CuLa2Ge2O8 forms a distorted triangular lattice of quantum spin-1/2 Cu2+ ions. A crystal growth method was developed using the traveling-solvent floating zone technique resulting in the synthesis of a large single crystal (4 mm×4 mm×10 mm). The crystal was characterized with regard to phase purity and crystallinity using powder X-ray diffraction, energy dispersive X-ray analysis and Laue diffraction, and found to be of excellent quality. The magnetic properties were characterized using dc-susceptibility, magnetization, and heat capacity measurements which revealed weak magnetic frustration with long-range magnetic order occurring below TN=1.14(1)~K. The magnetic structure determined using neutron powder diffraction is a commensurate, noncollinear antiferromagnetic, different from the 120∘ order of an equilateral triangular antiferromagnet. The ordered moments lie in the {\bf bc}-plane, with components mb=0.50(3)~μB and mc=0.73(5)~μB along the {\bf b}- and {\bf c}-axes respectively, giving a total ordered moment of Mtotal= 0.89(6)μB/Cu2+ at 20~mK.
@article{arxiv.2603.05126,
title = {Crystal growth and magnetic properties of spin-$1/2$ distorted triangular lattice antiferromagnet CuLa$_2$Ge$_2$O$_8$},
author = {S. Thamban and C. Aguilar-Maldonado and S. Chillal and R. Feyerherm and K. Prokeš and A. J. Studer and D. Abou-Ras and K. Karmakar and A. T. M. N. Islam and B. Lake},
journal= {arXiv preprint arXiv:2603.05126},
year = {2026}
}