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We present the theoretical and detailed experimental characterizations of Photothermal Heterodyne Imaging. An analytical expression of the photothermal heterodyne signal is derived using the theory of light scattering from a fluctuating…

We demonstrate a prototype light scattering instrument combining a frequency domain approach to the intermediate scattering function from Super-Heterodyning Doppler Velocimetry with the versatility of a standard homodyne Dynamic Light…

We report experimental results on heterodyne holographic microscopy of subwavelength-sized gold particles. The apparatus uses continuous green laser illumination of the metal beads in a total internal reflection configuration for dark-field…

The acoustic vibrations of single monomers and dimers of gold nanoparticles were investigated by measuring for the first time their ultra-low frequency micro-Raman scattering. This experiment provides access not only to the frequency of the…

Light scattering detection in the near field, a rapidly expanding family of scattering techniques, has recently proved to be an appropriate procedure for performing dynamic measurements. Here we report an innovative algorithm, based on the…

We describe a scheme into which a camera is turned into an efficient tunable frequency filter of a few Hertz bandwidth in an off-axis, heterodyne optical mixing configuration, enabling to perform parallel, high-resolution coherent spectral…

Optics · Physics 2009-09-01 Michael Atlan , Michel Gross

We introduce a dynamic light scattering technique capable of resolving motion that changes systematically, and rapidly, with time. It is based on the visibility of a speckle pattern for a given exposure duration. Applying this to a vibrated…

Soft Condensed Matter · Physics 2007-05-23 P. K. Dixon , D. J. Durian

We measure spectral properties of surface thermal fluctuations of liquids, solids, complex fluids and biological matter using light scattering methods. The random thermal fluctuations are delineated from random noise at sub-shot noise…

Soft Condensed Matter · Physics 2015-05-13 Takahisa Mitsui , Kenichiro Aoki

The selective optical detection of individual metallic nanoparticles (NPs) with high spatial and temporal resolution is a challenging endeavour, yet is key to the understanding of their optical response and their exploitation in…

Mesoscale and Nanoscale Physics · Physics 2012-06-05 Francesco Masia , Wolfgang Langbein , Paola Borri

We introduce a new, highly sensitive, and simple heterodyne optical method for imaging individual non-fluorescent nano-objects. A two orders of magnitude improvement of the signal is achieved compared to previous methods. This allows for…

Other Condensed Matter · Physics 2007-05-23 Stephane Berciaud , Laurent Cognet , Gerhard Blab , Brahim Lounis

The ultrafast response of metals to light is governed by intriguing non-equilibrium dynamics involving the interplay of excited electrons and phonons. The coupling between them gives rise to nonlinear diffusion behavior on ultrashort…

The photothermal heterodyne imaging technique enabled studies of individual weakly absorbing nano-objects in various environments. It uses a photo-induced change in the refractive index of the environment. Taking advantage of the dramatic…

We introduce a charge coupled device (CCD) camera based detection scheme in dynamic light scattering that provides information on the single-scattered auto-correlation function even for fairly turbid samples. It is based on the single…

Soft Condensed Matter · Physics 2009-11-11 Pavel Zakharov , Suresh Bhat , Peter Schurtenberger , Frank Scheffold

We describe a multispeckle dynamic light scattering technique capable of resolving the motion of scattering sites in cases that this motion changes systematically with time. The method is based on the visibility of the speckle pattern…

Soft Condensed Matter · Physics 2007-05-23 R. Bandyopadhyay , A. S. Gittings , S. S. Suh , P. K. Dixon , D. J. Durian

A differential interference contrast microscopy technique, which employs a photonic crystal fiber as a white-light source, is used to measure both the real and imaginary parts of the complex dielectric constant of single 10 and 15 nm gold…

Materials Science · Physics 2009-11-11 Patrick Stoller , Volker Jacobsen , Vahid Sandoghdar

Droplets, particularly water, are abundant in nature and artificial systems. Thermal fluctuations imply that droplet interfaces behave like a stormy sea at the sub-nanometer scale.Thermal capillary-waves have been widely studied since 1908…

Soft Condensed Matter · Physics 2015-12-25 Shai Maayani , Leopoldo L. Martin , Samuel Kaminski , Tal Carmon

We report the observation of dynamic fringe patterns in the diffuse scattering of extreme ultraviolet light from surfaces, following femtosecond optical excitation. At each point on the detector, the diffuse scattering intensity exhibits…

We introduce a new, highly sensitive, and simple heterodyne optical method for imaging individual nonfluorescent nanoclusters and nanocrystals. A 2 order of magnitude improvement of the signal is achieved compared to previous methods. This…

Optics · Physics 2007-05-23 Stéphane Berciaud , Laurent Cognet , Gerhard A Blab , Brahim Lounis

In this review, we discuss the use of continuous variable spectroscopy techniques for investigating quantum coherence and light-matter interactions in semiconductor systems with ultrafast dynamics. We focus on multichannel homodyne…

Mesoscale and Nanoscale Physics · Physics 2023-06-05 Carolin Lüders , Franziska Barkhausen , Matthias Pukrop , Elena Rozas , Jan Sperling , Stefan Schumacher , Marc Aßmann

Previous research has shown that gold nanoparticles immersed in water in an optical vortex lattice formed by the perpendicular intersection of two standing light waves with a \pi/2 rad phase difference will experience enhanced dispersion…

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