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We describe an all-electron implementation of the Bethe-Salpeter equation (BSE) for the calculation of optical absorption spectra in the full-potential linearized augmented-plane-wave (FLAPW) method. So far, FLAPW implementations have…

Materials Science · Physics 2026-03-27 Jörn Stöhler , Stefan Blügel , Christoph Friedrich

We show efficient electro-optic modulation in a subwavelength gap-plasmon waveguide (GPW) formed by an electro-optic polymer with metal coatings. The proposed device is studied in the attenuated total reflection and end-fire configurations.…

Optics · Physics 2010-03-03 Subimal Deb , K. Sarat Kumar , P. Anantha Lakshmi , S. Dutta Gupta

We formulate a Hartree-Fock-LAPW method for electronic band structure calculations. The method is based on the Hartree-Fock-Roothaan approach for solids with extended electron states and closed core shells where the basis functions of…

Materials Science · Physics 2016-08-31 A. V. Nikolaev , P. N. Dyachkov

The vertex function ($\Gamma$) within the Green's function formalism encapsulates information about all higher-order electron-electron interaction beyond those mediated by density fluctuations. Herein, we present an efficient approach that…

Chemical Physics · Physics 2023-03-28 Guorong Weng , Rushil Mallarapu , Vojtech Vlcek

In this article we present the exact representation of a fully correlated electronic wavefunction as the single-particle basis approaches completeness. It consists of a half-infinite chain of matrices of exponentially increasing size. The…

Quantum Physics · Physics 2022-05-04 Gero Friesecke , Benedikt R. Graswald , Örs Legeza

We present an efficient algorithm for the all-electron periodic Coulomb matrix based on the Ewald summation combined with the Fourier-transformed Coulomb method. The short-range contributions involving compact densities are evaluated in…

Chemical Physics · Physics 2025-09-23 Hieu Q. Dinh , Adam Rettig , Xintian Feng , Joonho Lee

Accurate and efficient predictions of the quasiparticle properties of complex materials remain a major challenge due to the convergence issue and the unfavorable scaling of the computational cost with respect to the system size.…

Materials Science · Physics 2020-07-14 Weiyi Xia , Weiwei Gao , Gabriel Lopez-Candales , Yabei Wu , Wei Ren , Wenqing Zhang , Peihong Zhang

We have developed an efficient computational scheme utilizing the real-space finite-difference formalism and the projector augmented-wave (PAW) method to perform precise first-principles electronic-structure simulations based on the density…

Using the simple (symmetric) Hubbard dimer, we analyze some important features of the $GW$ approximation. We show that the problem of the existence of multiple quasiparticle solutions in the (perturbative) one-shot $GW$ method and its…

Chemical Physics · Physics 2021-10-12 Stefano Di Sabatino , Pierre-François Loos , Pina Romaniello

We construct a reference database of materials properties calculated using density-functional theory in the local or generalized-gradient approximation, and an all-electron or a projector augmented-wave (PAW) formulation, for verification…

Materials Science · Physics 2014-04-14 E. Kucukbenli , M. Monni , B. I. Adetunji , X. Ge , G. A. Adebayo , N. Marzari , S. de Gironcoli , A. Dal Corso

The GW Approximation is an ab initio approach to calculating electronic structure which avoids using the Local Density (LDA) Approximation, the Generalized Gradient (GGA) Approximation, or similar density functionals. It goes beyond the…

Mesoscale and Nanoscale Physics · Physics 2019-04-05 Vincent Sacksteder

We combine the single site dynamical mean field theory (DMFT) with the non-local GW method. This is done fully self-consistently and we apply our formalism to a one-band Hubbard model. Eventually at self-consistency the full self-energy and…

Strongly Correlated Electrons · Physics 2007-05-23 K. Karlsson

We report a successful combination of magnetic force linear response theory with quasiparticle self-consistent GW method. The self-consistently determined wavefunctions and eigenvalues can just be used for the conventional magnetic force…

Materials Science · Physics 2019-09-04 Hongkee Yoon , Seung Woo Jang , Jae-Hoon Sim , Takao Kotani , Myung Joon Han

The self-consistent GW band gaps are known to be significantly overestimated. We show that this overestimation is, to a large extent, due to the neglect of the contribution of the lattice polarization to the screening of the…

Materials Science · Physics 2015-06-15 Silvana Botti , Miguel A. L. Marques

The rigorous coupled-wave analysis (RCWA) is one of the most successful and widely used methods for modeling periodic optical structures. It yields fast convergence of the electromagnetic far-field and has been adapted to model various…

Optics · Physics 2015-07-24 Martin Weismann , Dominic F. G. Gallagher , Nicolae C. Panoiu

The cumulant expansion is a powerful approach for including correlation effects in electronic structure calculations beyond the GW approximation. However, current implementations are incomplete since they ignore terms that lead to partial…

Strongly Correlated Electrons · Physics 2014-02-04 J. J. Kas , J. J. Rehr , L. Reining

A method for performing variable-width (thawed) Gaussian wavepacket (GWP) variational dynamics on machine-learned potentials is presented. Instead of fitting the potential energy surface (PES), the anharmonic correction to the global…

Chemical Physics · Physics 2024-12-17 Rami Gherib , Ilya G. Ryabinkin , Scott N. Genin

We solve the Dyson equation for atoms and diatomic molecules within the GW approximation, in order to elucidate the effects of self-consistency on the total energies and ionization potentials. We find GW to produce accurate energy…

Materials Science · Physics 2015-03-30 Adrian Stan , Nils Erik Dahlen , Robert van Leeuwen

We develop the plasmon-pole approximation for an interacting electron gas confined in a semiconductor quantum wire. We argue that the plasmon-pole approximation becomes a more accurate approach in quantum wire systems than in higher…

Condensed Matter · Physics 2009-10-28 S. Das Sarma , E. H. Hwang , Lian Zheng

In one of the most important methods in Density Functional Theory - the Full-Potential Linearized Augmented Plane Wave (FLAPW) method - dense generalized eigenproblems are organized in long sequences. Moreover each eigenproblem is strongly…

Distributed, Parallel, and Cluster Computing · Computer Science 2013-05-23 Mario Berljafa , Edoardo Di Napoli
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