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We determined the magnetic structure of CuCr$_2$O$_4$ using neutron diffraction and irreducible representation analysis. The measurements identified a new phase between 155 K and 125 K as nearly collinear magnetic ordering in the Cr…

Strongly Correlated Electrons · Physics 2018-03-20 K. Tomiyasu , S. Lee , H. Ishibashi , Y. Takahashi , T. Kawamata , Y. Koike , T. Nojima , S. Torii , T. Kamiyama

The study of quantum spin-liquid states (QSL) with lattice dimension $>1$ has proven an enduring problem in solid state physics. Key candidate materials are the $S=\frac{1}{2}$ kagome magnets due to their ability to host quantum…

Materials Science · Physics 2016-10-04 E Connolly , P Reeves , D Boldrin , A S Wills

High-entropy spinel oxides provide an excellent platform for investigating entropy-stabilized correlated systems with strong configurational disorder. In this work, we systematically study the temperature evolution of the structural and…

The structural and magnetic properties of spinel compounds $CoB_2O_4$ (B=Cr,Mn and Fe) are studied using the DFT+U method and generalized gradient approximation (GGA). We concentrate on understanding the trends in the properties of these…

Strongly Correlated Electrons · Physics 2016-09-21 Debashish Das , Rajkumar Biswas , Subhradip Ghosh

Strategies such as chemical substitution, strain engineering and van der Waals stacking offer powerful means to control magnetism in 2D materials, enabling the emergence of novel quantum phenomena. Here, we investigate the magnetic…

Materials Science · Physics 2024-12-30 Alberto M. Ruiz , José J. Baldoví

Spin-frustrated systems are one avenue for inducing macroscopic quantum states in materials. However, experimental realization of this goal has been difficult because of the lack of simple materials and, if available, the separation of the…

Strongly Correlated Electrons · Physics 2010-04-07 S. Chu , T. M. McQueen , R. Chisnell , D. E. Freedman , P. Müller , Y. S. Lee , D. G. Nocera

The mixed valence Cr compound NaCr$_2$O$_4$, synthesized using a high-pressure technique, offers a unique playground for investigating unconventional physical properties in condensed matter. In the present study, muon spin…

We present a microscopic study of the electronic and magnetic properties of the newly synthesized Cu(II)-spin tetrahedron-based Cu4Te5O12Cl4 compound based on Density Functional calculations and on ab initio-derived effective models. In…

Strongly Correlated Electrons · Physics 2009-11-11 Badiur Rahaman , Harald O. Jeschke , Roser Valenti , T. Saha-Dasgupta

We studied the crystal and magnetic structure of the La$_{1-x}$Ca$_{x}$MnO$_{3}$ compound for $x=0.8$ and $x=0.85$. At T=300 K both samples are paramagnetic with crystallographic symmetry $Pnma$. At low temperatures they undergo a…

Strongly Correlated Electrons · Physics 2016-08-16 M. Pissas , G. Kallias , M. Hofmann , D. M. Többens

We have investigated magnetic properties of Rb$_2$Cu$_2$Mo$_3$O$_{12}$ powder. Temperature dependence of magnetic susceptibility and magnetic-field dependence of magnetization have shown that this cuprate is a model compound of a…

Other Condensed Matter · Physics 2009-11-10 Masashi Hase , Haruhiko Kuroe , Kiyoshi Ozawa , Osamu Suzuki , Hideaki Kitazawa , Giyuu Kido , Tomoyuki Sekine

On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases…

The novel magnetic phase diagram of the $Cs_2CuCl_{4-x}Br_x$ mixed system is established by means of single crystal neutron diffraction in the lowest temperature region and zero magnetic field. Two long-range ordered magnetic phases exist…

Polarized and unpolarized neutron diffraction studies have been carried out on single crystals of the coupled spin tetrahedra systems Cu2Te2O5X2 (X=Cl, Br). A model of the magnetic structure associated with the propagation vectors k'Cl ~…

We report a quasi-one-dimensional S = 1 spin chain compound BaNiTe2O7. This magnetic system has been investigated by magnetic susceptibility, specific heat, and neutron powder diffraction. These results indicate that BaNiTe2O7 develops a…

Using elastic and inelastic neutron scattering we show that a cubic spinel, CdCr$_2$O$_4$, undergoes an elongation along the c-axis ($c > a = b$) at its spin-Peierls-like phase transition at $T_N$ = 7.8 K. The N\'{e}el phase ($T < T_N$) has…

Strongly Correlated Electrons · Physics 2009-11-11 J. -H. Chung , M. Matsuda , S. -H. Lee , K. Kakurai , H. Ueda , T. J. Sato , H. Takagi , K. -P. Hong , S. Park

The rare-earth-based geometrically frustrated triangular magnets have attracted considerable attention due to the intricate interplay between strong spin-orbit coupling and the crystal electric field (CEF), which often leads to effective…

We performed susceptibility, magnetization, specific heat, and single crystal neutron diffraction measurements on single crystalline BaMn$_2$Si$_2$O$_7$. Based on the results, we revisited its spin structure with a more accurate solution…

Strongly Correlated Electrons · Physics 2019-07-31 G. H. Wang , C. Y. Xu , H. B. Cao , T. Hong , Q. Huang , Q. Y. Ren , J. Q. Xu , H. D. Zhou , W. D. Luo , D. Qian , J. Ma

YbZn$_2$GaO$_5$ is a promising candidate for realizing a quantum spin liquid (QSL) state, particularly owing to its lack of significant site disorder. Pulsed-field magnetometry at 0.5 K shows magnetization saturating near 15 T, with a…

An inelastic neutron scattering study was performed on a Zn-substituted spin-1/2 Heisenberg 2-leg ladder compound Sr(Cu1-xZnx)2O3 (x < 0.04) to investigate nonmagnetic impurity effects on the quantum spin system with a large spin gap of…

Condensed Matter · Physics 2009-10-30 M. Azuma , M. Takano , R. S. Eccleston

We have prepared the complete delafossite solid solution series between diamagnetic CuAlO2 and the t2g^3 frustrated antiferromagnet CuCrO2. The evolution with composition x in CuAl(1-x)Cr(x)O2 of the crystal structure and magnetic…

Materials Science · Physics 2012-10-03 Phillip T. Barton , Ram Seshadri , Andrea Knöller , Matthew J. Rosseinsky