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We use a pump-probe scheme to measure the time evolution of the C K-edge X-ray absorption spectrum (XAS) from CO/Ru(0001) after excitation by an ultrashort high-intensity optical laser pulse. Due to the short duration of the X-ray probe…

We present a new method that combines fluorescence correlation spectroscopy (FCS) on the microsecond time scale with fluorescence antibunching measurements on the nanosecond time scale for measuring photophysical rate constants of…

Chemical Physics · Physics 2022-03-28 Damir Sakhapov , Ingo Gregor , Narain Karedla , Jörg Enderlein

Time-resolved X-ray absorption spectroscopy (TR-XAS), based on laser-pump/X-ray probe method, is powerful in capturing the change of geometrical and electronic structure of the absorbing atom upon excitation. TR-XAS data analysis is…

Chemical Physics · Physics 2017-03-08 Fei Zhan , Ye Tao , Haifeng Zhao

Fluorescence microscopy is a powerful tool for imaging biological samples with molecular specificity. In contrast, phase microscopy provides label-free measurement of the sample's refractive index (RI), which is an intrinsic optical…

Optics · Physics 2022-01-26 Yi Xue , David Ren , Laura Waller

Free-electron lasers (FEL) in the extreme ultraviolet (XUV) and X-ray regime opened up the possibility for experiments at high power densities, in particular allowing for fluence-dependent absorption and scattering experiments to reveal…

A non-destructive method for measuring the resonant absorption coefficient of rare-earth-doped optical fibers is introduced. It can be applied to a broad range of fiber designs and host materials. The method compares the side-collected…

Optics · Physics 2019-03-27 Mostafa Peysokhan , Esmaeil Mobini , Behnam Abaie , Arash Mafi

Due to its specificity, fluorescence microscopy (FM) has become a quintessential imaging tool in cell biology. However, photobleaching, phototoxicity, and related artifacts continue to limit FM's utility. Recently, it has been shown that…

We have implemented the newly-introduced, coherence-based technique of x-ray near-field speckle (XNFS) at 8-ID-I at the Advanced Photon Source. In the near field regime of high-brilliance synchrotron x-rays scattered from a sample of…

Soft Condensed Matter · Physics 2011-02-16 Xinhui Lu , Simon GJ Mochrie , S. Narayanan , A. R. Sandy , M. Sprung

Absorbing a focused, femtosecond X-ray pulse from a Free-Electron Laser (FEL) can lead to extreme electronic excitations in solids. This excitation drives changes of the electronic system over the course of the pulse duration and the…

Materials Science · Physics 2023-12-12 Robin Y. Engel , Markus Scholz , Jan O. Schunck , Martin Beye

We present a comprehensive computational framework for reproducing the full X-ray absorption fine structure (XAFS) through quantum-chemical simulations. The near-edge region is accurately captured using an efficient implementation of…

Materials Science · Physics 2025-12-04 Philipp Hönicke , Yves Kayser , Pouya Partovi-Azar

X-ray imaging is a fundamental tool of routine clinical diagnosis. Fluoroscopic imaging can further acquire X-ray images at video frame rates, thus enabling non-invasive in-vivo motion studies of joints, gastrointestinal tract, etc. For…

Image and Video Processing · Electrical Eng. & Systems 2018-10-22 Jacky C. K. Chow , Derek Lichti , Kathleen Ang , Gregor Kuntze , Gulshan Sharma , Janet Ronsky

We demonstrate two new approaches that have been developed to aid the production of future hard X-ray catalogs, and specifically to reduce the reliance on human intervention during the detection of faint excesses in maps that also contain…

High Energy Astrophysical Phenomena · Physics 2022-01-19 V. A. Lepingwell , A. J. Bird , S. R. Gunn

Photoabsorption cross sections for 235 stable nuclei, ranging from $^{40}$Ca to $^{209}$Bi, were investigated by the quasiparticle finite amplitude method (QFAM) based on the axially deformed relativistic Hartree-Bogoliubov (RHB) approach…

Nuclear Theory · Physics 2025-06-25 C. Chen , Y. F. Niu , R. Xu , Y. Tian

Reaching the high angular resolution and contrast level desired for exoplanetary science requires us to equip large telescopes with extreme adaptive optics (XAO) systems to compensate for the effect of the atmospheric turbulence at a very…

Instrumentation and Methods for Astrophysics · Physics 2025-11-20 A. Striffling , C. -T. Héritier , R. J. -L Fétick , O. Fauvarque , J. -F Sauvage , A. Carlotti , B. Neichel T. Fusco

The nonlinear interaction of x-rays with matter is at the heart of understanding and controlling ultrafast molecular dynamics from an atom-specific viewpoint, providing new scientific and analytical opportunities to explore the structure…

Conventional absorption spectroscopy relies on coherent laser sources, and in turn suffers from the inherent limitation of shot noise, especially in estimating weak absorption. Here we propose a measurement strategy with correlated photons…

Quantum Physics · Physics 2025-04-17 Zhucheng Zhang , Xue Zhang , Jing Liu , Hui Dong

We study a sample of six X-ray selected broad absorption line (BAL) quasi-stellar objects (QSOs) from the XMM-Newton Wide Angle Survey. All six objects are classified as BALQSOs using the classic balnicity index, and together they form the…

We develop and apply a novel method of analysis to study the X-ray spectral properties of 908 QSOs in the Large Bright Quasar Survey (LBQS) that were observed during the soft X-ray ROSAT All-Sky Survey (RASS). Due to the relatively short…

X-ray absorption spectroscopy (XAS) is a premier technique for materials characterization, providing key information about the local chemical environment of the absorber atom. In this work, we develop a database of sulfur K-edge XAS spectra…

X-ray absorption spectroscopy (XAS) has gained popularity in recent years as it probes matter with high spatial and elemental sensitivity. However, the theoretical modelling of XAS is a challenging task since XAS spectra feature a fine…

Chemical Physics · Physics 2023-02-03 Lukas Konecny , Stanislav Komorovsky , Jan Vicha , Kenneth Ruud , Michal Repisky