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Imaging of the optical properties of individual nanosystems beyond fluorescence can provide a wealth of information. However, the minute signals for absorption and dispersion are challenging to observe, and only specialized techniques…

Optics · Physics 2015-09-10 Matthias Mader , Jakob Reichel , Theodor W. Hänsch , David Hunger

We describe a new scheme for the measurement of mean photon flux at an arbitrary optical sideband frequency using homodyne detection. Experimental implementation of the technique requires an AOM in addition to the homodyne detector, and…

Quantum Physics · Physics 2009-11-11 J. G. Webb , T. C. Ralph , E. H. Huntington

We experimentally study a homodyne detection technique for the characterization of a quadrature squeezed field where the correlated bands, here created by four-wave mixing in a hot atomic vapor, are separated by a large frequency gap of…

Quantum Physics · Physics 2016-12-21 Christopher S. Embrey , Joshua Hordell , Plamen G. Petrov , Vincent Boyer

Homodyne measurement is a corner-stone of quantum optics. It measures the fundamental variables of quantum electrodynamics - the quadratures of light, which represent the cosine-wave and sine-wave components of an optical field and…

We measure the transient absorption of single gold particles with a common-path interferometer. The prompt electronic part of the signal provides high-contrast images for diameters as small as 10 nm. Mechanical vibrations of single…

Other Condensed Matter · Physics 2007-05-23 Meindert A. van Dijk , Markus Lippitz , Michel Orrit

We report observations of nanosecond nanometer scale heterogeneous dynamics in a free flowing colloidal jet revealed by ultrafast x-ray speckle visibility spectroscopy. The nanosecond double-bunch mode of the Linac Coherent Light Source…

We exploit the optical lever principle to detect minute fluctuations of a liquid-air interface. Waves propagating on the interface deflect a specularly reflected laser beam, inducing angular deviations captured by a dual-element photodiode.…

The advent of diffraction limited sources and developments in detector technology opens up new possibilities for the study of materials in situ and operando. Coherent X-ray diffraction techniques such as coherent X-ray diffractive imaging…

We have theoretically investigated the possibility of using any of several continuous-variable Bell-type inequalities - for which the dichotomic measurements are achieved with coarse-grained quadrature (homodyne) measurements - in a…

Quantum Physics · Physics 2018-12-12 William N. Plick , Francesco Arzani , Nicolas Treps , Eleni Diamanti , Damian Markham

A multispeckle technique for efficiently measuring correctly ensemble-averaged intensity autocorrelation functions of scattered light from non-ergodic and/or non-stationary systems is described. The method employs a CCD camera as a…

Soft Condensed Matter · Physics 2009-11-07 Virgile. Viasnoff , Francois Lequeux , D. J. Pine

Transient absorption and Raman scattering measurements on noble metal nanoparticles offer complimentary information on their vibrational modes and mechanical interactions with their surroundings. We have developed a comprehensive modeling…

Mesoscale and Nanoscale Physics · Physics 2024-10-29 Rachel Gelfand , Matthew Pelton

UV-Vis absorption spectroscopy is frequently used to characterize the size and shape of gold nanoparticles. We present a full-spectrum model that yields reliable results for the commonly encountered case of mixtures of spheres and rods in…

Soft Condensed Matter · Physics 2015-04-07 Kostyantyn Slyusarenko , Benjamin Abécassis , Patrick Davidson , Doru Constantin

X-ray diffraction studies of nanoporous gold face the poorly understood diffraction scenario where large coherent crystals are riddled with nanoscale holes. Theoretical considerations derived in this study show that the ligament size of the…

Materials Science · Physics 2017-12-27 Matthias Graf , Bao-Nam Dinh Ngô , Jörg Weissmüller , Jürgen Markmann

An experimental scheme is introduced to measure multiple parameters that are encoded in the phase quadrature of a light beam. Using a modal description and a spectrally-resolved homodyne detection, it is shown that all of the information is…

Optics · Physics 2017-03-29 Valérian Thiel , Jonathan Roslund , Pu Jian , Claude Fabre , Nicolas Treps

We present a new technique that combines off-axis Digital Holography and Dark Field Microscopy to track 100nm gold particles diffusing in water. We show that a single hologram is sufficient to localize several particles in a thick sample…

Optics · Physics 2015-06-03 Frédéric Verpillat , Fadwa Joud , Pierre Desbiolles , Michel Gross

Light scattering techniques are widely used in many fields of condensed and sof t matter physics. Usually these methods are based on the study of the scattered light in the far field. Recently, a new family of near field detection schemes…

When a coherent laser beam impinges on a random sample (e.g. a colloidal suspension), the scattered light exhibits characteristic speckles. If the temporal coherence of the light source is too short, then the speckles disappear, along with…

Optics · Physics 2011-12-13 D. Brogioli , D. Salerno , F. Croccolo , R. Ziano , F. Mantegazza

We propose a time-resolved optical measurement scheme for sampling transient charge and spin currents in a bulk centrosymmetric semiconductor. The technique relies on emission of second harmonic light triggered by a pulsed below-gap optical…

Mesoscale and Nanoscale Physics · Physics 2024-06-18 Amin Lakhal , Stéphane Virally , Jacob B. Khurgin , Denis V. Seletskiy

Absorption microscopy is a powerful technique, enabling the detection of single non- fluorescent molecules at room temperature. So far, the molecular absorption has been probed optically via the attenuation of a probing laser. The…

Applied Physics · Physics 2018-11-21 Miao-Hsuan Chien , Mario Brameshuber , Gerhard J. Schütz , Silvan Schmid

We perform balanced homodyne detection of the electromagnetic field in a single-mode tapered optical nanofiber surrounded by rubidium atoms in a magneto-optical trap. Resonant fluorescence of atoms into the nanofiber mode manifests itself…