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We performed molecular dynamics simulations to study relaxation phenomena during vapor-liquid transitions in a single component Lennard-Jones system. Results from two different overall densities are presented; one in the neighborhood of the…

Statistical Mechanics · Physics 2019-06-04 Sutapa Roy , Arabinda Bera , Suman Majumder , Subir K. Das

A mechanism for relationship of solvent viscosity with reaction rate constant at enzyme action is suggested. It is based on fluctuations of electric field in enzyme active site produced by thermally equilibrium rocking (cranckshaft motion)…

Biomolecules · Quantitative Biology 2009-11-13 A. E. Sitnitsky

The steady state reached by a system of particles sliding down a fluctuating surface has interesting properties. Particle clusters form and break rapidly, leading to a broad distribution of sizes and large fluctuations. The density-density…

Statistical Mechanics · Physics 2015-05-13 Apoorva Nagar , Mustansir Barma

Many functional materials, such as paints and inks used in applications like coating and 3D printing, are concentrated granular suspensions. In such systems, the contact line dynamics and the internal structure of the suspension interact…

Linear polymers and other connected "line liquids" exhibit a coupling between density and equilibrium nematic order on the macroscopic level that gives rise to a Meyer-de Gennes vectorial conservation law. Nevertheless, isotropic linear…

Soft Condensed Matter · Physics 2019-04-08 Aleksandar Popadić , Daniel Svenšek , Rudolf Podgornik , Matej Praprotnik

A brief review is presented of the scaling of complex fluids, polymers and polyelectrolytes in solution and in confined geometry, in thermodynamical, structural and rheology properties using equilibrium and nonequilibrium dissipative…

Soft Condensed Matter · Physics 2016-12-06 Armando Gama Goicochea

Investigating million-atom systems for very long simulation times, we demonstrate that the collective density-density correlation time ($\tau_{\alpha}$) in simulated supercooled water and silica becomes wavevector independent ($q^0$) when…

Statistical Mechanics · Physics 2019-05-20 Philip H. Handle , Lorenzo Rovigatti , Francesco Sciortino

We first review the phenomenology of viscous liquids and the standard models used for explaining the non-Arrhenius average relaxation time. Then the focus is turned to the so-called elastic models, arguing that these models are all…

Soft Condensed Matter · Physics 2009-11-11 Jeppe C. Dyre

Molecular dynamics simulation is used for studying the contact angle of nanoscale sessile drops on a planar solid wall in a system interacting via the truncated and shifted Lennard-Jones potential. The entire range between total wetting and…

Mesoscale and Nanoscale Physics · Physics 2015-07-28 Stefan Becker , Herbert M. Urbassek , Martin Horsch , Hans Hasse

The theoretical framework for higher-order correlation functions involving multiple times and multiple points in a classical, many-body system developed by Van Zon and Schofield [Phys. Rev. E 65, 011106 (2002)] is extended here to include…

Statistical Mechanics · Physics 2007-05-23 Ramses van Zon , Jeremy Schofield

Among the challenges in discriminating between theoretical approaches to the glass transition is obtaining suitable data. In particular, particle--resolved data in liquids supercooled past the mode--coupling crossover has until recently…

Soft Condensed Matter · Physics 2021-03-16 Levke Ortlieb , Trond S. Ingebrigtsen , James E. Hallett , Francesco Turci , C. Patrick Royall

Surface tension-driven flow techniques have recently emerged as an efficient means of shedding light into the rheology of thin polymer films. Motivated by experimental and theoretical approaches in films bearing a varying surface…

Soft Condensed Matter · Physics 2017-04-26 Ioannis Tanis , Hendrik Meyer , Thomas Salez , Elie Raphaël , Anthony C. Maggs , Jörg Baschnagel

The emergent fluctuating hydrodynamics of a viscoelastic fluid modeled by the multiparticle collision dynamics (MPC) approach is studied. The fluid is composed of flexible, Gaussian phantom polymers, which interact by local…

Soft Condensed Matter · Physics 2020-01-29 David Toneian , Gerhard Kahl , Gerhard Gompper , Roland G. Winkler

We characterize the heterogeneous character of the dynamics of liquids approaching the glass transition through an experimental determination of the number of dynamically correlated molecules N_{corr} as obtained from dynamical…

Soft Condensed Matter · Physics 2015-06-12 Christiane Alba-Simionesco , Cecile Dalle-Ferrier , Gilles Tarjus

X-ray photon correlation is used to probe the slow dynamics of the glass-former B2O3 across the glass transition. In the undercooled liquid phase the decay times of the measured correlation functions are consistent with visible light…

Disordered Systems and Neural Networks · Physics 2019-07-03 Giovanna Pintori , Giacomo Baldi , Beatrice Ruta , Giulio Monaco

Glass-forming liquids grow dramatically sluggish upon cooling. This slowdown has long been thought to be accompanied by a growing correlation length. Characteristic dynamical and static length scales, however, have been observed to grow at…

Disordered Systems and Neural Networks · Physics 2016-08-22 Patrick Charbonneau , Ethan Dyer , Jaehoon Lee , Sho Yaida

Stress vs. strain fluctuations in athermal amorphous solids are an example of `crackling noise' of the type studied extensively in the context of elastic membranes moving through random potentials. Contrary to the latter, we do not have a…

Statistical Mechanics · Physics 2010-10-07 Edan Lerner , Itamar Procaccia

We solve numerically the equations of nonlinear fluctuating hydrodynamics (NFH) for the supercooled liquid. The time correlation of the density fluctuations in equilibrium obtained here shows quantitative agreement with molecular…

Soft Condensed Matter · Physics 2008-10-02 Bhaskar Sen Gupta , Shankar P. Das , Jean-Louis Barrat

A dynamic scaling Ansatz for the approach to the Self-Organized Critical (SOC) regime is proposed and tested by means of extensive simulations applied to the Bak-Sneppen model (BS), which exhibits robust SOC behavior. Considering the…

Adaptation and Self-Organizing Systems · Physics 2009-11-11 Karina Laneri , Alejandro F. Rozenfeld , Ezequiel V. Albano

We identify the pattern of microscopic dynamical relaxation for a two dimensional glass forming liquid. On short timescales, bursts of irreversible particle motion, called cage jumps, aggregate into clusters. On larger time scales, clusters…

Soft Condensed Matter · Physics 2010-10-04 R. Candelier , A. Widmer-Cooper , J. K. Kummerfeld , O. Dauchot , G. Biroli , P. Harrowell , D. R. Reichman