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We present a study of the structural phase transition, mechanical and thermodynamic properties of UO$_{2}$ by means of the local density approximation (LDA)$+U$ approach. A phase transition pressure of 40 GPa, which agrees well with the…

Strongly Correlated Electrons · Physics 2013-09-25 Bao-Tian Wang , Ping Zhang , Raquel Lizárraga , Igor Di Marco , Olle Eriksson

The elastic, thermodynamic, and electronic properties of fluorite RuO_2 under high pressure are investigated by plane-wave pseudopotential density functional theory. The optimized lattice parameters, elastic constants, bulk modulus, and…

Materials Science · Physics 2017-08-23 Z. J. Yang , A. M. Guo , Y. D. Guo , J. Li , Z. Wang , Q. Liu , R. F. Linghu , X. D. Yang

The mechanical properties, electronic structure and phonon dispersion of ground state ThO$_{2}$ as well as the structure behavior up to 240 GPa are studied by using first-principles density-functional theory. Our calculated elastic…

Materials Science · Physics 2015-05-14 Baotian Wang , Hongliang Shi , Weidong Li , Ping Zhang

The structural, electronic, mechanical, optical, thermodynamic properties of plutonium monoxide monohydride (PuOH) are studied by density-functional calculations within the framework of LDA/GGA and LDA/GGA+U.From the total energy…

Materials Science · Physics 2020-01-14 Ruizhi Qiu , Haiyan Lu , Bingyun Ao , Tao Tang , Piheng Chen

The electronic structure and properties of PuO$_{2}$ and Pu$_{2}$O$_{3}$ have been studied from first principles by the all-electron projector-augmented-wave (PAW) method. The local density approximation (LDA)+$U$ and the generalized…

Materials Science · Physics 2007-12-24 Bo Sun , Ping Zhang , Xian-Geng Zhao

Plutonium dihydride and trihydride show strikingly similar crystal structures when viewed as close-packed Pu planes with ABC and AB stacking, respectively. The similarity serves as a framework for density functional theory (DFT)…

Materials Science · Physics 2013-07-03 Sven P. Rudin

The structural behavior of UO2 under high pressure up to 300GPa has been studied by first-principles calculations with LSDA+U approximation. The results show that a pressure-induced structural transition to the cotunnite-type (orthorhombic…

Materials Science · Physics 2007-05-23 H. Y. Geng , Y. Chen , Y. Kaneta , M. Kinoshita

In this work, the ground-state properties of the platinum isotopic chain, 160-238Pt, are studied within the covariant density functional theory. The calculations are carried out for a large number of even-even Pt isotopes by using the…

Nuclear Theory · Physics 2019-11-20 Younes El Bassem , Mostafa Oulne

We have performed a systematic first-principles investigation to calculate the structural, electronic, and magnetic properties of PbCrO$_{3}$, CrPbO$_{3}$ as well as their equiproportional combination. The local density approximation…

Strongly Correlated Electrons · Physics 2012-01-25 Bao-Tian Wang , Wen Yin , Wei-Dong Li , Fangwei Wang

Plutonium (Pu), in which the 5$f$ valence electrons always wander the boundary between localized and itinerant states, exhibits quite complex crystal structures and unprecedentedly anomalous properties with respect to temperature and…

Strongly Correlated Electrons · Physics 2020-03-26 Li Huang , Haiyan Lu

Formation Gibbs free energy of point defects and oxygen clusters in uranium dioxide at high-pressure high-temperature conditions are calculated from first principles, using the LSDA+U approach for the electronic structure and the Debye…

Materials Science · Physics 2011-12-21 Hua Y. Geng , Hong X. Song , K. Jin , S. K. Xiang , Q. Wu

The physical properties of plutonium and plutonium-based intermetallic compounds are extremely sensitive to temperature, pressure, and chemical alloying. A celebrated example is the high-temperature $\delta$ phase plutonium, which can be…

Strongly Correlated Electrons · Physics 2024-05-15 Li Huang , Haiyan Lu

In this work using the density functional theory (DFT), we have studied the structural, electronic and magnetic properties of uranium dioxide with antiferromagnetic 1k-, 2k-, and 3k-order structures. Ordinary approximations in DFT, such as…

Materials Science · Physics 2020-08-25 Samira Sheykhi , Mahmoud Payami

The electronic structure of fluorite crystals are studied by means of density functional theory within the local density approximation for the exchange correlation energy. The ground-state electronic properties, which have been calculated…

Materials Science · Physics 2011-08-01 Emiliano Cadelano , Giancarlo Cappellini

Using density functional theory (DFT), the structural, mechanical, electronic, thermal, and optical properties of Hf2AB (A = Pb, Bi) borides were studied, considering the pressure effect up to 50 GPa. The lattice constants were found to be…

Materials Science · Physics 2022-12-20 M. S. Hossain , N. Jahan , M. M. Hossain , M. M. Uddin , M. A. Ali

Using density-functional theory (DFT) we calculate the Gibbs free energy to determine the lowest-energy structure of a RuO_2(110) surface in thermodynamic equilibrium with an oxygen-rich environment. The traditionally assumed stoichiometric…

Materials Science · Physics 2009-11-07 Karsten Reuter , Matthias Scheffler

By LDA+U method with spin-orbit coupling (LDA+U+SO) the magnetic state and electronic structure have been investigated for plutonium in \delta and \alpha phases and for Pu compounds: PuN, PuCoGa5, PuRh2, PuSi2, PuTe, and PuSb. For metallic…

Strongly Correlated Electrons · Physics 2007-05-23 A. O. Shorikov , A. V. Lukoyanov , M. A. Korotin , V. I. Anisimov

Plutonium's phase diagram is host to complex structures and interactions that make the description of its ground state properties elusive. Using all-electron density functional theory, we study the thermodynamic properties of $\alpha$-Pu.…

\textit{Ab initio} random structure searching based on density functional theory is used to determine the ground-state structures of ice at high pressures. Including estimates of lattice zero-point energies, ice is found to adopt three…

Other Condensed Matter · Physics 2013-05-29 Jeffrey M. McMahon

We develop a new implementation of the Gutzwiller approximation (GA) and interface it with the local density approximation (LDA). This formulation enables us to study complex $4f$ and $5f$ systems. We perform calculations of praseodymium…

Strongly Correlated Electrons · Physics 2015-05-11 Nicola Lanatà , Yongxin Yao , Cai-Zhuang Wang , Kai-Ming Ho , Gabriel Kotliar
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