English

Crystal growth and magnetic properties of spin-$1/2$ distorted triangular lattice antiferromagnet CuLa$_2$Ge$_2$O$_8$

Strongly Correlated Electrons 2026-04-17 v2

Abstract

CuLa2_2Ge2_2O8_8 forms a distorted triangular lattice of quantum spin-1/2 Cu2+^{2+} ions. A crystal growth method was developed using the traveling-solvent floating zone technique resulting in the synthesis of a large single crystal (4 mm×\times4 mm×\times10 mm). The crystal was characterized with regard to phase purity and crystallinity using powder X-ray diffraction, energy dispersive X-ray analysis and Laue diffraction, and found to be of excellent quality. The magnetic properties were characterized using dc-susceptibility, magnetization, and heat capacity measurements which revealed weak magnetic frustration with long-range magnetic order occurring below TN=1.14(1)T_N=1.14(1)~K. The magnetic structure determined using neutron powder diffraction is a commensurate, noncollinear antiferromagnetic, different from the 120^{\circ} order of an equilateral triangular antiferromagnet. The ordered moments lie in the {\bf bc}-plane, with components mb=0.50(3)m_b=0.50(3)~μB\mu_{B} and mc=0.73(5)m_c= 0.73(5)~μB\mu_{B} along the {\bf b}- and {\bf c}-axes respectively, giving a total ordered moment of MtotalM_{total}= 0.89(6)μB/\mu_{B}/Cu2+^{2+} at 20~mK.

Keywords

Cite

@article{arxiv.2603.05126,
  title  = {Crystal growth and magnetic properties of spin-$1/2$ distorted triangular lattice antiferromagnet CuLa$_2$Ge$_2$O$_8$},
  author = {S. Thamban and C. Aguilar-Maldonado and S. Chillal and R. Feyerherm and K. Prokeš and A. J. Studer and D. Abou-Ras and K. Karmakar and A. T. M. N. Islam and B. Lake},
  journal= {arXiv preprint arXiv:2603.05126},
  year   = {2026}
}

Comments

11 pages, 13 figures