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Spin tunneling in molecular magnets controlled by dipole-dipole interactions (DDI) in the disordered state has been considered numerically on the basis of the microscopic model using the quantum mean-field approximation. In the actual case…

Statistical Mechanics · Physics 2014-01-07 D. A. Garanin

Renormalized tunnel splitting with a finite distribution in the biaxial spin model for molecular magnets is obtained by taking into account the dipolar interaction of enviromental spins. Oscillation of the resonant tunnel splitting with a…

Strongly Correlated Electrons · Physics 2009-11-07 Zhi-De Chen , J. -Q. Liang , Shun-Qing Shen

We study the macroscopic quantum tunneling of magnetization of the F=1 spinor condensate interacting through dipole-dipole interaction with an external magnetic field applied along the longitudinal or transverse direction. We show that the…

Other Condensed Matter · Physics 2007-05-23 Limin Yang , Yunbo Zhang

We study the magnetic relaxation of a system of localized spins interacting through weak dipole interactions, at a temperature large with respect to the ordering temperature but low with respect to the crystal field level splitting. The…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 A. Cuccoli , A. Fort , A. Rettori , E. Adam , J. Villain

We review the present state of theory and experiments on the quantum tunneling of magnetization in mesoscopic spin systems. Most attention is paid to the relaxation of magnetization in the molecular complexes Mn12 and Fe8. The role of the…

Condensed Matter · Physics 2007-05-23 Igor Tupitsyn , Bernard Barbara

Combination of the thermal effet in magnetic deflagration with resonance spin tunneling controlled by the dipole-dipole interaction in molecular magnets leads to the increase of the deflagration speed in the dipolar window near tunneling…

Mesoscale and Nanoscale Physics · Physics 2012-01-10 D. A. Garanin , Reem Jaafar

We report measurements and theoretical analysis of resonant spin tunneling in randomly oriented nanospheres of a molecular magnet. Amorphous nanospheres of Mn$_{12}$ acetate have been fabricated and characterized by chemical, infrared, TEM,…

Mesoscale and Nanoscale Physics · Physics 2015-07-30 S. Lendinez , R. Zarzuela , J. Tejada , M. W. Terban , S. J. L. Billinge , J. Espin , I. Imaz , D. Maspoch , E. M. Chudnovsky

Dissipative spin-tunneling transitions at biased resonances in molecular magnets such as Mn-12 Ac are controlled by the dipolar field that can bring the system on and off resonance. It is shown that this leads to spin relaxation in form of…

Statistical Mechanics · Physics 2012-01-10 D. A. Garanin

Motivated by the idea of using simple macroscopic examples to illustrate the physics of complex systems, we modify a historic experimental setup in which interacting floating magnets spontaneously self-assemble into ordered clusters. By…

Soft Condensed Matter · Physics 2024-12-20 P. D. S. de Lima , A. Lyons , A. Irannezhad , J. M. de Araújo , S. Hutzler , M. S. Ferreira

Below 360 mK, Fe magnetic molecular clusters are in the pure quantum relaxation regime and we show that the predicted square-root time relaxation is obeyed, allowing us to develop a new method for watching the evolution of the distribution…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 W. Wernsdorfer , T. Ohm , C. Sangregorio , R. Sessoli , D. Mailly , C. Paulsen

We study the formation and dynamics of dipolar rings composed by microscopic ferromagnetic ellipsoids, which self-assemble in water by switching the direction of the applied field. We show how to manipulate these fragile structures and…

Soft Condensed Matter · Physics 2016-08-30 Fernando Martinez-Pedrero , Andrejs Cebers , Pietro Tierno

The dynamic interplay of transport, electrostatic, and magnetic effects in the resonant tunneling through ferromagnetic quantum wells is theoretically investigated. It is shown that the carrier-mediated magnetic order in the ferromagnetic…

Mesoscale and Nanoscale Physics · Physics 2008-08-13 Christian Ertler , Jaroslav Fabian

The spin-reversal in dilute Li$_2$(Li$_{1-x}$Fe$_{x}$)N with $x < 1$ % is dominated by resonant quantum tunneling of spatially well-separated states. We report on the effect of finite couplings between those states that give rise to…

Strongly Correlated Electrons · Physics 2024-11-04 M. Fix , J. H. Atkinson , F. Müller , E. del Barco , A. Jesche

The tunneling of a giant spin at excited levels is studied theoretically in mesoscopic magnets with a magnetic field at an arbitrary angle in the easy plane. Different structures of the tunneling barriers can be generated by the…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Rong Lu , Hui Pan , Jia-Lin Zhu , Bing-Lin Gu

We examine the quantum tunneling of magnetization in molecular spin in weak interaction with a bath subject to Redfield master equation. By designing a microscopic model for a multilevel spin system using only a generic Hamiltonian and…

Materials Science · Physics 2022-12-27 Le Tuan Anh Ho , Liviu Ungur , Liviu F. Chibotaru

Decoherence processes in crystals of molecular magnets are prototypical for interacting electronic spin systems. We analyze the Landau-Zener dynamics of the archetypical TbPc$_2$ complex diluted in a diamagnetic monocrystal. The dependence…

Mesoscale and Nanoscale Physics · Physics 2020-04-21 Gheorghe Taran , Edgar Bonet , Wolfgang Wernsdorfer

Using a microscopic theory based on the density matrix formalism we investigate quantum revivals and collapses of the charge polarization and charge current dynamics in mesoscopic rings driven by short asymmetric electromagnetic pulses. The…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 A. S. Moskalenko , A. Matos-Abiague , J. Berakdar

We study the dynamical magnetization process in the ordered ground-state phase of the transverse Ising model under sweeps of magnetic field with constant velocities. In the case of very slow sweeps and for small systems studied previously…

Other Condensed Matter · Physics 2009-11-13 Seiji Miyashita , Hans De Raedt , Bernard Barbara

The reversal of the magnetization of crystals of molecular magnets that have a large spin and high anisotropy barrier generally proceeds below the blocking temperature by quantum tunneling. This is manifested as a series of controlled steps…

Mesoscale and Nanoscale Physics · Physics 2013-02-21 Myriam P. Sarachik

The ground state of colloidal magnetic particles in a modulated channel are investigated as function of the tilt angle of an applied magnetic field. The particles are confined by a parabolic potential in the transversal direction while in…

Soft Condensed Matter · Physics 2014-04-02 J. E. Galván-Moya , D. Lucena , W. P. Ferreira , F. M. Peeters
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