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The adsorption of atomic oxygen and its inclusion into subsurface sites on Ag(210) and Ag(410) surfaces have been investigated using density functional theory. We find that--in the absence of adatoms on the first metal layer--subsurface…

Condensed Matter · Physics 2009-11-10 A. Kokalj , N. Bonini , A. Dal Corso , S. de Gironcoli , S. Baroni

Graphene is a new material that exhibits remarkable properties from both fundamental and applied issues. This is a 2D matter system whose physical and mechanical features have been approached by using tight binding model, first principle…

Strongly Correlated Electrons · Physics 2011-08-10 Lalla Btissam Drissi , El Hassan Saidi , Mosto Bousmina

To understand the interaction between nitrogen dopants and native point defects in graphene, we have studied the energetic stability of N-doped graphene with vacancies and Stone-Wales (SW) defect by performing the density functional theory…

Mesoscale and Nanoscale Physics · Physics 2012-05-03 Zhufeng Hou , Xianlong Wang , Takashi Ikeda , Kiyoyuki Terakura , Masaharu Oshima , Masa-aki Kakimoto , Seizo Miyata

Graphene and other two-dimensional materials display remarkable optical properties, including a simple light transparency of $T \approx 1 - \pi \alpha$ for light in the visible region. Most theoretical rationalizations of this "universal"…

Mesoscale and Nanoscale Physics · Physics 2016-12-07 Daniel J. Merthe , Vitaly V. Kresin

Although very similar in many technological applications, graphene and MoS2 bear significant differences if exposed to humid environments. As an example, lubrication properties of graphene are reported to improve while those of MoS2 to…

Mesoscale and Nanoscale Physics · Physics 2016-07-20 Giacomo Levita , Paolo Restuccia , M. C. Righi

Graphene is one of the most promising 2D materials for various applications due to its unique electronic properties and high thermal stability. In previous studies, it was shown that when graphene is deposited onto some transition metal…

Materials Science · Physics 2018-02-13 Tianbai Li , Jory A. Yarmoff

A great efficacy of molecular quantum chemistry applied to basic graphene problems has been recently demonstrated by the authors when studying the formation of peculiar composites between carbon nanotubes and graphene as well as considering…

Mesoscale and Nanoscale Physics · Physics 2011-02-07 Elena F Sheka , Nadezhda A Popova

The density of states (DOS) of graphene underneath a metal is estimated through a quantum capacitance measurement of the metal/graphene/SiO2/n+-Si contact structure fabricated by a resist-free metal deposition process. Graphene underneath…

Materials Science · Physics 2013-07-22 Ryota Ifuku , Kosuke Nagashio , Tomonori Nishimura , Akira Toriumi

Using first-principles calculations we demonstrate sizable exchange coupling between a magnetic molecule and a magnetic substrate via a graphene layer. As a model system we consider cobaltocene (CoCp$_2$) adsorbed on graphene deposited on…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Simone Marocchi , Paolo Ferriani , Nuala Mai Caffrey , Franca Manghi , Stefan Heinze , Valerio Bellini

Deviations from the perfect atomic arrangements in crystals play an important role in affecting their properties. Similarly, diffusion of such deviations is behind many microstructural changes in solids. However, observation of point defect…

Materials Science · Physics 2014-07-28 Jani Kotakoski , Clemens Mangler , Jannik C. Meyer

We present exemplary results of extensive studies of mechanical, electronic and transport properties of covalent functionalization of graphene monolayers (GML) with -NH2. We report new results of ab initio studies of covalent…

Materials Science · Physics 2014-01-24 Karolina Z. Milowska , Jacek A. Majewski

Our study of the adsorption of oxygen molecules on individual semiconductiong single-walled carbon nanotubes at ambient conditions reveals that the adsorption is physisorption, that the resistance without O2 increases by ~two orders of…

Materials Science · Physics 2009-11-11 A. Tchernatinsky , B. Nagabhirava , S. Desai , G. Sumanasekera , B. Alphenaar , C. S. Jayanthi , S. Y. Wu

Nitrogen-doped graphene was recently synthesized and was reported to be a catalyst for hydrogen dissociative adsorption under a perpendicular applied electric field (F). In this work, the diffusion of H atoms on N-doped graphene, in the…

Materials Science · Physics 2012-02-15 Z. M. Ao , A. D. Hernández-Nieves , F. M. Peeters , S. Li

We demonstrate the growth of graphene nanocrystals by molecular beam methods that employ a solid carbon source, and that can be used on a diverse class of large area dielectric substrates. Characterization by Raman and Near Edge X-ray…

The influence of attractive boron impurities, embedded on a graphene sheet, on the phase diagrams of $^4$He and H$_2$ adsorbed on top was studied using the diffusion Monte Carlo method. The doping of graphene was made by distributing the…

Other Condensed Matter · Physics 2023-10-20 M. C. Gordillo , J. Boronat

Graphene quality indicators obtained by Raman spectroscopy have been correlated to the structural changes of the graphene/Germanium interface as a function of in-vacuum thermal annealing. Specifically, it is found that graphene becomes…

The design and production of novel 2-dimensional materials has seen great progress in the last decade, prompting further exploration of the chemistry of such materials. Doping and hydrogenating graphene is an experimentally realised method…

Chemical Physics · Physics 2017-11-22 Yasmine S. Al-Hamdani , Angelos Michaelides , O. Anatole von Lilienfeld

We studied theoretically the effect of a low concentration of adsorbed polar molecules on the optical conductivity of graphene, within the Kubo linear response approximation. Our analysis is based on a continuum model approximation that…

Mesoscale and Nanoscale Physics · Physics 2021-07-07 Horacio Falomir , Marcelo Loewe , Enrique Muñoz

Molecular hydrogen is at the core of hydrogen energy applications and has the potential to significantly reduce the use of carbon dioxide emitting energy processes. However, hydrogen gas storage is a major bottleneck for its large-scale use…

Materials Science · Physics 2025-01-22 Yasmine S. Al-Hamdani , Andrea Zen , Dario Alfé

Pristine graphene is not suitable for hydrogen storage at ambient conditions since it binds the hydrogen molecules only by van der Waals interactions. However, the adsorption energy of the hydrogen molecules can be improved by doping or…

Materials Science · Physics 2022-10-24 Vikram Mahamiya , Alok Shukla , Nandini Garg , Brahmananda Chakraborty
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