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Metal catalysts supporting the growth of Single Wall Carbon Nanotubes display different carbon solubilities and chemical reactivities. In order to specifically assess the role of carbon solubility, we take advantage of the physical…

Materials Science · Physics 2017-02-23 Juan-Manuel Aguiar-Hualde , Yann Magnin , Hakim Amara , Christophe Bichara

Surface interaction is extremely important to both fundamental research and practical application. Physisorption can induce shape and structural distortion (i.e. conformational changes) in macromolecular and biomolecular adsorbates, but…

Microstructure and mechanical properties of bulk polycristalline rhombohedral boron subnitride B13N2 synthesized by crystallization from the B-BN melt at 7 GPa have been systematically studied by micro- and nanoindentation, atomic force…

Materials Science · Physics 2017-12-08 Vladimir L. Solozhenko , Volodymyr Bushlya

We apply first-principles calculations to study the electronic structure of boron nitride nanocones with disclinations of different angles $\theta=n\pi/3$. Nanocones with odd values of $n$ present antiphase boundaries that cause a reduction…

Materials Science · Physics 2007-05-23 Sergio Azevedo , Mario S. C. Mazzoni , H. Chacham , R. W. Nunes

The nonlinear mechanical response of carbon nanotubes, referred to as their "buckling" behavior, is a major topic in the nanotube research community. Buckling means a deformation process in which a large strain beyond a threshold causes an…

Materials Science · Physics 2015-06-03 Hiroyuki Shima

The carbon rich phase diagrams of nickel-carbon nanoparticles, relevant to catalysis and catalytic chemical vapor deposition synthesis of carbon nanotubes, are calculated for system sizes up to about 3 nanometers (807 Ni atoms). A tight…

Atomic and Molecular Clusters · Physics 2015-06-11 Yann Magnin , Alexandre Zappelli , Hakim Amara , François Ducastelle , Christophe Bichara

Carbon nanotubes are one-dimensional and very narrow. These obvious facts imply that under doping with boron and nitrogen, microscopic doping inhomogeneity is much more important than for bulk semiconductors. We consider the possibility of…

Materials Science · Physics 2009-11-07 Paul E. Lammert , Vincent H. Crespi , Angel Rubio

Investigation on oxidation resistance of two-dimensional (2D) materials is critical for many of their applications, because 2D materials could have higher oxidation kinetics than their bulk counterparts due to predominant surface atoms and…

Materials Science · Physics 2014-03-06 Lu Hua Li , Jiri Cervenka , Kenji Watanabe , Takashi Taniguchi , Ying Chen

The structural and electronic properties of hexagonal boron nitride (hBN) grown on stepped Ni surfaces are systematically investigated using a cylindrical Ni crystal as a tunable substrate. Our experiments reveal homogeneous hBN monolayer…

Materials Science · Physics 2023-01-30 L. Fernandez , A. A. Makarova , C. Laubschat , D. V. Vyalikh , D. Yu. Usachov , J. E. Ortega , F. Schiller

Recently, two-dimensional nanostructures consisting of alternating graphene and boron nitride (BN) domains have been synthesized. These systems possess interesting electronic and mechanical properties, with potential applications in…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Yan Li , Riccardo Mazzarello

We present an ab-initio study of boron nitride as well as carbon allotropes. Their relative thermodynamic stabilities and structural phase transitions from low- to high-density phases are investigated. Pressure-temperature phase diagrams…

Materials Science · Physics 2019-02-22 Thomas Gruber , Andreas Grüneis

Growth of carbon nanotubes (CNTs) was performed by atmospheric pressure chemical vapour deposition (APCVD) of propane on Si(111) with a pre-treated Ni overlayer acting as a catalyst. Prior to the growth of CNTs, a thin film of Ni was…

Materials Science · Physics 2019-06-04 J Sengupta , SK Panda , C Jacob

Nanotubed titanic acid (H2Ti2O4(OH)2) was prepared from nanotubed sodium titanate (Na2Ti2O4(OH)2) by an ion exchange reaction in a pH=1 HCl solution. The effect of annealing temperature on the morphology, structure and photocatalytic…

Materials Science · Physics 2010-09-16 Min Zhang , Zhensheng Jin , Jingwei Zhang , Xinyong Guo , Jianjun Yang , Wei Li , Xiaodong Wang , Zhijun Zhang

Hexagonal boron nitride (h-BN) is a layered two-dimensional material with properties that make it promising as a dielectric in various applications. We report the growth of h-BN films on Ni foils from elemental B and N using molecular beam…

Materials Science · Physics 2015-05-29 S. Nakhaie , J. M. Wofford , T. Schumann , U. Jahn , M. Ramsteiner , M. Hanke , J. M. J. Lopes , H. Riechert

This study investigates the structural, electronic, and catalytic properties of pristine and doped C$_4$N$_2$ nanosheets as potential electrocatalysts for the hydrogen evolution reaction. The pristine C$_{36}$N$_{18}$ nanosheets exhibit…

The effect of Fe and Ni catalysts on the synthesis of carbon nanotubes (CNTs) using atmospheric pressure chemical vapor deposition (APCVD) was investigated. Field emission scanning electron microscopy (FESEM) analysis suggests that the…

Materials Science · Physics 2019-08-02 J. Sengupta , C. Jacob

The nitrogen reduction reaction (NRR), as an efficient and green pathway for ammonia synthesis, plays a crucial role in achieving on-demand ammonia production. This study proposes a novel design concept based on dual-iron atomic sites and…

Materials Science · Physics 2025-03-06 Zhe Zhang , Wenxin Ma , Jiajie Qiao , Xiaoliang Wu , Shaowen Yu , Weiye Hou , Xiang Huang , Rubin Huo , Hongbo Wu , Yusong Tu

The electrolysis of CO$_2$ in molten carbonate has been introduced as an alternative mechanism to synthesize carbon nanomaterials inexpensively at high yield. Until recently, CO$_2$ was thought to be unreactive, making its removal a…

Materials Science · Physics 2022-01-21 Xinye Liu , Gad Licht , Xirui Wang , Stuart Licht

Au nanoclusters grown on SiO$_2$ by physical vapor deposition are exposed to Br$_2$ and then measured with 1.5 keV Na$^+$ low energy ion scattering. It is found that the clusters are able to dissociate the molecules which then adsorb as…

Mesoscale and Nanoscale Physics · Physics 2018-10-08 Christopher R. Salvo , Josiah Keagy , Jory A. Yarmoff

Based on first-principles calculations, we propose that a layered electride Mg2O can serve as an effective substrate, in place of metal substrate, to grow honeycomb borophene (h-borophene). We first confirm the thermodynamic stability of…

Materials Science · Physics 2019-04-09 Xiaojuan Ni , Huaqing Huang , Kyung-Hwan Jin , Zhengfei Wang , Feng Liu