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We evaluate the electron transmission through a dangling-bond wire on Si(100)-H (2x1). Finite wires are modelled by decoupling semi-infinite Si electrodes from the dangling-bond wire with passivating H atoms. The calculations are performed…

The transport properties of nanofluidic channels are usually studied under constant (DC) voltage or pressure driving. However, the frequency response under sinusoidal (AC) drivings offers rich insights into the time-dependent transport…

Mesoscale and Nanoscale Physics · Physics 2026-04-07 Baptiste Coquinot , Mathieu Lizée , Lydéric Bocquet , Nikita Kavokine

Nanoscopic heterogeneities in composition and structure are quintessential for the properties of electrocatalyst materials. Here, we present a semiclassical model to study the electrochemical properties of supported electrocatalyst…

Materials Science · Physics 2025-02-27 Yufan Zhang , Tobias Binninger , Jun Huang , Michael Eikerling

Conductance switching has been reported in many molecular junction devices, but in most cases has not been convincingly explained. We investigate conductance switching in Pt/stearic acid monolayer/Ti devices using pressure-modulated…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Feng Miao , Douglas Ohlberg , Duncan Stewart , R. Stanley Williams , Chun Ning Lau*

Solid-state electrolytes, by enabling lithium metal anodes, may significantly increase the energy density of current lithium-ion batteries. However, similar to their liquid counterparts, these hard and stiff electrolytes can still be…

Chemical Physics · Physics 2024-10-04 Rajeev Gopal , Longan Wu , Youngju Lee , Jinzhao Guo , Peng Bai

We have measured conductance histograms of atomic point contacts made from the noble-transition metal alloys CuNi, AgPd, and AuPt for a concentration ratio of 1:1. For all alloys these histograms at low bias voltage (below 300 mV) resemble…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Jan W. T. Heemskerk , Yves Noat , David J. Bakker , Jan M. van Ruitenbeek , Barend J. Thijsse , Peter Klaver

The quasiparticle method, which has achieved a great success in solid state electronics and crystal lattice vibration, is adopted to study the solid state ion transport. A general recipe is put forward to map the classical solid state ion…

Materials Science · Physics 2024-02-13 Jiaming Hu

We present first-principles calculations on electron transport through Na nanowires at finite bias voltages. The nanowire exhibits a nonlinear current-voltage characteristic and negative differential conductance. The latter is explained by…

Materials Science · Physics 2016-08-31 Shigeru Tsukamoto , Kikuji Hirose

The electron transport properties of a four-terminal molecular device are computed within the framework of density functional theory and non-equilibrium Keldysh theory. The additional two terminals lead to new properties, including a…

Mesoscale and Nanoscale Physics · Physics 2009-09-01 Kamal K. Saha , Wenchang Lu , J. Bernholc , Vincent Meunier

Lectures deal with the theory of electronic transport, in particular with the electrical conductivity, in systems dominated by strong electron-electron repulsion. The concept of charge stiffness is introduced to distinguish conductors and…

Strongly Correlated Electrons · Physics 2009-11-07 P. Prelovsek , X. Zotos

The quest for safe high-energy batteries with "5V-class" cathodes and lithium metal anodes drives research into solid electrolytes. However, reasons for the large charge transfer resistances -- the major bottleneck of all-solid-state…

Chemical Physics · Physics 2021-01-26 Katharina Becker-Steinberger , Simon Schardt , Birger Horstmann , Arnulf Latz

Ion mobility and ionic conductance in nanodevices are known to deviate from bulk behavior, a phenomenon often attributed to surface effects. We demonstrate that dielectric mismatch between the electrolyte and the surface can qualitatively…

Soft Condensed Matter · Physics 2018-09-17 Hanne S. Antila , Erik Luijten

A crucial ingredient in lithium (Li) and sodium (Na)-ion batteries (LIBs and NIBs) is the electrolytes. The use of Li-metal (Na-metal) as anode in liquid electrolyte LIBs (NIBs) is constrained by several issues including thermal runway and…

Materials Science · Physics 2022-12-14 Juefan Wang , Abhishek A. Panchal , Gopalakrishnan Sai Gautam , Pieremanuele Canepa

We introduce a model that accounts for the bipolar resistive switching phenomenom observed in transition metal oxides. It qualitatively describes the electric field-enhanced migration of oxygen vacancies at the nano-scale. The numerical…

Materials Science · Physics 2015-05-14 M. J. Rozenberg , M. J. Sanchez , R. Weht , C. Acha , F. Gomez-Marlasca , P. Levy

We present a qualitative model for a fundamental process in molecular electronics: the change in conductance upon bond breaking. In our model a diatomic molecule is attached to spin-polarized contacts. Employing a Hubbard Hamiltonian,…

Materials Science · Physics 2008-06-24 Ali Goker , Francois Goyer , Matthias Ernzerhof

We study the effect of laser driving on a minimal model for a hexagonal two-dimensional material with broken inversion symmetry. Through the application of circularly polarised light and coupling to a thermal free electron bath, the system…

Strongly Correlated Electrons · Physics 2019-09-04 Oliver Hart , Garry Goldstein , Claudio Chamon , Claudio Castelnovo

When the electron density of highly crystalline thin films is tuned by chemical doping or ionic liq- uid gating, interesting effects appear including unconventional superconductivity, sizeable spin-orbit coupling, competition with…

Mesoscale and Nanoscale Physics · Physics 2018-12-19 G. Dezi , N. Scopigno , S. Caprara , M. Grilli

For several years the electronic structure properties of the novel two-dimensional system silicene have been studied extensively. Electron transport across metal-silicence junctions, however, remains relatively unexplored. To address this…

Materials Science · Physics 2015-04-15 Yun-Peng Wang , J. N. Fry , Hai-Ping Cheng

We study transport in a Weyl semimetal with donor and acceptor impurities. At sufficiently high temperatures transport is dominated by electron-electron interactions, while the low-temperature resistivity comes from the scattering of…

Mesoscale and Nanoscale Physics · Physics 2017-06-13 Ya. I. Rodionov , S. V. Syzranov

Electronic properties of heterostructures in which a finite number of Mott-insulator layers are sandwiched by semi-infinite metallic leads are investigated by using the dynamical-mean-field method combined with the Keldysh Green's function…

Strongly Correlated Electrons · Physics 2009-11-13 Satoshi Okamoto