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We report the structural and magnetic properties of a new system LiRhMnO$_{4}$ (LRMO) through x-ray diffraction, bulk magnetization, heat capacity and $^{7}$Li nuclear magnetic resonance (NMR) measurements. LRMO crystallizes in the cubic…

Strongly Correlated Electrons · Physics 2019-03-11 S. Kundu , T. Dey , M. Prinz-Zwick , N. Büttgen , A. V. Mahajan

We present the results of the first neutron powder and single crystal diffraction studies of the coupled spin tetrahedra systems ${\CuTeX}$ (X=Cl, Br). Incommensurate antiferromagnetic order with the propagation vectors…

Strongly Correlated Electrons · Physics 2009-11-10 O. Zaharko , A. Daoud-Aladine , S. Streule , J. Mesot , P. -J. Brown , H. Berger

Using the Becke-3-LYP functional, we have performed band structure calculations on the high temperature superconductor parent compound, La2CuO4. Under the restricted spin formalism (rho(alpha) equal to rho(beta)), the R-B3LYP band structure…

Superconductivity · Physics 2013-05-29 Jason K. Perry , Jamil Tahir-Kheli , William A. Goddard

The three-dimensional $S = {\frac{1}{2}}$ system Y$_{3}$Cu$_{2}$Sb$_{3}$O$_{14}$ consists of two inequivalent Cu$^{2+}$ sites, each forming an edge shared triangular lattice. Our magnetic susceptibility $\chi(T)$, specific heat $C_p(T)$,…

We report a detailed study of structural and magnetic properties of the pyrochlore-type (Bi2-xPrx)Ru2O7 series. Eleven compositions with 0 <= x <= 2 were prepared by solid state reaction at 1050 degrees C and found to form a solid solution…

Materials Science · Physics 2008-12-16 Siwar Zouari , Rafik Ballou , Abdelwaheb Cheikh-Rouhou , Pierre Strobel

Materials based on a crown ether complex together with magnetic ions, especially Cu(II), can be used to synthesize new low dimesional quantum spin systems. We have prepared the new crown ether complex…

Finding distinct signatures of a quantum spin liquid (QSL) is an ongoing quest in condensed matter physics, invariably complicated by the presence of disorder in real materials. In this regard the 2D Kagome system…

Strongly Correlated Electrons · Physics 2024-01-22 B. S. Shivaram , J. Prestigiacomo , Aini Xu , Zhenyuan Zeng , Trevor D. Ford , Itamar Kimchi , Shiliang Li , Patrick A. Lee

Two new transition-metal tellurium oxy-chlorides of the general formula Ni_5(TeO_3)_4X_2 (X=Cl, Br) have been isolated during the investigation of the ternary phase diagram NiO-NiCl2-TeO2. They crystallize in the monoclinic system, space…

Strongly Correlated Electrons · Physics 2010-03-09 M. Johnsson , K. W. Toernroos , P. Lemmens , P. Millet

High-resolution ac susceptibility and thermal conductivity measurement on Cu2Te2O5X2(X=Br,Cl) single crystals are reported. For Br-sample, sample dependence prevents to distinguish between possibilities of magnetically ordered and…

Strongly Correlated Electrons · Physics 2009-11-10 M. Prester , A. Smontara , I. Zivkovic , A. Bilusic , D. Drobac , H. Berger , F. Bussy

We report a detailed examination the magnetic structure of anhydrous cupric chloride CuCl2 carried out by powder neutron diffraction, magnetic susceptibility and specific heat measurements on polycrystalline and single crystal samples as…

Strongly Correlated Electrons · Physics 2009-04-21 M. G. Banks , R. K. Kremer , C. Hoch , A. Simon , B. Ouladdiaf , J. -M. Broto , H. Rakoto , C. Lee , M. -H. Whangbo

We investigate the structural and magnetic properties of the new quantum magnet BaCuTe$_2$O$_6$. This compound is synthesized for the first time in powder and single crystal form. Synchrotron X-ray and neutron diffraction reveal a cubic…

Strongly Correlated Electrons · Physics 2021-03-17 A. Samartzis , D. Khalyavin , A. T. M. N. Islam , S. Chillal , K. Siemensmeyer , K. Prokes , D. J. Voneshen , A. Senyshyn , B. Lake

Thermodynamic experiments as well as Raman scattering have been used to study the magnetic instabilities in the spin-tetrahedra systems Cu_2Te_2O_5X_2, X=Cl and Br. While the phase transition observed in the Cl system at T_o=18.2 K is…

Strongly Correlated Electrons · Physics 2009-11-07 P. Lemmens , K. -Y. Choi , E. E. Kaul , Ch. Geibel , K. Becker , W. Brenig , R. Valenti , C. Gros , M. Johnsson , P. Millet , F. Mila

We examine the evolution of magnetic properties in the normal spinel oxides Mg(1-x)Cu(x)Cr2O4 using magnetization and heat capacity measurements. The end-member compounds of the solid solution series have been studied in some detail because…

Materials Science · Physics 2012-09-11 Moureen C. Kemei , Stephanie L. Moffitt , Daniel P. Shoemaker , Ram Seshadri

The crystal and magnetic structures of stoichiometric ZnCr2Se4 have been investigated using synchrotron X-ray and neutron powder diffraction, muon spin relaxation (muSR) and inelastic neutron scattering. Synchrotron X-ray diffraction shows…

Strongly Correlated Electrons · Physics 2017-04-12 P. Zajdel , W-Y. Li , W. Van Beek , A. Lappas , A. Ziolkowska , S. Jaskiewicz , C. Stock , M. A. Green

The ground state of the solid solution of the two spin gap systems (CH3)2CHNH3CuCl3 and (CH3)2CHNH3CuBr3 has been investigated by 1H-NMR. The existence of a magnetic ordering in the sample with the Cl-content x=0.85 was clearly demonstrated…

Other Condensed Matter · Physics 2009-11-11 Keishi Kanada , Takehiro Saito , Akira Oosawa , Takayuki Goto , Takao Suzuki , Hirotaka Manaka

A recent study [Tassel {\it et al.}, Phys. Rev. Lett. {\bf 105}, 167205 (2010)] has proposed a remarkable spin model for (CuCl)LaNb2O7, in which dimers are ferromagnetically coupled to each other on the distorted Shastry-Sutherland lattice.…

Strongly Correlated Electrons · Physics 2011-08-17 Shunsuke Furukawa , Tyler Dodds , Yong Baek Kim

Cs2CuCl4 is known to possess a quantum spin liquid phase with antiferromagnetic interaction below 2.8 K. We report the observation of a new metastable magnetic phase of the triangular frustrated quantum spin system Cs2CuCl4 induced by the…

Strongly Correlated Electrons · Physics 2017-12-18 Hyeong-Jin Kim , C. R. S. Haines , C. Liu , Sae Hwan Chun , Kee Hoon Kim , H. T. Yi , Sang-Wook Cheong , Siddharth S. Saxena

We present the magnetic properties of complete solid solutions of ZnCr$_2$O$_4$ and CoCr$_2$O$_4$: two well-studied oxide spinels with very different magnetic ground states. ZnCr$_2$O$_4$, with non-magnetic $d^{10}$ cations occupying the A…

Materials Science · Physics 2009-06-04 Brent C. Melot , Jennifer E. Drewes , Ram Seshadri , Arthur P. Ramirez

A quantum spin liquid (QSL) is a state of matter where unpaired electrons' spins in a solid are quantum entangled, but do not show magnetic order in the zero-temperature limit. Because such a state may be important to the microscopic origin…

Structural, electronic, and magnetic properties of modified cubic spinel compound LiNi$_{0.5}$Mn$_{1.5}$O$_{4}$ are studied via x-ray diffraction, resistivity, DC and AC magnetization, heat capacity, neutron diffraction, $^7$Li nuclear…

Materials Science · Physics 2020-12-02 S. S. Islam , Vikram Singh , K Somesh , Prashanta K Mukharjee , A. Jain , S. M. Yusuf , R. Nath