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Magnetoelastic effects in multiferroic YMnO$_3$

Strongly Correlated Electrons 2012-12-24 v1 Materials Science

Abstract

We have investigated magnetoelastic effects in multiferroic YMnO3_3 below the antiferromagnetic phase transition, TN70T_N \approx 70 K, using neutron powder diffraction. The aa lattice parameter of the hexagonal unit cell of YMnO3_3 decreases normally above TNT_N, but decreases anomalously below TN_N, whereas the cc lattice parameter increases with decreasing temperature and then increases anomalously below TN_N. The unit cell volume also undergoes an anomalous contraction below TNT_N. By fitting the background thermal expansion for a non-magnetic lattice with the Einstein-Gr\"uneisen equation, we determined the lattice strains Δa\Delta a, Δc\Delta c and ΔV\Delta V due to the magnetoelastic effects as a function of temperature. We have also determined the temperature variation of the ordered magnetic moment of the Mn ion by fitting the measured Bragg intensities of the nuclear and magnetic reflections with the known crystal and magnetic structure models and have established that the lattice strain due to the magnetoelastic effect in YMnO3_3 couples with the square of the ordered magnetic moment or the square of the order parameter of the antiferromagnetic phase transition.

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Cite

@article{arxiv.1207.0301,
  title  = {Magnetoelastic effects in multiferroic YMnO$_3$},
  author = {Tapan Chatterji and Bachir Ouladdiaf and Paul F. Henry and Dipten Bhattacharya},
  journal= {arXiv preprint arXiv:1207.0301},
  year   = {2012}
}
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