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The Fe3+ lattice in the Bi2Fe4O9 compound is found to materialize the first analogue of a magnetic pentagonal lattice. Due to its odd number of bonds per elemental brick, this lattice, subject to first neighbor antiferromagnetic…

Strongly Correlated Electrons · Physics 2016-11-25 Eric Ressouche , Virginie Simonet , Benjamin Canals , Marin Gospodinov , Vassil Skumryev

We report the characterisation of natural samples of the cubic pyrite mineral MnS2 using very high resolution synchrotron X-ray diffraction techniques. At low temperatures we find a new low temperature polymorph, which results from coupling…

Strongly Correlated Electrons · Physics 2015-05-21 Simon A. J. Kimber , Tapan Chatterji

We have carried out the ESR study of the multiferroic triangular antiferromagnet CuCrO2 in the presence of an electric field. The shift of ESR spectra by the electric field was observed; the observed value of the shift exceeds that one in…

Strongly Correlated Electrons · Physics 2018-03-08 S. K. Gotovko , T. A. Soldatov , L. E. Svistov , H. D. Zhou

We report on the emergence of antiferromagnetic spin chains from two-dimensionally aligned spins on the anisotropic triangular lattice (ATL) in the insulating calcium rhenium oxychloride Ca3ReO5Cl2. The compound contains Re6+ ions each with…

Strongly Correlated Electrons · Physics 2019-04-15 Daigorou Hirai , Kazuhiro Nawa , Mitsuaki Kawamura , Takahiro Misawa , Zenji Hiroi

We report a neutron diffraction study of the multiferroic mechanism in (ND4)2FeCl5D2O, a molecular compound that exhibits magnetically induced ferroelectricity. This material exhibits two successive magnetic transitions on cooling: a…

We report a neutron scattering study of the metallic triangular lattice antiferromagnet PdCrO$_2$. Powder neutron diffraction measurements confirm that the crystalline space group symmetry remains $R\bar{3}m$ below $T_N$. This implies that…

We measured two magnetic modes with finite and discrete energies in an antiferromagnetic ordered phase of a geometrically frustrated magnet MgCr2O4 by single-crystal inelastic neutron scattering, and clarified the spatial spin correlations…

Strongly Correlated Electrons · Physics 2008-10-22 K. Tomiyasu , H. Suzuki , M. Toki , S. Itoh , M. Matsuura , N. Aso , K. Yamada

CuLa$_2$Ge$_2$O$_8$ forms a distorted triangular lattice of quantum spin-1/2 Cu$^{2+}$ ions. A crystal growth method was developed using the traveling-solvent floating zone technique resulting in the synthesis of a large single crystal (4…

Strongly Correlated Electrons · Physics 2026-04-17 S. Thamban , C. Aguilar-Maldonado , S. Chillal , R. Feyerherm , K. Prokeš , A. J. Studer , D. Abou-Ras , K. Karmakar , A. T. M. N. Islam , B. Lake

The magnetocaloric effect is studied at the transition to saturation in the antiferromagnetic spin-1/2 Heisenberg model on the simplest two-dimensional lattices, namely the square and the triangular lattice. Numerical results are presented…

Strongly Correlated Electrons · Physics 2007-05-23 A. Honecker , S. Wessel

In antiferromagnets, the interplay of spin frustration and spin-lattice coupling has been extensively studied as the source of complex spin patterns and exotic magnetism. Here, we demonstrate that, although neglected in the past, the…

We report density functional calculations addressing the electronic structure and magnetic properties of delafossite PdCrO2. We find substantial magnetic interactions in the c-axis direction as well as beyond first nearest neighbors…

Strongly Correlated Electrons · Physics 2015-03-19 K. P. Ong , D. J. Singh

We report a thorough theoretical study of the low temperature phase diagram of Cs_2CuCl_4, a spatially anisotropic spin S=1/2 triangular lattice antiferromagnet, in a magnetic field. Our results, obtained in a quasi-one-dimensional limit in…

Strongly Correlated Electrons · Physics 2015-03-17 Oleg A. Starykh , Hosho Katsura , Leon Balents

We present a combined neutron and synchrotron powder diffraction study of the crystal and magnetic structure of VOCl. The occurrence of antiferromagnetic order in VOCl is accompanied by a monoclinic distortion. The high sensitivity of the…

Strongly Correlated Electrons · Physics 2009-04-07 A. C. Komarek , T. Taetz , M. T. Fernandez-Diaz , D. M. Trots , A. Möller , M. Braden

We report an ultrasonic investigation of the elastic moduli on a single crystal of hexagonal YMnO_3 as a function of temperature. Stiffening anomalies in the antiferromagnetic N\'eel state below T_N = 72.4 K are observed on all the four…

Strongly Correlated Electrons · Physics 2007-08-07 Mario Poirier , Francis Laliberte , Loreynne Pinsard , Alexandre Revcolevschi

Spin wave dispersion in the frustrated fcc type-III antiferromagnet MnS$_2$ has been determined by inelastic neutron scattering using a triple-axis spectrometer. Existence of multiple spin wave branches, with significant separation between…

Strongly Correlated Electrons · Physics 2019-02-20 T. Chatterji , L. P. Regnault , S. Ghosh , A. Singh

We show that the motion of a single hole in the infinite $U$ Hubbard model with frustrated hopping leads to weak metallic antiferromagnetism of kinetic origin. An intimate relationship is demonstrated between the simplest versions of this…

Strongly Correlated Electrons · Physics 2009-11-11 Jan O Haerter , B Sriram Shastry

Sr2Cr3As2O2 is composed of alternating square-lattice CrO2 and Cr2As2 stacking layers, where CrO2 is isostructural to the CuO2 building-block of cuprate high-Tc superconductors and Cr2As2 to Fe2As2 of Fe-based superconductors. Current…

Motivated by puzzling spin-glass behaviors observed in many pyrochlore-based magnets, effects of magnetoelastic coupling to local lattice distortions were recently studied by the authors for a bond-disordered antiferromagnet on a pyrochlore…

Strongly Correlated Electrons · Physics 2013-07-25 Hiroshi Shinaoka , Yusuke Tomita , Yukitoshi Motome

The magnetic phase diagram and the thermodynamic properties of a square lattice containing antiferromagnetically coupled spin-1/2 triangles are studied. A Heisenberg Hamiltonian with three strong intra-triangle exchange coupling constants…

Strongly Correlated Electrons · Physics 2009-10-31 Stefan Wessel , Stephan Haas

Sr$_2$CuTeO$_6$ presents an opportunity for exploring low-dimensional magnetism on a square lattice of $S=1/2$ Cu$^{2+}$ ions. We employ ab initio multi-reference configuration interaction calculations to unravel the Cu$^{2+}$ electronic…