Related papers: Vibrational wave packet induced oscillations in tw…
We perform a thorough theoretical analysis of resonance effects when an arbitrarily polarized plane monochromatic wave is incident onto a double periodically modulated metal film sandwiched by two different transparent media. The proposed…
Vibrational coherences in ultrafast pump-probe (PP) and 2D electronic spectroscopy (2DES) provide insight into the excited state dynamics of molecules. Femtosecond coherence spectra (FCS) and 2D beat maps yield information about…
New experimental techniques based on non-linear ultrafast spectroscopies have been developed over the last few years, and have been demonstrated to provide powerful probes of quantum dynamics in different types of molecular aggregates,…
In the past decade, the advent of time-resolved spectroscopic tools has provided a new ground to explore fundamental interactions in solids and to disentangle degrees of freedom whose coupling leads to broad structures in the frequency…
Nanomechanical and other mesoscopic vibrational systems typically have several nonlinearly coupled modes with different frequencies and with long lifetime. We consider the power spectrum of one of these modes. Thermal fluctuations of the…
In this work, robustness of controlled density of optical states in doubly driven artificial atoms is studied under phonon dissipation. By using both perturbative and polaron approaches, we investigate the influence of carrier-phonon…
Vapour cell spectroscopy is an essential technique in many fields; in particular, nearly all atom and ion trapping experiments rely on simultaneous spectroscopy of two atomic transitions, traditionally employing separate apparatus for each…
We study theoretically the fluctuation properties of acoustic phonons created in a semiconductor quantum dot after ultrafast optical excitation. An excitation with a single ultrafast pulse creates an exciton confined to the quantum dot,…
Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…
We present a variation of two-dimensional electronic spectroscopy that is capable of mapping spatially-varying differences in electronic couplings using a correlated map of excitation and detection frequencies, with sensitivity orders of…
We present a comprehensive study of the photon energy ($h \nu$) dependent line-shape evolution of molecular orbital signals of large $\pi$-conjugated molecules by resonant photoelectron spectroscopy (RPES). A comparison to RPES data of…
We first extend our recent experiments of correlation imaging through scattering media to the case of a thick medium, composed of two phase scatterers placed respectively in the image and the Fourier planes of the crystal. The spatial…
We show that the electron-phonon coupling in graphene, in contrast with the non-relativistic two-dimensional electron gas, leads to shifts in the phonon frequencies that are non-trivial functions of the electronic density. These shifts can…
We consider ramifications of the use of high speed light modulators to questions of correlation and measurement of time-energy entangled photons. Using phase modulators, we find that temporal modulation of one photon of an entangled pair,…
We analyze the time-dependent interaction between a two-level atom and a spectrally encoded single-photon wave packet using the Heisenberg-Langevin equations and derive the atomic excitation probability. Spectral phase encoding broadens the…
Coherent control of ultrafast quantum phenomena benefits from pulse-shaping capabilities allowing to modulate the envelope and instantaneous phase of optical fields on femtosecond time scales. While such control is available for optical…
Electron-phonon coupling directly determines the stability of cooperative order in solids, including superconductivity, charge and spin density waves. Therefore, the ability to enhance or reduce electron-phonon coupling by optical driving…
Optical fibers containing multiple cores are being developed towards capacity enhancement in space-division multiplexed optical communication networks. In many cases, the fibers are designed for negligible direct coupling of optical power…
We calculate the frequency-dispersed nonlinear transmission signal of a phase-shaped visible pulse to fourth order in the field. Two phase profiles, a phase-step and phase-pulse, are considered. Two dimensional signals obtained by varying…
The light-harvesting efficiency of a photoactive molecular complex is largely determined by the properties of its electronic quantum states. Those, in turn, are influenced by molecular vibrational states of the nuclear degrees of freedom.…