Related papers: Attosecond electron spectroscopy using a novel int…
Attosecond science has demonstrated that electrons can be controlled on the sub-cycle time scale of an optical wave, paving the way toward optical frequency electronics. Using controlled few-cycle optical waveforms, the study of sub-cycle…
Phase-shift differences and amplitude ratios of the outgoing $s$ and $d$ continuum wave packets generated by two-photon ionization of helium atoms are determined from the photoelectron angular distributions obtained using velocity map…
Interference results when a quantum particle is free to choose among a few indistinguishable paths. A canonical example of Bohr's complementarity principle [1] is a two-path interferometer with an external detector coupled to one of the…
Pump-probe microscopy is an emerging nonlinear imaging technique based on high repetition rate lasers and fast intensity modulation. Here we present new methods for pump-probe microscopy that keep the beam intensity constant and instead…
We demonstrate femtosecond pump-probe transient absorption spectroscopy using a programmable dispersive filter as an ultra-fast delay line. Combined with fast synchronous detection this delay line allows for recording of 6 ps decay traces…
A nonlinear interferometry scheme is described theoretically to induce and resolve electron wave- function beating on time scales shorter than the optical cycle of the time-delayed pump and probe pulses. By employing two moderately intense…
We report measurements of energy-dependent attosecond photoionization delays between the two outer-most valence shells of N$_2$O and H$_2$O. The combination of single-shot signal referencing with the use of different metal foils to filter…
We theoretically investigate the generation of intense keV attosecond pulses in an orthogonally polarized multicycle midinfrared two-color laser field. It is demonstrated that multiple continuum-like humps, which have a spectral width of…
When two indistinguishable photons are each incident on separate input ports of a beamsplitter they `bunch' deterministically, exiting via the same port as a direct consequence of their bosonic nature. This two-photon interference effect…
The nonlinear response of materials, an increasingly important aspect of light-matter interaction, can be challenging to measure in highly absorbing materials. Here, we introduce an interferometric technique that enables a direct…
Since the first proof-of-principle experiments 25 years ago, quantum metrology has matured from fundamental concepts to versatile and powerful tools in a large variety of research branches, such as gravitational-wave detection, atomic…
Infrared femtosecond laser pulses are important tools both in strong-field physics, driving X-ray high-harmonic generation, and as the basis for widely tuneable, if inefficient, ultrafast sources in the visible and ultraviolet. Although…
We propose a novel quantum nonlinear interferometer design that incorporates a passive PT symmetric coupler sandwiched between two nonlinear sections where signal-idler photon pairs are generated. The PT-symmetry enables efficient coupling…
We investigate the control of electronic energy transfer in molecular dimers through the preparation of specific vibrational coherences prior to electronic excitation, and its observation by nonlinear wave-packet interferometry.…
An interferometric imaging technique has been proposed to instantly measure the diameter of individual spherical dust particles suspended in a gas discharge plasma. The technique is based on the defocused image analysis of both spherical…
Attosecond pulses in the soft-X-ray (SXR) to water-window energy region offer the tools for creating and studying target specific localized inner-shell electrons or holes in materials, enable monitoring or controlling charge and energy…
In this paper we describe the technical implementation of pump-probe cathodoluminescence microscopy (PP-CL), a novel technique for studying ultrafast dynamics in materials using combined excitation of electron and laser pulses. The PP-CL…
We develop a first-principles simulation method for attosecond time-resolved photoelectron spectroscopy. This method enables us to directly simulate the whole experimental processes, including excitation, emission and detection on equal…
We have proposed and developed a method to utilize attosecond pulses in diffraction imaging techniques applied to complex samples. In this study, the effects of the broadband properties of the wavefield owing to attosecond pulses are…
Characterizing quantum states of the electromagnetic field at microwave frequencies requires fast and sensitive detectors that can simultaneously probe the field time-dependent amplitude and its quantum fluctuations. In this work, we…