We use inelastic neutron scattering to study spin waves and their correlation with the magnetoelectric effect in Y0.7Lu0.3MnO3. In the undoped YMnO3 and LuMnO3, the Mn trimerization distortion has been suggested to play a key role in determining the magnetic structure and the magnetoelectric effect. In Y0.7Lu0.3MnO3, we find a much smaller in-plane (hexagonal ab-plane) single ion anisotropy gap that coincides with a weaker in-plane dielectric anomaly at TN. Since both the smaller in-plane anisotropy gap and the weaker in-plane dielectric anomaly are coupled to a weaker Mn trimerization distortion in Y0.7Lu0.3MnO3 comparing to YMnO3 and LuMnO3, we conclude that the Mn trimerization is responsible for the magnetoelectric effect and multiferroic phenomenon in Y1−yLuyMnO3.
@article{arxiv.1308.2908,
title = {Doping influence of spin dynamics and magnetoelectric effect in hexagonal Y$_{0.7}$Lu$_{0.3}$MnO$_{3}$},
author = {W. Tian and Guotai Tan and Liu Liu and Jinxing Zhang and Barry Winn and Tao Hong and J. A. Fernandez-Baca and Chenglin Zhang and Pengcheng Dai},
journal= {arXiv preprint arXiv:1308.2908},
year = {2014}
}