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We report a first principles study based on density functional theory on the structural and electronic properties of transition metal Zr and Hf doped small aluminum clusters with 1 to 7 aluminum atoms. We have used B3PW91 with LANL2DZ basis…

Materials Science · Physics 2018-06-28 Hardik L. Kagdada , Shweta D. Dabhi , Venu Mankad , Satyam M. Shinde , Prafulla K. Jha

The freezing behavior of gold nanoclusters was studied by employing molecular dynamics simulations based on a semi-empirical embedded-atom method. Investigations of the gold nanoclusters revealed that, just after freezing, ordered…

Atomic and Molecular Clusters · Physics 2009-11-07 H. -S. Nam , Nong M. Hwang , B. D. Yu , J. -K. Yoon

In order to get homogeneous nanostructured Aluminum Nitride deposits, thin films were grown at room temperature on [001] Si substrates by radio frequency magnetron reactive sputtering. The deposits were analysed by Transmission Electron…

Materials Science · Physics 2019-09-05 Valerie Brien , P. Pigeat

In this paper, we study nanoparticles with constituent atoms ranging from dozens to hundreds of them. These types of particles display structural and magnetic properties that strongly depend on the number of constituents N. The metal…

Mesoscale and Nanoscale Physics · Physics 2010-02-09 Karina L. D. Barturen H. , F. A. R. Navarro , Justo T Rojas

A computational approach to determine the equilibrium structures of nanoclusters in the whole temperature range from 0 K to melting is developed. Our approach relies on Parallel Tempering Molecular Dynamics (PTMD) simulations complemented…

Atomic and Molecular Clusters · Physics 2023-08-16 Manoj Settem , Riccardo Ferrando , Alberto Giacomello

The adsorption profiles and electronic structures of Pt$_n$ (n = 1--4) clusters on stoichiometric, reduced and reconstructed rutile TiO$_2$(110) surfaces were systematically studied using on site d-d Coulomb interaction corrected hybrid…

Strongly Correlated Electrons · Physics 2011-01-06 Veysel Celik , Hatice Unal , Ersen Mete , Sinasi Ellialtioglu

In metallic nanoparticles, the cluster geometric structures control the particle's electronic band structure, polarizability, and catalytic properties. Analyzing the structural properties is a complex problem; the structure of an assembled…

Materials Science · Physics 2022-10-12 Jiale Shi , Shanghui Huang , François Gygi , Jonathan K. Whitmer

The thermodynamics and kinetics of crystallization of nanoparticles, as opposed to bulk phases, may be influenced by surface and size effects. We investigate the importance of such factors in the crystallization process of gold, silver, and…

Statistical Mechanics · Physics 2024-07-09 Arthur France-Lanord , Sarath Menon , Julien Lam

Atomically precise thiolate-stabilized gold nanoclusters are currently of interest for many cross-disciplinary applications in chemistry, physics and molecular biology. Very recently, synthesis and electronic properties of "nanoalloy"…

Atomic and Molecular Clusters · Physics 2011-09-05 Sami Malola , Hannu Häkkinen

Traditionally, the condensation sequence of circumstellar dust is predicted based on the thermodynamic stabilities of specific condensates in the macroscopic bulk phase. However, at the (sub-)nanometer scale clusters with non-crystalline…

Astrophysics of Galaxies · Physics 2025-10-16 David Gobrecht

Low-energy deposition of neutral Pd_N clusters (N=2-7 and 13) on a MgO(001) surface F-center (FC) was studied by spin-density-functional molecular dynamics simulations. The incident clusters are steered by an attractive "funnel" created by…

Materials Science · Physics 2009-11-07 M. Moseler , H. Hakkinen , U. Landman

We report on the structures of aluminum hydrides derived from a tetrahedral aluminum Al4 cluster using ab initio quantum chemical calculation. Our calculation of binding energies of the aluminum hydrides reveals that stability of these…

Atomic and Molecular Clusters · Physics 2011-09-15 Kazuhide Ichikawa , Yuji Ikeda , Ayumu Wagatsuma , Kouhei Watanabe , Pawel Szarek , Akitomo Tachibana

This paper presents a broad theoretical and simulation study of the high temperature behavior of crystalline alkali halide surfaces typified by NaCl(100), of the liquid NaCl surface near freezing, and of the very unusual partial wetting of…

Materials Science · Physics 2007-05-23 T. Zykova-Timan , D. Ceresoli , U. Tartaglino , E. Tosatti

Gold nanoclusters have been the focus of numerous computational studies but an atomistic understanding of their structural and dynamical properties at finite temperature is far from satisfactory. To address this deficiency, we investigate…

Mesoscale and Nanoscale Physics · Physics 2018-11-13 Diego Guedes-Sobrinho , Weiqi Wang , Ian Hamilton , Juarez L. F. Da Silva , Luca M. Ghiringhelli

A systematic, decoration-based technique to discover the atomic structure of a decagonal quasicrystal, given pair potentials and experimentally measured lattice constants, is applied to the ``basic'' cobalt-rich decagonal Al-Co-Ni…

Materials Science · Physics 2007-05-23 Nan Gu , M. Mihalkovic , C. L. Henley

We simulate structure in the vicinity of different size nanovoids using a new variant of the Molecular Statics, wherein atomic structure in the vicinity of nanovoids and the parameters that define the displacements of atoms placed in…

Materials Science · Physics 2022-02-02 A. V. Nazarov , A. P. Melnikov , A. A. Mikheev , I. V. Ershova

Alumina ultrathin films obtained by high temperature oxidation of a Ni$_3$Al (111) surface are a good template to grow regular arrays of metal clusters. Up to now two hexagonal organizations called 'dot' and 'network' structures have been…

Chemical Physics · Physics 2020-10-26 Georges Sitja , Aude Bailly , Maurizio de Santis , Vasile Heresanu , Claude Henry

While the growth of germanene has been claimed on many substrates, the exact crystal structures remain controversial. Here, we systematically explore the possible structures formed by Ge deposition onto Al(111) surface by combining…

Materials Science · Physics 2022-08-17 Feini Yan , Shaogang Xu , Chao He , Changchun He , Changming Zhao , Hu Xu

Geometry, electronic structure, and magnetic properties of methylthiolate-stabilized Au$_{25}$L$_{18}$ and MnAu$_{24}$L$_{18}$ (L = SCH$_3$) clusters adsorbed on noble-metal (111) surfaces have been investigated by using spin-polarized…

Atomic and Molecular Clusters · Physics 2015-06-03 Xi Chen , Mikkel Strange , Hannu Hakkinen

A rule due to Bravais of wide validity for crystals is that their surfaces correspond to the densest planes of atoms in the bulk of the material. Comparing a theoretical model of i-AlPdMn with experimental results, we find that this…

Materials Science · Physics 2009-11-10 Z. Papadopolos , P. Pleasants , G. Kasner , V. Fournee , T. Cai , C. Jenks , P. Thiel , J. Ledieu , R. McGrath