English

Spin Disorder and Magnetic Anisotropy in Fe3O4 Nanoparticles

Materials Science 2007-05-23 v5

Abstract

We have studied the magnetic behavior of dextran-coated magnetite (Fe3_3O4_4) nanoparticles with median particle size <d>=8\left<d\right>=8 nmnm. Magnetization curves and in-field M\"ossbauer spectroscopy measurements showed that the magnetic moment MSM_S of the particles was much smaller than the bulk material. However, we found no evidence of magnetic irreversibility or non-saturating behavior at high fields, usually associated to spin canting. The values of magnetic anisotropy KeffK_{eff} from different techniques indicate that surface or shape contributions are negligible. It is proposed that these particles have bulk-like ferrimagnetic structure with ordered A and B sublattices, but nearly compensated magnetic moments. The dependence of the blocking temperature with frequency and applied fields, TB(H,ω)T_B(H,\omega), suggests that the observed non-monotonic behavior is governed by the strength of interparticle interactions.

Keywords

Cite

@article{arxiv.cond-mat/0505682,
  title  = {Spin Disorder and Magnetic Anisotropy in Fe3O4 Nanoparticles},
  author = {E. Lima and A. L. Brandl and A. D. Arelaro and G. F. Goya},
  journal= {arXiv preprint arXiv:cond-mat/0505682},
  year   = {2007}
}

Comments

11 pages, 7 figures, 3 Tables