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The structural and magnetic properties of the hexagonal four-layer form of SrMnO$_3$ have been investigated by combining magnetization measurements, electron diffraction and high-resolution synchrotron X-ray and neutron powder diffraction.…

Strongly Correlated Electrons · Physics 2007-05-23 A. Daoud-Aladine , C. Martin , L. C. Chapon , M. Hervieu , K. S. Knight , M. Brunelli , P. G. Radaelli

Density functional band calculations have been performed to study LaNiO$_3$/LaAlO$_3$ superlattices. Motivated by recent experiments reporting the magnetic and metal-insulator phase transition as a function of LaNiO$_3$ layer thickness, we…

Strongly Correlated Electrons · Physics 2012-07-30 Myung Joon Han , Michel van Veenendaal

The electronic structure of La0.8Sr0..2MnO3/SrTiO thin film, which was prepared by Laser MBE, was studied by X-ray photoemission spectra (XPS) in the temperature interval of 300 to 1000 K. Experimental results showed that the electronic…

Strongly Correlated Electrons · Physics 2007-05-23 Guotai Tan , S. Dai , P. Duan , H. B. Lu , K. Xie , Y. L. Zhou , Z. H. Chen

Hybrid nanoparticles allow exploiting the interplay of confinement, proximity between different materials and interfacial effects. However, to harness their properties an in-depth understanding of their (meta)stability and interfacial…

The effects of the cooperative Jahn-Teller effect on the crystal structure and the stability of the charge ordered (CO) state were studied by measurements of powder X-ray diffraction, resistivity, and ultrasound for Pr1-xCaxMnO3…

Strongly Correlated Electrons · Physics 2009-11-10 R. K. Zheng , G. Li , Y. Yang , A. N. Tang , W. Wang , T. Qian , X. G. Li

LaTiO$_3$ is known as Mott-insulator which orders antiferromagnetically at $T_{\rm N}=146$ K. We report on results of thermal expansion and temperature dependent x-ray diffraction together with measurements of the heat capacity, electrical…

Using spin-density functional theory we investigated various possible structures of the hematite (0001) surface. Depending on the ambient oxygen partial pressure, two geometries are found to be particularly stable under thermal equilibrium:…

Materials Science · Physics 2009-10-31 X. -G. Wang , W. Weiss , Sh. K. Shaikhutdinov , M. Ritter , M. Petersen , F. Wagner , R. Schloegl , M. Scheffler

The electronic structure and thermodynamic stability of tetragonal $\rm{BiFeO_3}$(001) surfaces have been investigated using density functional theory. In this work, four different structures having different lattice constants with two…

Materials Science · Physics 2022-05-13 Soumyasree Jena , Sanjoy Datta

Using the multiband $d-p$ model and unrestricted Hartree-Fock approximation we investigate the electronic structure and spin-orbital order in three-dimensional MnO$_3$ lattice such as realized in LaMnO$_3$. The orbital order is induced and…

Strongly Correlated Electrons · Physics 2019-04-04 Krzysztof Rościszewski , Andrzej M. Oleś

Cooperative Jahn-Teller ordering is well-known to drive the cubic $Fd\overline{3}m$ to tetragonal $I$4$_1$/$amd$ structural distortion in Mn$_3$O$_4$ at 1170 $^{\circ}$C. Further structural distortion occurs in Mn$_3$O$_4$ upon magnetic…

Materials Science · Physics 2014-08-26 Moureen C. Kemei , Jaye K. Harada , Ram Seshadri , Matthew R. Suchomel

Exotic quantum phases, arising from a complex interplay of charge, spin, lattice and orbital degrees of freedom, are of immense interest to a wide research community. A well-known example of such an entangled behavior is the Jahn-Teller…

The multi-order Raman scattering is studied up to a fourth order for a detwinned LaMnO_3 crystal. Based on a comprehensive data analysis of the polarisation-dependent Raman spectra, we show that the anomalous features in the multi-order…

We propose a mechanism for A-type antiferromagnetism in orthorombic LaMnO_3, compatible with the large Jahn-Teller splitting inferred from structural data. Orbital ordering resulting from Jahn-Teller distortions effectively leads to A-type…

Strongly Correlated Electrons · Physics 2009-10-30 D. Feinberg , P. Germain , M. Grilli , G. Seibold

The possible role of the van Hove singularity (vHs) in stabilizing the low-temperature orthorhombic (LTO) phase transition in La$_{2-x}$\-Sr$_x$\-CuO$_ 4$ (LSCO) is discussed. It is found that the vHs can drive a structural distortion in…

Condensed Matter · Physics 2009-10-22 R. S. Markiewicz

The structural, dielectric and dynamical properties of the low temperature antiferromagnetic orthorhombic phase of CaMnO$_3$ have been computed from first principles using a density functional theory approach within the local spin density…

Materials Science · Physics 2009-11-13 Satadeep Bhattacharjee , Eric Bousquet , Philippe Ghosez

By combining ab initio simulations including an on-site Coulomb repulsion term and Boltzmann theory, we explore the thermoelectric properties of (LaNiO$_3$)$_n$/(LaAlO$_3$)$_n$(001) superlattices ($n=1,3$) and identify a strong dependence…

Materials Science · Physics 2018-05-17 Benjamin Geisler , Rossitza Pentcheva

Based on previously computed parameters for the electron-phonon couplings and the Coulomb exchange, we compute and classify the static Jahn-Teller distortions, i.e. the minima of the lowest adiabatic potential energy surface, of C60(n+),…

Strongly Correlated Electrons · Physics 2015-06-24 Martin Lueders , Nicola Manini

The Mn-terminated (001) surface of the stable anti-ferromagnetic insulating phase of cubic perovskite CaMnO$_3$ is found to undergo a magnetic reconstruction consisting on a spin-flip process at surface: each Mn spin at the surface flips to…

Materials Science · Physics 2009-10-31 Alessio Filippetti , Warren E. Pickett

The structural, magnetic and resistive properties of (La1-yYy)FeAsO compounds (y = 0.10, 0.20, 0.30) have been investigated by means of X-ray and neutron powder diffraction as well as by resistivity measurements. The temperatures at which…

Materials Science · Physics 2015-05-14 A. Martinelli , A. Palenzona , M. Tropeano , C. Ferdeghini , M. R. Cimberle , C. Ritter

The Mn spin correlations were studied near the O'-O phase transition at T{JT} = 750 K, up to 950 K with 17O and 139La NMR in a stoichiometric LaMnO3 crystalline sample. The measured local hyperfine fields originate from the electron density…

Strongly Correlated Electrons · Physics 2015-06-15 A. Trokiner , S. Verkhovskii , A. Gerashenko , Z. Volkova , O. Anikeenok , K. Mikhalev , M. Eremin