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Competing interactions stabilize exotic mesoscopic structures, yet the microscopic mechanisms by which they influence non-equilibrium processes leading to disordered states remain largely unexplored, despite their critical role in…

Soft Condensed Matter · Physics 2025-05-13 Joeri Opdam , Michio Tateno , Hajime Tanaka

We study the effective electrostatic interactions between a pair of charged colloidal particles without salt ions while the system is confined in two dimensions. In particular we use a simplified model to elucidate the effects of rotational…

Soft Condensed Matter · Physics 2010-09-09 Chi-Lun Lee , Sio-Kit Ng

We study the aging dynamics in a model for dense simple liquids, in which particles interact through a hard-core repulsion complemented by a short-ranged attractive potential, of the kind found in colloidal suspensions. In this system, at…

Statistical Mechanics · Physics 2007-05-23 G. Foffi , E. Zaccarelli , S. Buldyrev , F. Sciortino , P. Tartaglia

Electrostatic repulsions can drive crystallization in many-particle systems. For charged colloidal systems, the phase boundaries as well as crystal structure are highly tunable by experimental parameters such as salt concentration and pH.…

Soft Condensed Matter · Physics 2016-03-17 Jeffrey Everts , Niels Boon , René van Roij

In this Rapid Communication we demonstrate the applicability of an augmented Gibbs ensemble Monte Carlo approach for the phase behavior determination of model colloidal systems with short-ranged depletion attraction and long-ranged…

Soft Condensed Matter · Physics 2007-05-23 P. Charbonneau , D. R. Reichman

We study metastable clusters in a colloidal system with competing interactions. A short-ranged polymer-induced attraction drives clustering, while a weak, long-ranged electrostatic repulsion prevents extensive aggregation. We compare…

We study the structure of clusters in a model colloidal system with competing interactions using Brownian dynamics simulations. A short-ranged attraction drives clustering, while a weak, long-ranged repulsion is used to model electrostatic…

Soft Condensed Matter · Physics 2010-10-05 Alex Malins , Stephen R. Williams , Jens Eggers , Hajime Tanaka , C. Patrick Royall

The dynamical arrest of attractive colloidal particles into out-of-equilibrium structures, known as gelation, is central to biophysics, materials science, nanotechnology, and food and cosmetic applications, but a complete understanding is…

Soft Condensed Matter · Physics 2020-07-22 Joep Rouwhorst , Christopher Ness , Simeon Stoyanov , Alessio Zaccone , Peter Schall

Within the framework of the mode-coupling theory of super-cooled liquids, we investigate new phenomena in colloidal systems on approach to their glass transitions. When the inter-particle potential contains an attractive part, besides the…

Soft Condensed Matter · Physics 2009-11-07 K. A. Dawson , G. Foffi , F. Sciortino , P. Tartaglia , E. Zaccarelli

In colloidal suspensions, the competition between attractive and repulsive interactions gives rise to a rich and complex phenomenology. Here, we study the equilibrium phase diagram of a model system using a DLVO interaction potential by…

Soft Condensed Matter · Physics 2009-11-11 A. de Candia , E. Del Gado , A. Fierro , N. Sator , M. Tarzia , A. Coniglio

We present simulation results addressing the dynamics of a colloidal system with attractive interactions close to gelation. Our interaction also has a soft, long range repulsive barrier which suppresses liquid-gas type phase separation at…

Soft Condensed Matter · Physics 2007-05-23 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

We study the rheological properties of colloidal microphases in two dimensions simulating a model of colloidal particles with competing interactions. Due to the competition between short-range attraction and long-range repulsion, as a…

Soft Condensed Matter · Physics 2009-11-13 A. Imperio , L. Reatto , S. Zapperi

The addition of enough non-adsorbing polymer to an otherwise stable colloidal suspension gives rise to a variety of phase behavior and kinetic arrest due to the depletion attraction induced between the colloids by the polymers. We report a…

Soft Condensed Matter · Physics 2024-06-19 Sam E Griffiths , Nick Koumakis , Aidan T Brown , Teun Vissers , Patrick B Warren , Wilson C K Poon

We present molecular dynamics simulations of aggregation kinetics in a colloidal suspension modeled as a highly asymmetric binary mixture. Starting from a configuration with largely uncorrelated colloidal particles the system relaxes by…

Statistical Mechanics · Physics 2007-05-23 Sorin Bastea

Charged colloids can form ordered structures like Wigner crystals or glasses at very low concentrations due to long-range electrostatic repulsions. Here, we combine small-angle x-ray scattering (SAXS) and optical experiments with…

Soft Condensed Matter · Physics 2025-03-19 Hanna Anop , Laura Dal Compare , Frederic Nallet , Achille Giacometti , Eric Grelet

Colloid-polymer mixtures may undergo either fluid-fluid phase separation or gelation. This depends on the depth of the quench (polymer concentration) and polymer-colloid size ratio. We present a real-space study of dynamics in phase…

Soft Condensed Matter · Physics 2012-09-19 Isla Zhang , C. Patrick Royall , Paul Bartlett , Malcolm A. Faers

Using computer simulations, we study the dynamic arrest in a schematic model of colloid-polymer mixtures combining short-ranged attractions with long-ranged repulsions. The arrested gel is a dilute rigid network of colloidal particles…

Soft Condensed Matter · Physics 2018-08-17 David Richard , C. Patrick Royall , Thomas Speck

We numerically study a simple model for thermo-reversible colloidal gelation in which particles can form reversible bonds with a predefined maximum number of neighbors. We focus on three and four maximally coordinated particles, since in…

We study a two-dimensional model for interacting colloidal particles which displays spontaneous clustering. Within this model we investigate the competition between the pinning to a periodic corrugation potential, and a sideways constant…

Soft Condensed Matter · Physics 2018-05-23 Mirko Rossini , Lorenzo Consonni , Andrea Stenco , Luciano Reatto , Nicola Manini

The recent observation of an electronic cluster glass state composed of random domains with unidirectional modulation of charge density and/or spin density on Bi_{2}Sr_{2}CaCu_{2}O_{8+\delta} reinvigorates the debate of existence of…

Superconductivity · Physics 2011-10-31 Chung-Pin Chou , Noboru Fukushima , Ting Kuo Lee