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Molecular dynamics simulations were conducted to investigate the structural properties of melts of nonconcatenated ring polymers and compared to melts of linear polymers. The longest rings were composed of N=1600 monomers per chain which…

Soft Condensed Matter · Physics 2011-05-02 Jonathan D. Halverson , Won Bo Lee , Gary S. Grest , Alexander Y. Grosberg , Kurt Kremer

Static structure factors are computed for large-scale, mechanically stable, jammed packings of frictionless spheres (three dimensions) and disks (two dimensions) with broad, power-law size dispersity characterized by the exponent $-\beta$.…

Soft Condensed Matter · Physics 2023-09-06 Joseph M. Monti , Ishan Srivastava , Leonardo E. Silbert , Jeremy B. Lechman , Gary S. Grest

In polymer physics it is typically assumed that excluded volume interactions are effectively screened in polymer melts. Hence, chains could be described by an effective random walk without excluded volume interactions. In this letter, we…

Soft Condensed Matter · Physics 2017-10-31 Hendrik Meyer , Eric Horwath , Peter Virnau

Molecular dynamics simulations were conducted to investigate the dynamic properties of melts of nonconcatenated ring polymers and compared to melts of linear polymers. The longest rings were composed of N=1600 monomers per chain which…

Soft Condensed Matter · Physics 2011-05-02 Jonathan D. Halverson , Won Bo Lee , Gary S. Grest , Alexander Y. Grosberg , Kurt Kremer

We present a Monte Carlo algorithm that provides efficient and unbiased sampling of polymer melts consisting of two chains of equal length that jointly visit all the sites of a cubic lattice with rod geometry L x L x rL and non-periodic…

Statistical Mechanics · Physics 2010-11-03 Jesper Lykke Jacobsen

We describe method to discuss thermodynamics of a defected semi-flexible homo-polymer chain in the two and three dimensions using fully directed self-avoiding walk lattice model. The defects are located along a line and these defects are…

Soft Condensed Matter · Physics 2020-11-23 Pramod Kumar Mishra

The nematic ordering in semiflexible polymers with contour length $L$ exceeding their persistence length $\ell_p$ is described by a confinement of the polymers in a cylinder of radius $r_{eff}$ much larger than the radius $r_\rho$, expected…

Soft Condensed Matter · Physics 2016-05-11 Sergei A. Egorov , Andrey Milchev , Kurt Binder

We study $D$-dimensional polymerized membranes embedded in $d$ dimensions using a self-consistent screening approximation. It is exact for large $d$ to order $1/d$, for any $d$ to order $\epsilon=4-D$ and for $d=D$. For flat physical…

Condensed Matter · Physics 2009-01-23 Pierre Le Doussal , Leo Radzihovsky

We systematically explore the self-assembly of semi-flexible polymers in deformable spherical confinement across a wide regime of chain stiffness, contour lengths and packing fractions by means of coarse-grained molecular dynamics…

Soft Condensed Matter · Physics 2021-07-12 Maxime M. C. Tortora , Daniel Jost

A cornerstone of modern polymer physics is the `Flory ideality hypothesis' which states that a chain in a polymer melt adopts `ideal' random-walk-like conformations. Here we revisit theoretically and numerically this pivotal assumption and…

Soft Condensed Matter · Physics 2015-06-25 J. P. Wittmer , P. Beckrich , J. Johner , A. N. Semenov , S. P. Obukhov , H. Meyer , J. Baschnagel

Polymer chains composing a polymer solution in strict two dimensions (2D) are characterized with irregular domain boundaries, whose fractal dimension ($\mathcal{D}^{\partial}$) varies with the area fraction of the solution and the solvent…

Soft Condensed Matter · Physics 2023-12-15 Lei Liu , Changbong Hyeon

We present Monte Carlo simulations of semidilute solutions of long self-attracting chain polymers near their Ising type critical point. The polymers are modeled as monodisperse self-avoiding walks on the simple cubic lattice with attraction…

Soft Condensed Matter · Physics 2009-10-30 H. Frauenkron , P. Grassberger , HLRZ Juelich , Germany

Following Flory's ideality hypothesis the chemical potential of a test chain of length $n$ immersed into a dense solution of chemically identical polymers of length distribution P(N) is extensive in $n$. We argue that an additional…

Soft Condensed Matter · Physics 2009-12-18 J. P. Wittmer , A. Johner , A. Cavallo , P. Beckrich , F. Crevel , J. Baschnagel

Some recent work pointed out the usefulness of taking a large-deviation perspective when trying to extract anything resembling a macroscopic order parameter from a computer simulation. In this paper we note that the end-to-end distance of…

Soft Condensed Matter · Physics 2026-03-20 Eleftherios Mainas , Jan Tobochnik , Richard Stratt

The conformational statistics of ring polymers in melts or dense solutions is strongly affected by their quenched microscopic topological state. The effect is particularly strong for non-concatenated unknotted rings, which are known to…

Soft Condensed Matter · Physics 2015-06-17 Angelo Rosa , Ralf Everaers

We calculate the mean end-to-end distance ($R$) of a self-avoiding polymer encapsulated in an infinitely long cylinder with radius $D$. A self-consistent perturbation theory is used to calculate $R$ as a function of $D$ for impenetrable…

Soft Condensed Matter · Physics 2016-08-31 G. Morrison , D. Thirumalai

The interplay of topological constraints and persistence length of ring polymers in their own melt is investigated by means of dynamical Monte Carlo simulations of a three dimensional lattice model. We ask if the results are consistent with…

Statistical Mechanics · Physics 2009-10-31 M. Muller , J. P. Wittmer , M. E. Cates

We present a numerical study of 2D random-bond Potts ferromagnets. The model is studied both below and above the critical value $Q_c=4$ which discriminates between second and first-order transitions in the pure system. Two geometries are…

Statistical Mechanics · Physics 2009-10-31 Christophe Chatelain , Bertrand Berche

Colloidal patchy particles with divalent attractive interaction can self-assemble into linear polymer chains. Their equilibrium properties in 2D and 3D are well described by Wertheim's thermodynamic perturbation theory which predicts a…

Soft Condensed Matter · Physics 2022-09-21 H. J. Jonas , P. Schall , P. G. Bolhuis

Drawing inspiration from the concept of the "primitive path" of a linear chain in melt conditions, we introduce here a numerical protocol which allows us to detect, in an unambiguous manner, the "primitive shapes" of ring polymers in…

Soft Condensed Matter · Physics 2025-11-26 Mattia A. Ubertini , Angelo Rosa