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We present a first-principles study of the large magneto-crystalline anisotropy in the intercalated di-chalcogenide material \ce{Fe_{0.25}TaS_2}, investigated with the DFT+U approach. We verify a uniaxial magnetocrystalline anisotropy…

Strongly Correlated Electrons · Physics 2016-05-24 Vaideesh Loganathan , Jian-Xin Zhu , Andriy H. Nevidomskyy

We have studied the magnetic behavior of dextran-coated magnetite (Fe$_3$O$_4$) nanoparticles with median particle size $\left<d\right>=8$ $nm$. Magnetization curves and in-field M\"ossbauer spectroscopy measurements showed that the…

Materials Science · Physics 2007-05-23 E. Lima , A. L. Brandl , A. D. Arelaro , G. F. Goya

The layered material Mn$_3$Si$_2$Te$_6$, with alternating stacking honeycomb and triangular layers, is attracting considerable attention due to its rich physical properties. Here, using density functional theory and classical Monte Carlo…

Strongly Correlated Electrons · Physics 2023-02-23 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Elbio Dagotto

A hallmark of the iron-based superconductors is the strong coupling between magnetic, structural and electronic degrees of freedom. However, a universal picture of the normal state properties of these compounds has been confounded by recent…

We perform density functional calculations to investigate the structure of the inter-metallic alloy FeRh under epitaxial strain. Bulk FeRh exhibits a metamagnetic transition from a low-temperature antiferromagnetic (AFM) phase to a…

Materials Science · Physics 2016-07-20 Ulrich Aschauer , Roisin Braddell , Sonia A. Brechbühl , Peter M. Derlet , Nicola A. Spaldin

Fe-doped III-V ferromagnetic semiconductors (FMSs) such as (In,Fe)As, (Ga,Fe)Sb, (In,Fe)Sb, and (Al,Fe)Sb are promising materials for spintronic device applications because of the availability of both n- and p-type materials and the high…

In 3d-electron magnetic systems, the magnetic structures that transform each other by spin rotation have very close degenerate energies due to small spin-orbit coupling and can be easily controlled by chemical substitution and external…

Materials Science · Physics 2025-11-20 Vu Thi Ngoc Huyen , Yuki Yanagi , Michi-To Suzuki

The magnetic and electronic properties of the layered Zintl-phase compound EuAl$_2$Ge$_2$ crystallizing in the trigonal CaAl$_2$Si$_2$-type structure are reported. Our neutron-diffraction measurements show that EuAl$_2$Ge$_2$ undergoes…

We use density functional theory to investigate effects of spin-orbit coupling and single-stripe-type antiferromagnetic (sAFM) ordering on the crystal structure and electronic properties of SmFeAsO. The results indicate that AFM ordering…

Superconductivity · Physics 2024-03-05 Toktam Morshedloo , Ali Kazempour , Hamideh Shakeripour , S. Javad Hashemifar , Mojtaba Alaei

Enhancement of magnetism of Fe that occurs by alloying with Cr or V is discussed on the basis of first-principles electronic structure calculation. The d states of Fe next to Cr(V) are pushed down to the lower energy side compared to those…

Materials Science · Physics 2011-10-04 Masako Ogura , Hisazumi Akai , Junjiro Kanamori

We study the effects of the exchange interaction between an adsorbed magnetic atom with easy-axis magnetic anisotropy and the conduction-band electrons from the substrate. We model the system using an anisotropic Kondo model and we compute…

Mesoscale and Nanoscale Physics · Physics 2010-08-10 Rok Zitko , Thomas Pruschke

Anisotropic antiferromagnetic systems of dimensionality greater than one in an external field are shown to exhibit a complicated array of ground states depending on the spin structure of the surface. The simplest structure that exhibits…

Materials Science · Physics 2009-11-10 B. A. Ivanov , C. E. Zaspel , A. Yu. Merkulov

Anisotropic magnetoresistance (AMR), originating from spin-orbit coupling (SOC), is the sensitivity of the electrical resistance in magnetic systems to the direction of spin magnetization. Although this phenomenon has been experimentally…

Materials Science · Physics 2020-08-12 Dongzhe Li , Fabian Pauly , Alexander Smogunov

Iridates such as Sr$_2$IrO$_4$ are of considerable interest owing to the formation of the Mott insulating state driven by a large spin-orbit coupling. However, in contrast to the expectation from the Nagaoka Theorem that a single doped hole…

Strongly Correlated Electrons · Physics 2018-06-13 Sayantika Bhowal , Jamshid Moradi Kurdestany , Sashi Satpathy

The magnetic properties of BaFe$_{2}$As$_{2}$(001) surface have been studied by using first-principles electronic structure calculations. We find that for As-terminated surface the magnetic ground state of the top-layer FeAs is in the…

Superconductivity · Physics 2018-04-06 Bing-Jing Zhang , Kai Liu , Zhong-Yi Lu

We study the phase diagram of a frustrated spin-1/2 ferromagnetic chain with anisotropic exchange interactions in an external magnetic field, using the density matrix renormalization group method. We show that an easy-axis anisotropy…

Strongly Correlated Electrons · Physics 2009-10-29 F. Heidrich-Meisner , I. P. McCulloch , A. K. Kolezhuk

From density functional DFT investigations helped with crystal chemistry rationale, diiron (pairs of Fe), mostly known in molecular diiron nona-carbonyl Fe2(CO)9 and diiron-mono-carbide Fe2C carbide, are embedded in hexagonal C6…

Materials Science · Physics 2021-04-07 Samir F. Matar

In view of the recent experimental reports of unexpected ferromagnetism in HfO$_{2}$ thin films, we carried out first principles investigations looking for magnetic order possibly brought about by the presence of small concentrations of…

Materials Science · Physics 2007-05-23 Chaitanya Das Pemmaraju , S. Sanvito

The orbital contribution to the magnetic properties of Fe in systems of decreasing dimensionality (bulk, surfaces, wire and free clusters) is investigated using a tight-binding hamiltonian in an $s, p,$ and $d$ atomic orbital basis set…

Materials Science · Physics 2008-04-22 Marie-Catherine Desjonquères , Cyrille Barreteau , Gabriel Autes , Daniel Spanjaard

We have investigated structural, electronic and magnetic properties of H$_2$Pc on Fe$_2$N/Fe using low-energy electron diffraction and soft x-ray absorption spectroscopy/x-ray magnetic circular dichroism. Element specific magnetization…