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We present a multi-aperture analyser set-up for performing X-ray phase contrast imaging in planar and three-dimensional modalities. A multi-slice representation of the sample is used to establish a quantitative relation between projection…

Instrumentation and Detectors · Physics 2017-06-21 M. Endrizzi , F. A. Vittoria , L. Rigon , D. Dreossi , A. Olivo

X-ray absorption spectroscopy (XAS) and resonant inelastic X-ray scattering (RIXS) are powerful probes of electronic structure owing to their chemical and orbital selectivity. For powder samples, however, interpreting RIXS spectral…

Materials Science · Physics 2026-05-12 Sihan Zhang , Oana Bunău , Marius Retegan , Pieter Glatzel

We theoretically analyze the intensity of the resonant inelastic X-ray scattering (RIXS) based on Ansatz that the electron is fractionalized into two components. By fitting the angle resolved photoemission spectroscopy (ARPES) data of a…

Strongly Correlated Electrons · Physics 2021-07-26 Masatoshi Imada

The Frenkel exciton model was adapted to describe X-ray absorption and resonant inelastic scattering spectra of polynuclear transition metal complexes by means of restricted active space self-consistent field method. The proposed approach…

Chemical Physics · Physics 2016-06-07 Marie Preuße , Sergey I. Bokarev , Saadullah G. Aziz , Oliver Kühn

To fully capitalize on the potential and versatility of resonant inelastic x-ray scattering (RIXS), it is essential to develop the capability to interpret different RIXS contributions through calculations, including the dependence on…

X-ray absorption spectroscopy (XAS) is a powerful experimental technique to probe the local order in materials with core electron excitations. Experimental interpretation requires supporting theoretical calculations. For water, these…

Computational Physics · Physics 2022-05-17 Fujie Tang , Zhenglu Li , Chunyi Zhang , Steven G. Louie , Roberto Car , Diana Y. Qiu , Xifan Wu

The Am $5d$-$5f$ resonant inelastic x-ray scattering (RIXS) data of americium sesquioxide were measured at incident photon energies throughout the Am $O_{4,5}$ edges. The experiment was supported by calculations using several model…

Strongly Correlated Electrons · Physics 2023-09-06 Sergei M. Butorin , David K. Shuh

We theoretically examine the momentum dependence of resonant inelastic x-ray scattering (RIXS) spectrum for one-dimensional and two-dimensional cuprates based on the single-band Hubbard model with realistic parameter values. The spectrum is…

Strongly Correlated Electrons · Physics 2007-05-23 T. Tohyama , K. Tsutsui , S. Maekawa

Resonance anomalous surface x-ray scattering (RASXS) technique was applied to electrochemical interface studies. It was used to determine the chemical states of electrochemically formed anodic oxide monolayers on platinum surface. It is…

Inelastic neutron and X-ray scattering experiments on surfaces and interfaces are a challenging topic in modern physics. Particular interest arises regarding surfaces and interfaces of soft matter and biological systems. We review both…

Biological Physics · Physics 2009-10-02 Maikel C. Rheinstädter , Tilo Seydel , Bela Farago , Tim Salditt

The real-space multiple-scattering (RSMS) approach is applied to model non-resonant inelastic scattering from deep core electron levels over a broad energy spectrum. This approach is applicable to aperiodic or periodic systems alike and…

Other Condensed Matter · Physics 2009-11-11 J. A. Soininen , A. L. Ankudinov , J. J. Rehr

Resonant Inelastic X-ray Scattering (RIXS), which probes the occupied and unoccupied electronic subspaces in an interrelated fashion, is one of the most detailed, complex and information-rich experimental techniques employed in the…

Materials Science · Physics 2022-09-16 Subhayan Roychoudhury , David Prendergast

X-ray absorption (XAS) and Resonant Inelastic X-ray Scattering (RIXS) spectra of LaPt$_2$Si$_2$ single crystal at the Si L and La N edges are presented. The data are interpreted in terms of density functional theory, showing that the Si…

X-ray absorption fine structure (XAFS) and x-ray emission spectroscopy (XES) are advanced x-ray spectroscopies that impact a wide range of disciplines. However, unlike the majority of other spectroscopic methods, XAFS and XES are…

X-ray spectroscopy has been a key method to determine ground and excited state properties of quantum materials with atomic specificity. Now, new x-ray facilities are opening the door to the study of pump-probe x-ray spectroscopy -…

Strongly Correlated Electrons · Physics 2025-02-11 Daniel Jost , Eder G. Lomeli , Ta Tang , Joshua J. Kas , John J. Rehr , Wei-Sheng Lee , Hong-Chen Jiang , Brian Moritz , Thomas P. Devereaux

A method to calculate particle fluxes applicable in most of the spectroscopy techniques is described. Flux intensities of backscattered or absorbed electrons and emitted photons are calculated using a method of convergence to solve the…

Materials Science · Physics 2015-06-05 C. Figueroa , N. Nieva , H. Brizuela , S. P. Heluani

X-ray photon correlation spectroscopy (XPCS) allows for the resolution of dynamic processes within a material across a wide range of length and time scales. X-ray speckle visibility spectroscopy (XSVS) is a related method that uses a single…

Numerical Analysis · Mathematics 2023-01-09 Shaswat Mohanty , Christopher B. Cooper , Hui Wang , Mengning Liang , Wei Cai

We theoretically demonstrate that a resonant inelastic x-ray scattering (RIXS) with a sizable momentum transfer can be utilized to study valence band dispersion for broad band materials. We take RIXS at the Si K edge of 3C-SiC as a typical…

Materials Science · Physics 2009-09-21 Yunori Nisikawa , Muneharu Ibuki , Manabu Usuda

We study resonant x-ray scattering (RXS) at Np M_{4,5} edges in the triple-\textbf{k} multipole ordering phase in NpO_{2}, on the basis of a localized electron model. We derive an expression for RXS amplitudes to characterize the spectra…

Strongly Correlated Electrons · Physics 2015-06-25 Tatsuya Nagao , Jun-ichi Igarashi

A new method to calculate the spectrum using cascaded open systems and master equations is presented. The method uses two state analyzer atoms which are coupled to the system of interest, whose spectrum of radiation is read from the…

Quantum Physics · Physics 2015-06-26 Martti Havukainen , Stig Stenholm