English
Related papers

Related papers: Attosecond electron spectroscopy using a novel int…

200 papers

We study the photoionization of argon atoms close to the 3s$^2$3p$^6$ $\rightarrow$ 3s$^1$3p$^6$4p $\leftrightarrow$ 3s$^2$3p$^5$ $\varepsilon \ell$, $\ell$=s,d Fano window resonance. An interferometric technique using an attosecond pulse…

We propose an attosecond XUV-pump IR-probe photoionization protocol that employs pairs of counter-rotating consecutive harmonics and angularly resolved photoelectron detection, thereby providing direct measurement of ionization phases. The…

Atomic Physics · Physics 2019-10-02 Stefan Donsa , Nicolas Douguet , Joachim Burgdörfer , Iva Březinová , Luca Argenti

We present an alternative approach to pump-probe spectroscopy for measuring fast charge dynamics with an atomic force microscope (AFM). Our approach is based on coherent multifrequency lock-in measurement of the intermodulation between a…

Mesoscale and Nanoscale Physics · Physics 2019-01-30 Riccardo Borgani , David B. Haviland

Attosecond science is well developed for atoms and promising results have been obtained for molecules and solids. Here, we review the first steps in developing attosecond time-resolved measurements in liquids. These advances provide access…

Other Condensed Matter · Physics 2020-09-11 H. J. Wörner , A. Schild , D. Jelovina , I. Jordan , C. Perry , T. T. Luu , Z. Yin

Interferometric measurements of high-harmonics induced by multiple laser fields in an emerging field of research that promises optimized yield of harmonics, and time and space-resolved nonlinear spectroscopy. Most of the measurements have…

Ultrashort electron pulses with a high average current provide a powerful means of enhancing time-resolved imaging and photon generation. In this study, we report the attosecond shaping of sub-relativistic electron beams using membranes in…

Attosecond pump-probe ionization process can be used to prepare atomic ions in the coherent superposition of states with opposite parity. The multiphoton shake-up ionization of Helium, in particular, generates ions with same principal…

Atomic Physics · Physics 2019-12-12 Saad Mehmood , Eva Lindroth , Luca Argenti

State-of-the-art attosecond metrology deals with the detection and characterization of photon pulses with typical energies up to the hundreds of eV and time resolution of several tens of attoseconds. Such short pulses are used for example…

Instrumentation and Detectors · Physics 2015-06-04 Andreas Ipp , Jörg Evers , Christoph H. Keitel , Karen Z. Hatsagortsyan

Fano resonances are ubiquitous phenomena appearing in many fields of physics, e.g. atomic or molecular photoionization, or electron transport in quantum dots. Recently, attosecond interferometric techniques have been used to measure the…

Attosecond nonlinear Fourier transform (NFT) pump probe spectroscopy is an experimental technique which allows investigation of the electronic excitation, ionization, and unimolecular dissociation processes. The NFT spectroscopy utilizes…

Chemical Physics · Physics 2021-02-11 Sergy Grebenshchikov , Sergio Carbajo

Photoionization of matter is one of the fastest electronic processes in nature. Experimental measurements of photoionization dynamics have become possible through attosecond metrology. However, all experiments reported to date contain a…

Quantum Physics · Physics 2025-02-11 Meng Han , Jia-Bao Ji , Leung Chung Sum , Kiyoshi Ueda , Hans Jakob Wörner

We present the first fully ab initio calculations for attosecond transient absorption spectroscopy of atomic krypton with overlapping pump and probe pulses. Within the time-dependent configuration interaction singles (TDCIS) approach, we…

Attosecond interferometry (AI) is an experimental technique based on ionizing a system with an attosecond pulse train in the presence of an assisting laser. This assisting laser provides multiple pathways for the photoelectron wave packet…

Chemical Physics · Physics 2020-10-07 Denis Jelovina , Armin Scrinzi , Hans Jakob Wörner , Axel Schild

Attosecond pulses from free-electron lasers have opened the doors to atomic site-specific pumping and probing of quantum systems. Key to their success has been electron beam shaping techniques enabling the generation of sub-femtosecond…

Studies of ultrafast dynamics along with femtosecond-pulse metrology rely on non-linear processes, induced solely by the exciting/probing pulses or the pulses to be characterized. Extension of these approaches to the extreme-ultraviolet…

Atomic Physics · Physics 2015-05-27 P. Tzallas , E. Skantzakis , L. A. A. Nikolopoulos , G. D. Tsakiris , D. Charalambidis

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

Atomic Physics · Physics 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen

The blooming of attosecond science (1 as = $10^{-18}$ s) has raised the need to exquisitely control the delay between two ultrashort light pulses, one of them being intense and in the visible spectral range, while the second is weak and in…

We show that time ordering underlying time-dependent quantum dynamics is a physical observable accessible by attosecond streaking. We demonstrate the extraction of time ordering for the prototypical case of time-resolved two-photon double…

Atomic Physics · Physics 2015-03-06 Renate Pazourek , Stefan Nagele , Joachim Burgdörfer

A nonlinear planar waveguide pumped by a beam orthogonal to its surface may serve as a versatile source of photon pairs. Changing pump-pulse duration, pump-beam transverse width, and angular decomposition of pump-beam frequencies…

Quantum Physics · Physics 2009-11-13 Jan Perina

We present an electrically tunable terahertz two dimensional plasmonic interferometer with an integrated detection element that down converts the terahertz fields to a DC signal. The integrated detector utilizes a resonant plasmonic…

Mesoscale and Nanoscale Physics · Physics 2016-05-11 Gregory C. Dyer , Gregory R. Aizin , S. James Allen , Albert D. Grine , Don Bethke , John L. Reno , Eric A. Shaner