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We have studied the crystal and magnetic structures of the magnetoelectric materials RMn2O5 (R = Tb, Ho, Dy) using neutron diffraction as a function of temperature. All three materials display incommensurate antiferromagnetic ordering below…

Strongly Correlated Electrons · Physics 2009-11-11 G. R. Blake , L. C. Chapon , P. G. Radaelli , S. Park , N. Hur , S-W. Cheong , J. Rodriguez-Carvajal

We report a neutron diffraction study of the multiferroic mechanism in (ND4)2FeCl5D2O, a molecular compound that exhibits magnetically induced ferroelectricity. This material exhibits two successive magnetic transitions on cooling: a…

The three-dimensional frustrated spin lattice in MgCrGaO4, where Cr3+ ions occupy a pyrochlore-like network, exemplifies a quantum magnet with competing interactions, macroscopic degeneracy, and exotic low-energy excitations. Using…

Strongly Correlated Electrons · Physics 2026-03-17 U. Jena , S. Kundu , Suheon Lee , Q. Faure , F. Damay , S. Rols , Adam Berlie , S. Petit , Kwang-Yong Choi , P. Khuntia

We use inelastic neutron scattering to study spin waves and their correlation with the magnetoelectric effect in Y$_{0.7}$Lu$_{0.3}$MnO$_3$. In the undoped YMnO$_3$ and LuMnO$_3$, the Mn trimerization distortion has been suggested to play a…

Strongly Correlated Electrons · Physics 2014-04-25 W. Tian , Guotai Tan , Liu Liu , Jinxing Zhang , Barry Winn , Tao Hong , J. A. Fernandez-Baca , Chenglin Zhang , Pengcheng Dai

Antiferromagnetic antiperovskites, of the form Mn$_3B$N ($B$ = Ni, Cu, Zn, Sn, Ir, and Pt), have shown an outstanding behavior in which, giant negative thermal expansion and chiral magnetic structures are intertwined. As such, aiming to…

Materials Science · Physics 2022-09-07 L. Florez-Gomez , W. Ibarra-Hernandez , A. C. Garcia-Castro

The recent neutron-scattering data for spin-wave dispersion in $\rm Ho Mn O_3$ are well described by an anisotropic Hubbard model on a triangular lattice with a planar (XY) spin anisotropy. Best fit indicates that magnetic excitations in…

Strongly Correlated Electrons · Physics 2015-06-25 Saptarshi Ghosh , Avinash Singh

The magnetic phase diagrams of RMnO3 (R = Er, Yb, Tm, Ho) are investigated up to 14 Tesla via magnetic and dielectric measurements. The stability range of the AFM order below the Neel temperature of the studied RMnO3 extends to far higher…

Strongly Correlated Electrons · Physics 2016-06-29 F. Yen , C. dela Cruz , B. Lorenz , E. Galstyan , Y. Y. Sun , M. Gospodinov , C. W. Chu

Hexagonal HoMnO$_{3}$ is a frustrated antiferromagnet (T$_{N}$=72 K) ferroelectric (T$_{C}$=875 K) in which these two order parameters are coupled. Our neutron measurements of the spin wave dispersion for the S=2 Mn$^{3+}$ on the layered…

Strongly Correlated Electrons · Physics 2009-11-11 O. P. Vajk , M. Kenzelmann , J. W. Lynn , S. B. Kim , S. -W. Cheong

We measured two magnetic modes with finite and discrete energies in an antiferromagnetic ordered phase of a geometrically frustrated magnet MgCr2O4 by single-crystal inelastic neutron scattering, and clarified the spatial spin correlations…

Strongly Correlated Electrons · Physics 2008-10-22 K. Tomiyasu , H. Suzuki , M. Toki , S. Itoh , M. Matsuura , N. Aso , K. Yamada

Strong magnetic-ferroelectric coupling in hexagonal HoMnO3 has been observed previously at spin reorientation temperature between P6'3cm' and the P6'3cm' magnetic phases. In contrast, YMnO3 has only a single magnetic phase (P6'3cm') and no…

Strongly Correlated Electrons · Physics 2013-03-26 Jagath Gunasekera , Owen P. Vajk , Yuan Wang , Kevin Tarwater , Tom W. Heitmann

Spin waves in the type-III ordered antiferromagnetic state of the frustrated $t$-$t'$ Hubbard model on the fcc lattice are calculated to investigate finite-$U$-induced competing interaction and frustration effects on magnetic excitations…

Strongly Correlated Electrons · Physics 2017-04-04 Avinash Singh , Shubhajyoti Mohapatra , Timothy Ziman , Tapan Chatterji

We present a study of the magnetic and crystallographic structure of TbMnO$_3$ in the presence of crossed electric and magnetic fields using circularly polarised X-ray non-resonant scattering. A comprehensive account is presented of the…

Strongly Correlated Electrons · Physics 2014-01-13 H. C. Walker , F. Fabrizi , L. Paolasini , F. de Bergevin , D. Prabhakaran , A. T. Boothroyd , D. F. McMorrow

We have used in-field neutron and X-ray single crystal diffraction to measure the incommensurability δ of the crystal and magnetic structure of multiferroic TbMnO3 . We show that the flop in the electric polarization at the critical…

Strongly Correlated Electrons · Physics 2009-11-11 N. Aliouane , D. N. Argyriou , J. Strempfer , I. Zegkinoglou , S. Landsgesell , M. v. Zimmermann

We performed inelastic neutron scattering experiments on single crystal samples of a linear magnetoelectric material Mn$_{3}$Ta$_{2}$O$_{8}$, which exhibits a collinear antiferromagnetic order, to reveal the spin dynamics. Numerous modes…

Strongly Correlated Electrons · Physics 2025-04-08 Hodaka Kikuchi , SHunsuke Hasegawa , Shinichiro Asai , Tao Hong , Kenta Kimura , Tsuyoshi Kimura , Shinichi Itoh , Takatsugu Masuda

The ferrimagnetic spinels MnB2O4 (B = Mn,V) exhibit a similar series of closely spaced magnetic and structural phase transitions at low temperatures, reflecting both magnetic frustration and a strong coupling between the spin and lattice…

Strongly Correlated Electrons · Physics 2015-01-28 S. L. Gleason , T. Byrum , Y. Gim , A. Thaler , P. Abbamonte , G. J. MacDougall , L. W. Martin , H. D. Zhou , S. L. Cooper

Two magnetic ordering transitions are found in InMnO3, the paramagnetic to antiferromagnetic transition near ~118 K and a lower possible spin rotation transition near ~42 K. Multiple length scale structural measurements reveal enhanced…

Materials Science · Physics 2015-06-22 T. Yu , T. A. Tyson , P. Gao , T. Wu , X. Hong , S. Ghose , Y. -S. Chen

In antiferromagnets, the interplay of spin frustration and spin-lattice coupling has been extensively studied as the source of complex spin patterns and exotic magnetism. Here, we demonstrate that, although neglected in the past, the…

MnTiO3 has been studied for many decades, but it was only in the last few years that its strong magnetoelectric behavior had been observed. Here, we use neutron scattering on two separately grown single crystals and two powder samples to…

Magnetic order of the manganese and rare-earth lattices according to different symmetry representations is observed in multiferroic hexagonal (h-) DyMnO$_3$ by optical second harmonic generation and neutron diffraction. The incompatibility…

Strongly Correlated Electrons · Physics 2012-08-08 C. Wehrenfennig , D. Meier , Th. Lottermoser , Th. Lonkai , J. -U. Hoffmann , N. Aliouane , D. N. Argyriou , M. Fiebig

We use neutron scattering to study the lattice and magnetic structure of the layered half-doped manganite Pr$_{0.5}$Ca$_{1.5}$MnO$_4$. On cooling from high temperature, the system first becomes charge- and orbital- ordered (CO/OO) near…

Strongly Correlated Electrons · Physics 2009-11-13 Songxue Chi , F. Ye , Pengcheng Dai , J. A. Fernandez-Baca , Q. Huang , J. W. Lynn , E. W. Plummer , R. Mathieu , Y. Kaneko , Y. Tokura