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The properties of a semiflexible polymer with fixed ends exposed to oscillatory shear flow are investigated by simulations. The two-dimensionally confined polymer is modeled as a linear bead-spring chain, and the interaction with the fluid…

Soft Condensed Matter · Physics 2021-12-14 Antonio Lamura , Roland G. Winkler

We investigate the tight packing of nematic polymers inside a confining hard sphere. We model the polymer {\sl via} the continuum Frank elastic free energy augmented by a simple density dependent part as well as by taking proper care of the…

Soft Condensed Matter · Physics 2010-05-05 Daniel Svenšek , Gregor Veble , Rudolf Podgornik

We study the dynamics and conformation of polymers composed by active monomers. By means of Brownian dynamics simulations we show that when the direction of the self-propulsion of each monomer is aligned with the backbone, the polymer…

Soft Condensed Matter · Physics 2018-11-28 Valentino Bianco , Emanuele Locatelli , Paolo Malgaretti

Semiflexible polymers in concentrated lyotropic solution are studied within a bead-spring model by molecular dynamics simulations, focusing on the emergence of a smectic A phase and its properties. We systematically vary the density of the…

Soft Condensed Matter · Physics 2019-01-28 Andrey Milchev , Arash Nikoubashman , Kurt Binder

We probe, using the Surface Forces Apparatus, the thermal response of poly(N-isopropylacrylamide) (PNIPAM) brushes of various grafting densities, grown from plasma-activated mica by means of surface-initiated polymerization. We thus show…

Soft Condensed Matter · Physics 2009-10-09 Ibrahim Bou Malham , Lionel Bureau

We present a molecular dynamics study of the flow of rigid spherical nanoparticles in a simple fluid. We evaluate the viscosity of the dispersion as a function of shear rate and nanoparticle volume fraction. We observe shear thinning…

Soft Condensed Matter · Physics 2020-07-15 Ekin Küçüksönmez , James Servantie

Friction between ring-polymer brushes at melt densities sliding past each other are studied using extensive course-grained molecular dynamics simulations and scaling arguments, and the results are compared to the friction between…

Soft Condensed Matter · Physics 2015-05-20 A. Erbas , J. Paturej

We study the conformations of polymer chains in a poor solvent, with and without bending rigidity, by means of a simple statistical mechanics model. This model can be exactly solved for chains of length up to N=55 using exact enumeration…

Statistical Mechanics · Physics 2007-11-26 Anthony J. Guttmann , Jesper L. Jacobsen , Iwan Jensen , Sanjay Kumar

We develop a general analysis of the diffusive dynamics of polydisperse polymers in the presence of chemical potential gradients, within the context of the tube model (with all species entangled). We obtain a set of coupled dynamical…

Soft Condensed Matter · Physics 2009-11-07 I. Pagonabarraga , M. E. Cates

In this paper, we present a theory to efficiently deal with mechanical properties of heterogeneous polymer chain in free space and the central problem is to evaluate the diffusion equation and orientation-orientation correlation function,…

Biological Physics · Physics 2019-11-05 Ming Li , Jizeng Wang

Inspired by recent experiments on chromosomal dynamics, we introduce an exactly solvable model for the interaction between a flexible polymer and a set of motor-like enzymes. The enzymes can bind and unbind to specific sites of the polymer…

Soft Condensed Matter · Physics 2019-04-03 Stefanie Put , Takahiro Sakaue , Carlo Vanderzande

We study the conformational properties of complex polymer macromolecules, consisting in general of $n$ subsequently connected chains (blocks) of different lengths and distinct chemical structure. Depending on the solvent conditions, the…

Soft Condensed Matter · Physics 2019-12-03 V. Blavatska , K. Haydukivska

The freely rotating chain is one of the classic discrete models of a polymer in dilute solution. It consists of a broken line of N straight segments of fixed length such that the angle between adjacent segments is constant and the N-1…

Probability · Mathematics 2017-11-15 Philip Kilanowski , Peter March , Marko Samara

Polymer brushes are attractive as surface coatings for a wide range of applications, from fundamental research to everyday life, and also play important roles in biological systems. How colloids (e.g., functional nanoparticles, proteins,…

Soft Condensed Matter · Physics 2025-04-07 Mikhail Y. Laktionov , Ekaterina B. Zhulina , Leonid Klushin , Ralf P. Richter , Oleg V. Borisov

We report on an extensive study of craze formation in glassy polymers. Molecular dynamics simulations of a coarse-grained bead-spring model were employed to investigate the molecular level processes during craze nucleation, widening, and…

Materials Science · Physics 2009-11-10 Joerg Rottler , Mark O. Robbins

Structure and dynamics of an active polymer on a smooth cylindrical surface are studied by Brownian dynamics simulations. The effect of active force on the polymer adsorption behavior and the combined effect of chain mobility, length N,…

Soft Condensed Matter · Physics 2024-08-21 Chen Shen , Chao-ran Qin , Tian-liang Xu , Kang Chen , Wen-de Tian

Molecular dynamics simulations are used to investigate the conformations of a single polymer chain, represented by the Kremer-Grest bead-spring model, in a solution with a Lennard-Jones liquid as the solvent when the interaction strength…

Soft Condensed Matter · Physics 2021-11-17 Yisheng Huang , Shengfeng Cheng

The absorption of free linear chains in a polymer brush was studied with respect to chain size $L$ and compatibility $\chi$ with the brush by means of Monte Carlo (MC) simulations and Density Functional Theory (DFT) / Self-Consistent Field…

Soft Condensed Matter · Physics 2015-05-18 A. Milchev , S. A. Egorov , K. Binder

We study self-assembly of a binary mixture of components A and B confined in a slit-like pore with the walls modified by the stripes of tethered brushes made of beads of a sort A. The emphasis is on solvent mediated transitions between…

Soft Condensed Matter · Physics 2013-03-26 Ja. M. Ilnytskyi , S. Sokolowski , T. Patsahan

Star polymers with magnetically functionalized end groups are presented as a novel polymeric system whose morphology, self-aggregation, and orientation can easily be tuned by exposing these macromolecules simultaneously to an external…

Soft Condensed Matter · Physics 2019-04-03 David Toneian , Christos N. Likos , Gerhard Kahl