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We present the observation of an isostructural Mott insulator-metal transition in van-der-Waals honeycomb antiferromagnet V$_{0.9}$PS$_3$ through high-pressure x-ray diffraction and transport measurements. The MPX$_3$ family of magnetic…

Strongly Correlated Electrons · Physics 2019-03-27 M. J. Coak , S. Son , D. Daisenberger , H. Hamidov , C. R. S. Haines , P. L. Alireza , A. R. Wildes , C. Liu , S. S. Saxena , J. -G. Park

Upon reduction of the film thickness we observe a metal-insulator transition in epitaxially stabilized, spin-orbit coupled SrIrO$_3$ ultrathin films. By comparison of the experimental electronic dispersions with density functional theory at…

Strongly Correlated Electrons · Physics 2017-12-27 P. Schütz , D. Di Sante , L. Dudy , J. Gabel , M. Stübinger , M. Kamp , Y. Huang , M. Capone , M. -A. Husanu , V. Strocov , G. Sangiovanni , M. Sing , R. Claessen

CaRuO_3 is perovskite with an orthorhombic distortion and is believed to be close to magnetic ordering. Magnetic studies of single crystal and polycrystalline CaRu_{1-x}Cu_xO_3 (0\le x \le 15 at.%Cu) reveal that spin-glass-like transition…

Strongly Correlated Electrons · Physics 2017-12-05 I. M. Bradaric , I. Felner , M. Gospodinov

A sequence of structural transitions occurring in the quasi-one-dimensional (1D) 3d1 system BaVS3 at low temperature was investigated by high resolution synchrotron X-ray diffraction. The orthorhombic Cmc21 structure of the…

Strongly Correlated Electrons · Physics 2009-11-10 S. Fagot , P. Foury-Leylekian , S. Ravy , J. P. Pouget , M. Anne , G. Popov , M. V. Lobanov , M. Greenblatt

We have investigated 3d electronic states of doped transition metals in II-VI diluted magnetic semiconductors, Zn1-xMxSe (M = Mn, Fe, Co) and Zn1-xMnxY (Y = Se, Te), using the transition-metal L2,3-edge X-ray absorption spectroscopy (XAS)…

Strongly Correlated Electrons · Physics 2009-10-31 Kwanghyun Cho , Hoon Koh , S. -J. Oh , Hyeong-Do Kim , Moonsup Han , J. -H. Park , C. T. Chen , Y. D. Kim , J. -S. Kim , B. T. Jonker

Exfoliated magnetic 2D materials enable versatile tuning of magnetization, e.g., by gating or providing proximity-induced exchange interaction. However, their electronic band structure after exfoliation has not been probed, most likely due…

We investigate the evolution of the electronic structure in SrRu_(1-x)Ti_xO_3 as a function of x using high resolution photoemission spectroscopy, where SrRuO3 is a weakly correlated metal and SrTiO3 is a band insulator. The surface spectra…

Strongly Correlated Electrons · Physics 2009-11-13 Kalobaran Maiti , Ravi Shankar Singh , V. R. R. Medicherla

We report a synchrotron x-ray scattering study of the magnetoresistive manganite La_0.875Sr_0.125MnO_3. At low temperatures, this material undergoes an x-ray induced structural transition at which charge ordering of Mn^3+ and Mn^4+ ions…

Strongly Correlated Electrons · Physics 2009-10-31 V. Kiryukhin , Y. J. Wang , F. C. Chou , M. A. Kastner , R. J. Birgeneau

We present measurements of the infrared response of the quasi-one-dimensional organic conductor (TMTSF)2$SO3 along (E||a) and perpendicular (E||b') to the stacking axis as a function of temperature. Above the metal-insulator transition…

Strongly Correlated Electrons · Physics 2007-06-13 A. Pashkin , K. Thirunavukkuarasu , Y. -L. Mathis , W. Kang , C. A. Kuntscher

We combine the results of magnetic and transport measurements with neutron diffraction data to construct the structural and magnetic phase diagram of the entire family of SrMn$_{1-x}$Ru$_{x}$O$_3$ ($0 \leqslant x \leqslant 1$) perovskites.…

Materials Science · Physics 2009-11-13 S. Kolesnik , B. Dabrowski , O. Chmaissem

Angle-resolved photoemission spectroscopy was used to investigate the evolution of the electronic structure across the metal-insulator transition in bi-layer manganite $La_{1.24}Sr_{1.76}Mn_2O_7$. We found that this system is a metal for…

Strongly Correlated Electrons · Physics 2015-06-25 Z. Sun , J. F. Douglas , A. V. Fedorov , Y. -D. Chuang , H. Zheng , J. F. Mitchell , D. S. Dessau

Resonant inelastic x-ray scattering (RIXS) experiment was performed at the Mn $L_3$ edge. A 10 $\%$ Mn-doped Sr$_{3}$Ru$_{2}$O$_{7}$ compound, where the Mn$^{3+}$ ions are in the 3$d^4$ state, were probed for $dd$ excitations. The dilute…

Magnetic fluctuations in transition metal oxides are a subject of intensive research because of the key role they are expected to play in the transition from the Mott insulator to the unconventional metallic phase of these materials, and…

Strongly Correlated Electrons · Physics 2016-01-06 J. Gunasekera , L. Harriger , A. Dahal , T. Heitmann , G. Vignale , D. K. Singh

X-ray and electron diffraction measurements on the metal-insulator (M-I) transition compound PrRu$_4$P$_{12}$ have revealed the emergence of a periodic ordering of charge density around the Pr atoms. It is found that the ordering is…

Strongly Correlated Electrons · Physics 2009-11-10 C. H. Lee , H. Matsuhata , H. Yamaguchi , C. Sekine , K. Kihou , T. Suzuki , T. Noro , I. Shirotani

We report X-ray diffraction and resonant elastic X-ray scattering (REXS) studies on two $\alpha$-RuCl$_{3}$ crystals with distinct magnetic transition temperatures: T$_{N}$=7.3K and 6.5K. We find that the sample with T$_{N}$=6.5K exhibits a…

Strongly Correlated Electrons · Physics 2024-03-08 Subin Kim , Ezekiel Horsley , Christie Nelson , Jacob Ruff , Young-June Kim

In ReS$_2$ a layer-independent direct band-gap of 1.5 eV implies a potential for its use in optoelectronic applications. ReS$_2$ crystallizes in the 1T$^{\prime}$-structure which leads to anisotropic physical properties and whose…

We investigated the size dependence of the metal-insulator transition (MIT) in Cr-doped V2O3 nanocrystals by photoemission spectroscopy using complementary probing depths, together with magnetic susceptibility measurements. Photoemission…

In the perovskite oxide SrCrO$_{3}$ the interplay between crystal structure, strain and orbital ordering enables a transition from a metallic to an insulating electronic structure under certain conditions. We identified a narrow window of…

Understanding of the metal-insulator transition (MIT) in correlated transition-metal oxides is a fascinating topic in condensed matter physics and a precise control of such transitions plays a key role in developing novel electronic…

In order to explore the origin of the Metal-Insulator (M-I) transition, the precise crystal structures of the hole-doped Mott insulator system, Y1-XCaXTiO3 (x=0.37, 0.39 and 0.41), are studied for the temperature range between 20K and 300K…

Strongly Correlated Electrons · Physics 2009-11-07 K. Kato , E. Nishibori , M. Takata , M. Sakata , T. Nakano , K. Uchihira , M. Tsubota , F. Iga , T. Takabatake