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We have measured near normal incidence far infrared (FIR) reflectivity spectra of a single crystal of TbMnO3 from 10K to 300K in the spectral range of 50 cm$^{-1}$ to 700 cm$^{-1}$. Fifteen transverse optic (TO) and longitudinal optic (LO)…

Materials Science · Physics 2015-05-13 Pradeep Kumar , Surajit Saha , C. R. Serrao , A. K. Sood , C. N. R. Rao

The reflectivity $R (\omega)$ of both the $ab$ plane and the c axis of two single crystals of La$_{1.875}$Ba$_{0.125-y}$Sr$_{y}$CuO$_4$ has been measured down to 5 cm$^{-1}$, using coherent synchrotron radiation below 30 cm$^{-1}$. For $y$…

Superconductivity · Physics 2009-11-11 M. Ortolani , P. Calvani , S. Lupi , U. Schade , A. Perla , M. Fujita , K. Yamada

The infrared reflectivity of a $\rm La_{0.67}Ca_{0.33}MnO_3$ single crystal is studied over a broad range of temperatures (78-340 K), magnetic fields (0-16 T), and wavenumbers (20-9000 cm$^{-1}$). The optical conductivity gradually changes…

Strongly Correlated Electrons · Physics 2019-08-17 A. V. Boris , N. N. Kovaleva , A. V. Bazhenov , P. J. M. van Bentum , Th. Rasing , S-W. Cheong , A. V. Samoilov , N. -C. Yeh

Optical properties of single-crystal monoclinic CuO in the range 70 - 6000 \cm were studied at temperatures from 7 to 300 K. Normal reflection spectra were obtained from the (001) and (010) crystal faces thus giving for the first time…

Strongly Correlated Electrons · Physics 2009-10-31 A. B. Kuz'menko , D. van der Marel , P. J. M. van Bentum , E. A. Tishchenko , C. Presura , A. A. Bush

The magnetic susceptibility between 1.5 and 800 K, the infrared reflectivity at room temperature and the temperature dependence of the dielectric constant at mm-wavelengths are reported for single crystalline BiFeO3. A well developed…

Strongly Correlated Electrons · Physics 2010-07-22 Jun Lu , M Schmidt , P Lunkenheimer , A Pimenov , A A Mukhin , V D Travkin , A Loidl

X-ray scattering by multiferroic LuFe2O4 is reported. Below 320 K, superstructure reflections indicate an incommensurate charge order with propagation close to (1/3,1/3,3/2). The corresponding charge configuration, also found by electronic…

Reflection and transmission as a function of temperature (5--300 K) have been measured on single crystals of the multiferroic compound FeTe$_{2}$O$_{5}$Br utilizing light spanning the far infrared to the visible portions of the…

Strongly Correlated Electrons · Physics 2015-06-12 K. H. Miller , X. S. Xu , H. Berger , V. Craciun , X. Xi , C. Martin , G. L. Carr , D. B. Tanner

Infrared reflection and transmission as a function of temperature have been measured on single crystals of Cu$_{3}$Bi(SeO$_{3}$)$_{2}$O$_{2}$Cl. The complex dielectric function and optical properties along all three principal axes of the…

Materials Science · Physics 2015-06-05 K. H. Miller , P. W. Stephens , C. Martin , E. Constable , R. A. Lewis , H. Berger , G. L. Carr , D. B. Tanner

We performed elastic neutron scattering measurements on the charge- and magnetically-ordered multiferroic material LuFe(2)O(4). An external electric field along the [001] direction with strength up to 20 kV/cm applied at low temperature…

Materials Science · Physics 2010-04-22 Jinsheng Wen , Guangyong Xu , Genda Gu , S. M. Shapiro

The reflectivity of single-crystalline CoO has been studied by optical spectroscopy for wave numbers ranging from 100 to 28,000\wn and for temperatures 8 $< T <$ 325 K\@. A splitting of the cubic IR-active phonon mode on passing the…

Strongly Correlated Electrons · Physics 2009-01-20 Ch. Kant , T. Rudolf , F. Schrettle , F. Mayr , J. Deisenhofer , P. Lunkenheimer , M. V. Eremin , A. Loidl

We present single-crystal neutron diffraction measurements on multiferroic LuFe2O4 showing phase transitions at 240 and 175 K. Magnetic reflections are observed below each transition indicating that the magnetic interactions in LuFe2O4 are…

Strongly Correlated Electrons · Physics 2009-11-13 A. D. Christianson , M. D. Lumsden , M. Angst , Z. Yamani , W. Tian , R. Jin , E. A. Payzant , S. E. Nagler , B. C. Sales , D. Mandrus

We discuss the first infrared reflectivity measurement on a BiFeO3 single crystal between 5 K and room temperature. The 9 predicted ab-plane E phonon modes are fully and unambiguously determined. The frequencies of the 4 A1 c-axis phonons…

Materials Science · Physics 2011-11-10 R. P. S. M. Lobo , R. L. Moreira , D. Lebeugle , D. Colson

Temperature-dependent FAR-infrared reflectivity spectra of partially ordered magnetodielectric La2CoMnO6 is presented, from room temperature up to 675 K. A clear first-ordered structural phase transition (SPT) from a monoclinic structure…

Materials Science · Physics 2018-02-22 R. X. Silva , A. Nonato , R. L. Moreira , R. M. Almeida , C. W. A. Paschoal

Reflection and transmission as a function of temperature have been measured on a single crystal of the magnetoelectric ferrimagnetic compound Cu$_{2}$OSeO$_{3}$ utilizing light spanning the far infrared to the visible portions of the…

Materials Science · Physics 2015-05-19 K. H. Miller , X. S. Xu , H. Berger , E. S. Knowles , D. J. Arenas , M. W. Meisel , D. B. Tanner

The structural features of the charge ordering states in LuFe2O4 are characterized by in-situ cooling TEM observations from 300K down to 20K. Two distinctive structural modulations, a major q1= (1/3, 1/3, 2) and a weak q2=q1/10 + (0, 0,…

Materials Science · Physics 2009-11-13 Y. Zhang , H. X. Yang , C. Ma , H. F. Tian , J. Q. Li *

We report an infrared reflection spectroscopy study of La$_{1/2}$Ca$_{1/2}$MnO$_3$ over a broad frequency range and temperature interval which covers the transitions from the high temperature paramagnetic to ferromagnetic and, upon further…

Strongly Correlated Electrons · Physics 2009-11-10 A. P. Litvinchuk , M. N. Iliev , M. Pissas , C. W. Chu

Polarized infrared reflectivity spectra of a (110)-oriented TbScO3 single crystal plate were measured down to 10 K. The number of observed polar phonons active along the crystallographic c axis at low temperatures is much higher than…

We provide a detailed study of the reflectivity of multiferroic TbMnO_3 for wave numbers from 40 cm^{-1} to 1000 cm^{-1} and temperatures 5 K < T < 300 K. Excitations are studied for polarization directions E || a, the polarization where…

Strongly Correlated Electrons · Physics 2010-01-22 M. Schmidt , Ch. Kant , T. Rudolf , F. Mayr , A. A. Mukhin , A. M. Balbashov , J. Deisenhofer , A. Loidl

Neutron diffraction measurements on multiferroic LuFe2O4 show changes in the antiferromagnetic (AFM) structure characterized by wavevector q = (1/3 1/3 1/2) as a function of electric field cooling procedures. The increase of intensity from…

Strongly Correlated Electrons · Physics 2011-11-09 A. M. Mulders , M. Bartkowiak , J. R. Hester , E. Pomjakushina , K. Conder

Microstructure properties, phase transitions, and charge ordering in the LuFe2O4 materials have been extensively investigated by means of transmission electron microscopy (TEM). The (001) twins as a common defect frequently appear in the…

Strongly Correlated Electrons · Physics 2007-05-23 Y. Zhang , H. X. Yang , C. Ma , H. F. Tian , J. Q. Li *
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