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The structure, thermodynamics and slow activated dynamics of the equilibrated metastable regime of glass-forming fluids remains a poorly understood problem of high theoretical and experimental interest. We apply a highly accurate…

Soft Condensed Matter · Physics 2024-08-21 Subhashish Chaki , Baicheng Mei , Kenneth S. Schweizer

We describe a comprehensive model for the formation and morphological development of atmospheric ice crystals growing from water vapor, also known as snow crystals. Our model derives in part from empirical measurements of the intrinsic ice…

Materials Science · Physics 2012-11-26 Kenneth G. Libbrecht

The plasticity of amorphous solids undergoing shear is characterized by quasi-localized rearrangements of particles. While many models of plasticity exist, the precise relationship between plastic dynamics and the structure of a particle's…

Soft Condensed Matter · Physics 2024-06-12 Jason W. Rocks , Sean A. Ridout , Andrea J. Liu

We propose a geometrical characterization of amorphous liquid structures that suppress crystallization by competing locally with crystalline order. We introduce for this purpose the crystal affinity of a liquid, a simple measure of its…

Soft Condensed Matter · Physics 2017-10-11 Pierre Ronceray , Peter Harrowell

Off-equilibrium dynamics of a three-dimensional lattice model with nearest- and next nearest-neighbors exclusions is studied. At equilibrium, the model undergoes a first-order fluid-solid transition. Non-equilibrium filling, through random…

Statistical Mechanics · Physics 2015-05-30 H. Levit , Z. Rotman , E. Eisenberg

Supercooled liquids exhibit spatial heterogeneity in the dynamics of their fluctuating atomic arrangements. The length and time scales of the heterogeneous dynamics are central to the glass transition and influence nucleation and growth of…

Materials Science · Physics 2018-05-09 Pei Zhang , Jason J. Maldonis , Ze Liu , Jan Schroers , Paul M. Voyles

We explore the relationship between a machine-learned structural quantity (softness) and excess entropy in simulations of supercooled liquids. Excess entropy is known to scale well the dynamical properties of liquids, but this…

Soft Condensed Matter · Physics 2023-06-07 Ian R. Graham , Paulo E. Arratia , Robert A. Riggleman

We use molecular dynamics simulations in two dimensions to investigate the possibility that a core-softened potential can reproduce static and dynamic anomalies found experimentally in liquid water: (i) the increase in specific volume upon…

Soft Condensed Matter · Physics 2009-10-31 A. Scala , M. Reza Sadr-Lahijany , N. Giovambattista , S. V. Buldyrev , H. E. Stanley

During the evolution of density inhomogeneties in an $\Omega=1$, matter dominated universe, the typical density contrast changes from $\delta\simeq 10^{-4}$ to $\delta\simeq 10^2$. However, during the same time, the typical value of the…

General Relativity and Quantum Cosmology · Physics 2019-08-17 J. S. Bagla , T. Padmanabhan

Using molecular dynamics simulations and integral equations we investigate the structure, the thermodynamics and the dynamics of a system of particles interacting through a continuous core- softened ramp-like interparticle potential. We…

Statistical Mechanics · Physics 2007-11-28 Alan Barros de Oliveira , Paulo A. Netz , Marcia C. Barbosa

We combine computer simulations and analytical theory to investigate the glassy dynamics in dense assemblies of athermal particles evolving under the sole influence of self-propulsion. The simulations reveal that when the persistence time…

Soft Condensed Matter · Physics 2015-06-30 Grzegorz Szamel , Elijah Flenner , Ludovic Berthier

We use computer simulations to study the microscopic dynamics of an athermal assembly of soft particles near the fluid-to-solid, jamming transition. Borrowing tools developed to study dynamic heterogeneity near glass transitions, we…

Materials Science · Physics 2010-06-24 Claus Heussinger , Ludovic Berthier , Jean-Louis Barrat

We review 15 years of theoretical and experimental work on the non-linear response of glassy systems. We argue that an anomalous growth of the peak value of non-linear susceptibilities is a signature of growing "amorphous order" in the…

Disordered Systems and Neural Networks · Physics 2021-01-12 Giulio Biroli , Jean-Philippe Bouchaud , Francois Ladieu

Hydrodynamics is shown to induce non-Hermitian topological phenomena in ordinary, passive soft matter. This is demonstrated for the first time by subjecting a 2D elastic lattice to a low-Reynolds viscous flow. The interplay of hydrodynamics…

Soft Condensed Matter · Physics 2021-08-11 Tsvi Tlusty

We describe a novel crystal growth instability that enhances the development of thin edges, promoting the formation of plate-like or hollow columnar morphologies. This instability arises when diffusion-limited growth is coupled with…

Materials Science · Physics 2012-09-25 Kenneth G. Libbrecht

Although density functional theory provides reliable predictions for the static properties of simple fluids under confinement, a theory of comparative accuracy for the transport coefficients has yet to emerge. Nonetheless, there is evidence…

The recently measured spin susceptibility of the two dimensional electron gas exhibits a strong dependence on temperature, which is incompatible with the standard Fermi liquid phenomenology. Here we show that the observed temperature…

Strongly Correlated Electrons · Physics 2017-05-16 Arkady Shekhter , Alexander M. Finkel'stein

The most accepted origin for the water anomalous behavior is the phase transition between two liquids (LLPT) in the supercooled regime connected to the glassy first order phase transition at lower temperatures. Two length scales potentials…

Soft Condensed Matter · Physics 2023-04-19 José Rafael Bordin , Leandro B. Krott

The recently-developed non-equilibrium extension of the self-consistent generalized Langevin equation theory of irreversible relaxation [Phys. Rev. E (2010) 82, 061503; ibid. 061504] is applied to the description of the irreversible process…

Soft Condensed Matter · Physics 2013-05-29 Luis Enrique Sanchez-Diaz , Pedro Ramirez-Gonzalez , Magdaleno Medina-Noyola

By analytically solving some simple models of phase-ordering kinetics, we suggest a mechanism for the onset of non-equilibrium behaviour in colloid-polymer mixtures. These mixtures can function as models of atomic systems; their physics…

Soft Condensed Matter · Physics 2016-08-31 R. M. L. Evans , W. C. K. Poon