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Optical response of free-electron gas leads to inherent nonlinear optical behaviour of nanostructured plasmonic materials enabled via both strong local field enhancements and inherent complex electron dynamics. We present a comprehensive…

Understanding how light interacts at the nanoscale with metals, semiconductors, or ordinary dielectrics is pivotal if one is to properly engineer nano-antennas, filters and, more generally, devices that aim to harness the effects of new…

Rigorous electrodynamical simulations based on the nonlinear Drude model are performed to investigate the influence of strong coupling on high harmonic generation by periodic metal gratings. It is shown that a thin dispersive material with…

Mesoscale and Nanoscale Physics · Physics 2019-08-13 Elena Drobnyh , Ruth Pachter , Maxim Sukharev

We show a new path to {\epsilon}~0 materials without resorting to metal-based metamaterial composites. A medium that can be modeled using Lorentz oscillators usually displays {\epsilon}=0 crossing points, e.g. {\epsilon}=0 at…

Optics · Physics 2013-05-29 M. A. Vincenti , D. de Ceglia , A. Ciattoni , M. Scalora

In this article, we develop a classical electrodynamic theory to study the optical nonlinearities of metallic nanoparticles. The quasi-free electrons inside the metal are approximated as a classical Coulomb-interacting electron gas, and…

Optics · Physics 2015-05-13 Yong Zeng , Walter Hoyer , Jinjie Liu , Stephan W. Koch , Jerome V. Moloney

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì

We study second and third harmonic generation in centrosymmetric semiconductors at visible and UV wavelengths in bulk and cavity environments. Second harmonic generation is due to a combination of symmetry breaking, the magnetic portion of…

Plasmonic waveguides provide an integrated platform to develop efficient nanoscale ultrafast photonic devices. Theoretical models that describe nonlinear optical phenomena in plasmonic waveguides, usually, only incorporate bulk…

We have conducted a theoretical study of harmonic generation from a silver grating having slits filled with GaAs. By working in the enhanced transmission regime, and by exploiting phase-locking between the pump and its harmonics, we…

Optics · Physics 2015-05-20 M. A. Vincenti , D. de Ceglia , V. Roppo , M. Scalora

Resonant structures in modern nanophotonics are non-Hermitian (leaky and lossy), and support quasinormal modes. Moreover, contemporary cavities frequently include 2D materials to exploit and resonantly enhance their nonlinear properties or…

Computational Physics · Physics 2023-01-25 Thomas Christopoulos , Emmanouil E. Kriezis , Odysseas Tsilipakos

The plasmon-enhanced second harmonic generation in the subwavelength neutral metal cubic nanoparticles is calculated for the first time in the hydrodynamic and cold plasma approximations. The theory is developed that takes into account all…

Mesoscale and Nanoscale Physics · Physics 2016-02-15 S. V. Fomichev , A. M. Bratkovsky

Optical properties of periodic arrays of nanoholes of a triangular shape with experimentally realizable parameters are examined in both linear and nonlinear regimes. Utilizing fully vectorial three-dimensional approach based on the…

Mesoscale and Nanoscale Physics · Physics 2020-03-18 Elena Drobnyh , Maxim Sukharev

The search for miniaturized components for nonlinear optical processes needs a way to overcome the efficiency loss due to the effective size reduction of the active medium. We investigate here a combination of a nanosized nonlinear…

We show that second harmonic generation can be enhanced by Fano resonant coupling of asymmetric plasmonic metal nanostructures. We develop a theoretical model examining the effects of electromagnetic interaction between two metal…

Notwithstanding its long history, the study of nonlinear optics from metal surfaces is still an active field of research. For instance, in view of the presence of absorption questions remain concerning the possibility of significantly…

Nanophotonics research has focused recently on the ability of non-linear optical processes to mediate and transform optical signals in a myriad of novel devices, including optical modulators, transducers, color filters, photodetectors,…

Monolayer transition metal dichalcogenides, coupled to metal plasmonic nanocavities, have recently emerged as new platforms for strong light-matter interactions. These systems are expected to have nonlinear optical properties that will…

We report comparative experimental and theoretical studies of second and third harmonic generation from a 20nm-thick indium tin oxide layer in proximity of the epsilon-near-zero condition. Using a tunable OPA laser we record both spectral…

Our theoretical examination of second and third harmonic generation from metal-based nanostructures predicts that nonlocal and quantum tunneling phenomena can significantly exceed expectations based solely on local, classical…

Second harmonic generation is a powerful tool directly connected to the symmetry of materials. Phase transitions, lattice rotations or electromagnetic coupling in multiferroic compounds can be revealed by using second harmonic…

Optics · Physics 2010-01-11 Pablo Molina , Mariola O Ramirez , Basilio J. Garcia , Luisa E. Bausa
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