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Two-photon optical transitions combined with long-range dipole-dipole interactions can be used for the coherent manipulation of collective metastable states composed of different atoms. We show that it is possible to induce optical…

Quantum Physics · Physics 2007-05-23 M. D. Lukin , P. R. Hemmer

We propose a scheme of optical pumping by which a system of atoms coupled to harmonic oscillators is driven to an entangled steady state through the atomic spontaneous emission. It is shown that the optical pumping can be tailored so that…

Quantum Physics · Physics 2011-01-18 Jaeyoon Cho , Sougato Bose , M. S. Kim

The present work is focused on theoretical and experimental study of localised levels in organic materials suitable for light-emitting devices and field effect transistors by means of thermal techniques. In our work we focused on low…

Other Condensed Matter · Physics 2007-05-23 M. Prelipceanu , O. S. Prelipceanu , O. G. Tudose , S. Schrader

The generation of nonclassical light states bears a paramount importance in quantum optics and is largely relying on the interaction between intense laser pulses and nonlinear media. Recently, electron beams, such as those used in ultrafast…

Optics · Physics 2025-09-23 Valerio Di Giulio , F. Javier García de Abajo

A new perturbative approach to canonical equation-of-motion coupled-cluster theory is presented using coupled-cluster perturbation theory. A second-order M{\o}ller-Plesset partitioning of the Hamiltonian is used to obtain the well known…

Chemical Physics · Physics 2015-07-09 Jason N. Byrd , Varun Rishi , Ajith Perera , Rodney J. Bartlett

Organic heterojunction solar cells are analyzed within a minimal model that includes the essential physical features of such systems. The dynamical properties of this model, calculated using a master equation approach, account for the…

Materials Science · Physics 2011-11-11 Mario Einax , Marcel Dierl , Abraham Nitzan

The physics of optical pumping of semiconductor electrons in the ferromagnet/semiconductor hybrids is discussed. Optically oriented semiconductor electrons detect the magnetic state of the ferromagnetic film. In turn, the ferromagnetism of…

Mesoscale and Nanoscale Physics · Physics 2011-08-15 V. L. Korenev

The study of isolated defects in solids is a natural target for classical or quantum embedding methods that treat the defect at a high level of theory and the rest of the solid at a lower level of theory. Here, in the context of…

Materials Science · Physics 2023-01-25 Bryan T. G. Lau , Brian Busemeyer , Timothy C. Berkelbach

Adaptive finite elements are the method of choice for accurate simulations of optical components. However as shown recently by Bienstman et al. many finite element mode solvers fail to compute the propagation constant's imaginary part of a…

Optics · Physics 2009-05-28 L. Zschiedrich , S. Burger , J. Pomplun , F. Schmidt

Achieving and controlling strong light-matter interactions in many-body systems is of paramount importance both for fundamental understanding and potential applications. In this paper we demonstrate both experimentally and theoretically how…

Mesoscale and Nanoscale Physics · Physics 2016-12-26 Pierre Fauche , Christian Gebhardt , Maxim Sukharev , Renaud A. L. Vallee

Partial atomic charges are a useful and intuitive concept for understanding molecular properties and chemical reaction mechanisms, showing how changes in molecular geometry can affect the flow of electronic charge within a molecule.…

Chemical Physics · Physics 2022-01-14 Ryan J. MacDonell , Serguei Patchkovskii , Michael S. Schuurman

Li2GeO3, a ternary electrolyte compound of Li+-based battery, presents the unusual essential properties. The main features are thoroughly explored from the first-principles calculations. The concise pictures, the critical orbital…

Polymer based organic photovoltaic (OPV) technology offers a relatively inexpensive option for solar energy conversion provided its efficiency increases beyond the current level (6-7%) along with significant improvements in operational…

Materials Science · Physics 2015-03-17 Biswajit Ray , Pradeep R. Nair , Muhammad A. Alam

Using a master-equation approach for the description of coherent and incoherent dynamics in `artificial atoms and molecules', we present a theoretical analysis of situations where intense laser fields lead to pronounced renormalizations of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Ulrich Hohenester , Filippo Troiani , Elisa Molinari

In this paper we present a detailed theory of the triplet states of oligoacenes containing up to seven rings, i.e., starting from naphthalene all the way up to heptacene. In particular, we present results on the optical absorption from the…

Chemical Physics · Physics 2014-10-24 Himanshu Chakraborty , Alok Shukla

The development of optical power limiting materials is important to protect individuals or materials from intense laser irradiation. The photophysical behavior of Os(II) polypyridinyl complexes having aromatic hydrocarbon terpyridyl ligands…

Chemical Physics · Physics 2015-03-03 Shashwat Alok , Jason Gunson

We present an analytic ansatz to find the effective electrostatic potential and Coulomb correlations in multicenter problems, specifically homogeneous and doped clusters of metal atoms. The approach is based on a quasi-classical…

Chemical Physics · Physics 2007-05-23 F. Despa , R. S. Berry

The observation and electrical manipulation of infrared surface plasmons in graphene have triggered a search for similar photonic capabilities in other atomically thin materials that enable electrical modulation of light at visible and…

Mesoscale and Nanoscale Physics · Physics 2017-02-08 F. Javier Garcia de Abajo , Alejandro Manjavacas

Optical properties of a plasmonic nano-antenna made of two metallic nanospheroids (prolate or oblate) are investigated analytically in quasistatic approximation. It is shown that in clusters of two nanospheroids, three types of plasmonic…

Optics · Physics 2010-10-28 D. V. Guzatov , V. V. Klimov

Controlling light-matter interactions is emerging as a powerful strategy to enhance the performance of organic light-emitting diodes (OLEDs). By embedding the emissive layer in planar microcavities or other modified optical environments,…

Materials Science · Physics 2026-02-06 Olli Siltanen , Kimmo Luoma , Konstantinos S. Daskalakis