudospin-$1/2$ easy-plane spin Hamiltonian with nearest neighbor…

Rare-earth (RE) based honeycomb-lattice materials with strong spin-orbit coupled Jeff=1/2 moments have attracted great interest as a platform to realize Kitaev quantum spin liquid (QSL) state. Herein, we report the discovery of a new family…

Strongly Correlated Electrons · Physics 2023-05-23 Andi Liu , Fangyuan Song , Zhaohu Li , Malik Ashtar , Yuqi Qin , Dingjun Liu , Zhengcai Xia , Jingxin Li , Zhitao Zhang , Wei Tong , Hanjie Guo , Zhaoming Tian

Magnetic moments arranged at the corners of a honeycomb lattice are predicted to form a novel state of matter, Kitaev quantum spin liquid, under the influence of frustration effects between bond-dependent Ising interactions. Some layered…

Strongly Correlated Electrons · Physics 2022-03-09 Sean K. Takahashi , Jiaming Wang , Alexandre Arsenault , Mykola Abramchuk , Fazel Tafti , Philip M. Singer , Takashi Imai

A Hubbard model at half-filling on an anisotropic triangular lattice has been proposed as the minimal model to describe conducting layers of $\kappa-(BEDT-TTF)_2X$ organic materials. The model interpolates between the square lattice and…

Superconductivity · Physics 2016-04-20 Shan-Wen Tsai , J. B. Marston

We analyze powder-averaged inelastic neutron scattering and magnetization data for the distorted honeycomb compound Cu$_5$SbO$_6$ using a first-order dimer expansion calculation and quantum Monte Carlo simulations. We show that, in contrast…

We study the ground-state (gs) phase diagram of the frustrated spin-1/2 $J_{1}$-$J_{2}$-$J_{3}$ antiferromagnet with $J_{2} = J_{3} =\kappa J_1$ on the honeycomb lattice, using coupled-cluster theory and exact diagonalization methods. We…

Strongly Correlated Electrons · Physics 2011-07-11 D. J. J. Farnell , R. F. Bishop , P. H. Y. Li , J. Richter , C. E. Campbell

We investigate the ground-state and finite-temperature properties of the bond-random $s=1/2$ Heisenberg model on a honeycomb lattice with frustrated nearest- and next-nearest-neighbor antiferromagnetic interactions, $J_1$ and $J_2$, by the…

Strongly Correlated Electrons · Physics 2018-10-24 Kazuki Uematsu , Hikaru Kawamura

Motivated by recent experiments on Bi$_3$Mn$_4$O$_{12}$(NO$_3$), we study a frustrated $J_1$-$J_2$ Heisenberg model on the two dimensional (2D) honeycomb lattice. The classical $J_1$-$J_2$ Heisenberg model on the two dimensional (2D)…

Strongly Correlated Electrons · Physics 2013-05-29 A. Mulder , R. Ganesh , L. Capriotti , A. Paramekanti

SrRu2O6 is a layered honeycomb lattice material with an extraordinarily high magnetic ordering temperature. We investigated this material using density functional calculations. We find that the energy scales for moment formation and…

Materials Science · Physics 2015-06-17 David J. Singh

We investigate the role of electron correlation in the electronic structure of honeycomb lattice Li$_2$RuO$_3$ using photoemission spectroscopy and band structure calculations. Monoclinic Li$_2$RuO$_3$ having Ru network as honeycomb lattice…

Strongly Correlated Electrons · Physics 2023-01-24 Sakshi Bansal , Asif Ali , B. H. Reddy , Ravi Shankar Singh

We investigate the lattice dynamics in the spin-1/2 frustrated kagome compound herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$ by a combination of infrared spectroscopy measurements and ab initio density functional theory calculations, and provide…

Strongly Correlated Electrons · Physics 2020-04-29 Ying Li , A. Pustogow , M. Bories , P. Puphal , C. Krellner , M. Dressel , Roser Valenti

We explore the magnetic properties of isolated a-b planes of trinuclear organometallic crystals, Mo3S7(dmit)3, in which an interplay of strong electronic correlations and spin molecular-orbital coupling (SMOC) occurs. The magnetic…

Strongly Correlated Electrons · Physics 2018-11-01 J. Merino , A. C. Jacko , A. L. Khosla , A. Ralko , B. J. Powell

The temperature-magnetic-field phase diagram of the mixed honeycomb triangular lattice system K$_{2}$Mn$_{3}$(VO$_{4}$)$_{2}$CO$_{3}$ is investigated by means of magnetization, heat capacity and neutron scattering measurements. The results…

The magnetic phase diagram and the thermodynamic properties of a square lattice containing antiferromagnetically coupled spin-1/2 triangles are studied. A Heisenberg Hamiltonian with three strong intra-triangle exchange coupling constants…

Strongly Correlated Electrons · Physics 2009-10-31 Stefan Wessel , Stephan Haas

We delineate quantum magnetism in the strongly spin-orbit coupled, distorted honeycomb-lattice antiferromagnet BiYbGeO$_{5}$. Our magnetization and heat capacity measurements reveal that its low-temperature behavior is well described by an…

Novel ground states might be realized in honeycomb lattices with strong spin-orbit coupling. Here we study the electronic structure of ${\alpha}$-RuCl$_3$, in which the Ru ions are in a d5 configuration and form a honeycomb lattice, by…

Strongly Correlated Electrons · Physics 2016-09-21 A. Koitzsch , C. Habenicht , E. Mueller , M. Knupfer , B. Buechner , H. Kandpal , J. van den Brink , D. Nowak , A. Isaeva , Th. Doert

We show that the honeycomb Heisenberg antiferromagnet with $J_1/2=J_2=J_3$, where $J_{1/2/3}$ are first-, second- and third-neighbour couplings respectively, forms a classical spin liquid with pinch-point singularities in the structure…

Strongly Correlated Electrons · Physics 2016-10-13 J. Rehn , Arnab Sen , Kedar Damle , R. Moessner

We show that the topological Kitaev spin liquid on the honeycomb lattice is extremely fragile against the second-neighbor Kitaev coupling $K_2$, which has recently been shown to be the dominant perturbation away from the nearest-neighbor…

Strongly Correlated Electrons · Physics 2015-12-08 Ioannis Rousochatzakis , Johannes Reuther , Ronny Thomale , Stephan Rachel , N. B. Perkins

We study the magnetic phase diagram of the $J_1$--$J_2$ Heisenberg antiferromagnet on a honeycomb lattice at the strongly frustrated point $J_2/J_1=1/2$ using large-scale Monte Carlo simulations. At low temperatures we find three different…

Strongly Correlated Electrons · Physics 2014-06-24 H. D. Rosales , D. C. Cabra , C. A. Lamas , P. Pujol , M. E. Zhitomirsky