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Low-frequency Raman scattering experiments have been performed on thin films consisting of nickel-silver composite nanoparticles embedded in alumina matrix. It is observed that the Raman scattering by the quadrupolar modes, strongly…

Condensed Matter · Physics 2007-05-23 H. Portales , L. Saviot , E. Duval , M. Gaudry , E. Cottancin , M. Pellarin , J. Lerme , M. Broyer

The purpose of this work is to calculate the vibrational modes of an elastically anisotropic sphere embedded in an isotropic matrix. This has important application to understanding the spectra of low-frequency Raman scattering from…

Mesoscale and Nanoscale Physics · Physics 2010-09-29 L. Saviot , D. B. Murray , E. Duval , A. Mermet , S. Sirotkin , M. C. Marco de Lucas

The acoustic vibrations of single monomers and dimers of gold nanoparticles were investigated by measuring for the first time their ultra-low frequency micro-Raman scattering. This experiment provides access not only to the frequency of the…

We calculate low-frequency Raman scattering from the confined acoustic phonon modes of CdS1-xSex nanoparticles embedded in borosilicate glass. The calculation of the Raman scattering by acoustic phonons in nanoparticles has been performed…

Mesoscale and Nanoscale Physics · Physics 2009-04-16 Sanjeev K. Gupta , Prafulla K. Jha , Satyaprakash Sahoo , A. K. Arora , Y. M. Azhniuk

Transient absorption and Raman scattering measurements on noble metal nanoparticles offer complimentary information on their vibrational modes and mechanical interactions with their surroundings. We have developed a comprehensive modeling…

Mesoscale and Nanoscale Physics · Physics 2024-10-29 Rachel Gelfand , Matthew Pelton

Acoustic vibrations of nanoparticles made of materials with anisotropic elasticity and nanoparticles with non-spherical shapes are theoretically investigated using a homogeneous continuum model. Cubic, hexagonal and tetragonal symmetries of…

Mesoscale and Nanoscale Physics · Physics 2009-06-02 Lucien Saviot , Daniel B. Murray

A theoretical model of resonant hyper-Raman scattering by an ensemble of spherical semiconductor quantum dots has been developed. The electronic intermediate states are described as Wannier-Mott excitons in the framework of the envelope…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 E. Menendez-Proupin , C. Trallero-Giner , A. Garcia-Cristobal

Revealing hidden non-radiative (dark) of resonant nanostructures using optical methods such as dark-field spectroscopy often becomes a sophisticated problem due to a weak coupling of these modes with a far-field radiation, whereas methods…

Vibrational mode frequencies and damping are calculated for an elastic sphere embedded in an infinite, homogeneous, isotropic elastic medium. Anisotropic elasticity of the sphere significantly shifts the frequencies in comparison to…

Materials Science · Physics 2007-05-23 Lucien Saviot , Daniel B Murray , Maria Del Carmen Marco De Lucas

Enhancement of optical response with high-index dielectric nanoparticles is attributed to the excitation of their Mie-type magnetic and electric resonances. Here we study Raman scattering from crystalline silicon nanoparticles and reveal…

Phonon modes found in low frequency Raman scattering from $CdS_{1-x}Se_x$ nanocrystals embedded in borosilicate glass arising from confined acoustic phonons are investigated. In addition to the breathing modes and quadrupolar modes, two…

Materials Science · Physics 2008-03-10 Sanjeev K. Gupta , Satyaprakash Sahoo , Prafulla K. Jha , A. K. Arora , Y. M. Azhniuk

Experiments have shown that the internal vibrational state of a molecule can affect the intensity of high harmonic light generated from that molecule. This paper presents a model which explains this modulation in terms of interference…

Atomic Physics · Physics 2015-05-13 Zachary B. Walters , Stefano Tonzani , Chris H. Greene

Raman spectroscopy is a useful experimental tool to investigate local deformation and structural changes in SiO$_2$-based glasses. Using a semi-classical modelling of Raman spectra in large samples of silica glasses, we show in this paper…

Disordered Systems and Neural Networks · Physics 2015-02-04 Nikita S. Shcheblanov , Boris Mantisi , Paolo Umari , Anne Tanguy

Resonantly enhanced Raman scattering in dielectric nanostructures has been recently proven to be an effcient tool for developing nanothermometry and experimental determination of their mode- composition. In this paper, we develop a rigorous…

Optics · Physics 2018-02-14 Kristina Frizyuk , Mehedi Hasan , Alex Krasnok , Andrea Alu , Mihail Petrov

The spectrum of acoustic vibrational modes of an inhomogeneous elastic continuum are analyzed with application to a spherical nanoparticle embedded in an infinite glass block. The relationship of these modes to the discrete vibrational…

Materials Science · Physics 2007-05-23 Daniel B. Murray , Lucien Saviot

We treat resonant Raman scattering via the multiphonon exciton transitions in cylindrical quantum dots with a parabolic confinement in the lateral direction and with a finite rectangular interface-barrier confinement in the axial direction.…

Mesoscale and Nanoscale Physics · Physics 2012-05-09 S. N. Klimin , V. M. Fomin , J. T. Devreese , J. -P. Leburton

A theoretical model describing the Raman scattering process in atomic vapors is constructed. The treatment investigates the low-excitation regime suitable for modern experimental applications. Despite the incorporated decoherence effects…

Quantum Physics · Physics 2012-07-16 Jan Kolodynski , Jan Chwedenczuk , Wojciech Wasilewski

Highly ordered periodic arrays of silver nanoparticles have been fabricated which exhibit surface plasmon resonances in the visible spectrum. We demonstrate the ability of these structures to alter the fluorescence properties of vicinal dye…

Other Condensed Matter · Physics 2009-11-13 Nic Cade , Tom Ritman-Meer , David Richards

The Raman intensity can be well described by the famous Albrecht equation that consists of A and B terms. It is well known that the contribution from Albrecht's A term can be neglected without loss of accuracy for far off-resonant Raman…

Optics · Physics 2015-11-11 Zu-Yong Gong , Guangjun Tian , Sai Duan , Yi Luo

In our recent paper [Phys. Rev. B 65, 075316 (2002)], the selection rules for the Raman scattering in spherical nanocrystals are analyzed. Here we show, that a physically expedient choice of the coordinate system, related to the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 E. P. Pokatilov , S. N. Klimin , V. M. Fomin , J. T. Devreese , F. W. Wise
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