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The properties of semiflexible polymers tethered by one end to an impenetrable wall and exposed to oscillatory shear flow are investigated by mesoscale simulations. A polymer, confined in two dimensions, is described by a linear bead-spring…

Soft Condensed Matter · Physics 2021-12-14 Antonio Lamura , Roland G. Winkler , Gerhard Gompper

Brownian diffusion of rod-like polymers in the presence of randomly distributed spherical obstacles is studied using molecular dynamics (MD) simulations. It is observed that dependence of the reduced diffusion coefficient of these…

Soft Condensed Matter · Physics 2015-05-20 Farzaneh Sakha , Hossein Fazli

Inwardly curved polymer brushes are present in cylindrical and spherical micelles or in membranes tubes and vesicles decorated with anchored polymers, and influence their stability. We consider such polymer brushes in good solvent and show…

Soft Condensed Matter · Physics 2010-06-22 Manoel Manghi , Miguel Aubouy , Cyprien Gay , Christian Ligoure

A brief review of modeling and simulation methods for a study of polymers at interfaces is provided. When studying truly multiscale problems as provided by realistic polymer systems, coarse graining is practically unavoidable. In this…

Soft Condensed Matter · Physics 2009-10-19 Fathollah Varnik , Kurt Binder

We investigate, using numerical simulations and analytical arguments, a simple one dimensional model for the swelling or the collapse of a closed polymer chain of size N, representing the dynamical evolution of a polymer in a \Theta-solvent…

Condensed Matter · Physics 2009-10-31 E. Pitard , J. -P. Bouchaud

The number of allowed configurations of a polymer is reduced by the presence of a repulsive surface resulting in an entropic force between them. We develop a method to calculate the entropic force, and detailed pressure distribution, for…

Statistical Mechanics · Physics 2014-02-11 Yosi Hammer , Yacov Kantor

We study by means of molecular dynamics simulations of periodic shear cells, the influence of particle shape on the global mechanical behavior of dense granular media. Results at macro-mechanical level show that for large shear deformation…

Materials Science · Physics 2016-08-16 A. A. Peña , R. García-Rojo , H. J. Herrmann

We revisit the classical problem of a polymer confined in a slit in both of its static and dynamic aspects. We confirm a number of well known scaling predictions and analyse their range of validity by means of comprehensive Molecular…

An exact solution of coarse-grained polymer models with fluctuating internal friction and hydrodynamic interactions has not been proposed so far due to a one-to-all coupling between the connector vector velocities that precludes the…

Soft Condensed Matter · Physics 2024-06-19 R. Kailasham , Rajarshi Chakrabarti , J. Ravi Prakash

We experimentally and theoretically consider highly condensed planar brushes made of charged polymers. Using x-ray reflectivity on polyelectrolytes which are anchored at the water-air interface, it is shown that such strongly stretched…

A coarse-grained model to describe the lateral structure of a one-component polymer brush is presented. In this model, a single polymer chain is described by just two coordinates, namely the position of the grafted monomer, and the monomer…

Soft Condensed Matter · Physics 2014-02-19 Richard L. C. Vink

When a liquid drop spreads on an adaptive substrate the latter changes its properties what may result in an intricate coupled dynamics of drop and substrate. Here we present a generic mesoscale hydrodynamic model for such processes that is…

Fluid Dynamics · Physics 2020-10-28 Uwe Thiele , Simon Hartmann

In this paper, we study the electrostatics of pH-responsive polyelectrolyte-grafted spherical particles by using a strong stretching theory that takes into account the excluded volume interaction and the density of chargeable sites on the…

Soft Condensed Matter · Physics 2022-08-31 Jun-Sik Sin , Il-Chon Choe , Chol-Song Im

Although the stretching of polymers and biomolecules is important in numerous settings, their response when confined to two-dimensions is relatively poorly-studied. In this paper, we derive closed-form analytical expressions for the…

Soft Condensed Matter · Physics 2013-05-28 Sara Iliafar , Dmitri Vezenov , Anand Jagota

An effective medium approach together with a multiple scattering formalism is considered to study the steady-state dynamics of suspensions of spheres and rigid stiff polymer chains (Gaussian) without excluded volume interactions. The…

Condensed Matter · Physics 2009-10-28 Radu P. Mondescu , M. Muthukumar

The macroscopic properties of polymeric fluids are inherited from the material properties of the fibers embedded in the solvent. The behavior of such passive fibers in flow has been of interest in a wide range of systems, including cellular…

Soft Condensed Matter · Physics 2019-06-20 John LaGrone , Ricardo Cortez , Wen Yan , Lisa Fauci

The statistics of polymers advected by a turbulent flow are investigated. To limit the polymer lengths above to coil-stretch transition, a FENE-P type relaxation law is used. The turbulence is modeled by a random strain, delta-correlated in…

Chaotic Dynamics · Physics 2009-11-07 Jean-Luc Thiffeault

Polymer brushes and grafted polymers have attracted significant interest at the intersection of polymers, interfacial chemistry, colloidal science, and nanostructuring. The confinement of high-density grafted polymers and differences in…

Soft Condensed Matter · Physics 2026-02-17 Rigoberto C. Advincula , Jihua Chen

Force versus extension curves measure entropic elasticity of single polymer chain in force spectroscopy experiments. A Worm-like Chain model is used to describe force extension experiments with an intrinsic chain parameter called…

Soft Condensed Matter · Physics 2021-07-28 Vikhyaat Ahlawat , Shatruhansingh Rajput , Shivprasad Patil

We investigate polyelectrolyte brushes in the osmotic regime using both theoretical analysis and molecular dynamics simulation techniques. In the simulations at moderate Bjerrum length, we observe that the brush height varies weakly with…

Soft Condensed Matter · Physics 2007-05-23 Ali Naji , Roland R. Netz , Christian Seidel