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The basic properties of point defects (atomic geometry, the position of charge-transfer levels, and formation energies) on the (110) surface of GaAs, GaP, and InP have been calculated employing density-functional theory. Based on these…

Materials Science · Physics 2007-05-23 G. Schwarz , J. Neugebauer , M. Scheffler

Electrical conductivity is an inherent property of a hydrophobic porous media (HPM) and has critical applications. This research aims to provide a solution for predicting the electrical conductivity of nanoscale HPM with heterogeneous pore…

Soft Condensed Matter · Physics 2021-05-31 Zhongliang Chen , Xiaohu Dong , Zhangxin Chen , Marc-Olivier Coppens

Results of recent density functional theory calculations for alkali metal adsorbates on close-packed metal surfaces are discussed. Single adatoms on the (111) surface of Al and Cu are studied with the self-consistent surface Green-function…

mtrl-th · Physics 2016-09-07 C. Stampfl , M. Scheffler

The first principles density functional theory (DFT) is applied to study effects of molecular adsorption on optical losses of silver (111) surface. The ground states of the systems including water, methanol, and ethanol molecules adsorbed…

Materials Science · Physics 2015-05-14 Alexander V. Gavrilenko , Carla S. McKinney , Vladimir I. Gavrilenko

Our ab initio calculations of CO adsorption on several low and high miller index surfaces of Cu show that the adsorption energy increases as the coordination of the adsorption site decreases from 11 to 6, in qualitative agreement with…

Materials Science · Physics 2013-05-29 Faisal Mehmood , Abdelkader Kara , Talat S. Rahman , Klaus Peter Bohnen

In this paper, we provide a comprehensive theoretical analysis of the electronic structure of InAs(111) surfaces with a special attention paid to the energy region close to the fundamental bandgap. Starting from the bulk electronic…

Materials Science · Physics 2021-03-05 Ivan Vrubel , Dmitry Yudin , Anastasiia Pervishko

We have studied the trends in CO adsorption on close-packed metal surfaces: Co, Ni, Cu from the 3d row, Ru, Rh, Pd, Ag from the 4d row and Ir, Pt, Au from the 5d row using density functional theory. In particular, we were concerned with the…

Materials Science · Physics 2009-11-10 M. Gajdos , A. Eichler , J. Hafner

Electronic and atomic structures of the clean, and As and Te covered Si(211) surface are studied using pseudopotential density functional method. The clean surface is found to have (2 X 1) and rebonded (1 X 1) reconstructions as stable…

Materials Science · Physics 2009-11-10 Prasenjit Sen , Inder P. Batra , S. Sivananthan , C. H. Grein , Nibir Dhar , S. Ciraci

The atomic and electronic structures of Pd3N, PdN and PdN2 were investigated using ab initio density-functional theory (DFT). We studied cohesive energy vs. volume equation of states (EOS) for a set of reported and hypothetical structures.…

Materials Science · Physics 2013-10-11 Mohammed S. H. Suleiman , Daniel P. Joubert

The adsorption of single atoms on pristine and defected hexagonal boron nitride (h-BN) was systematically investigated using density functional theory. Elements from the first three rows of the periodic table, together with selected…

Materials Science · Physics 2026-02-04 Ana S. Dobrota , Natalia V. Skorodumova , Igor A. Pašti

The adsorption of rare gases on metal surfaces serve as the paradigm of weak adsorption where it is typically assumed that the adsorbate occupies maximally coordinated hollow sites. Density-functional theory calculations using the…

Materials Science · Physics 2009-11-07 Juarez L. F. Da Silva , Catherine Stampfl , Matthias Scheffler

We show that a simple first-principles correction based on the difference between the singlet-triplet CO excitation energy values obtained by DFT and high-level quantum chemistry methods yields accurate CO adsorption properties on a variety…

Materials Science · Physics 2009-11-10 Sara E. Mason , Ilya Grinberg , Andrew M. Rappe

We present a 3D isotropic ab initio three-body (para-H$_2$)$_3$ interaction potential energy surface (PES). The electronic structure calculations are carried out at the correlated coupled-cluster theory level, with single, double, and…

Chemical Physics · Physics 2025-06-05 Alexander Ibrahim , Pierre-Nicholas Roy

CO adsorption on Cu(111) and Cu(001) surfaces has been studied within ab-initio density functional theory (DFT). The structural, vibrational and thermodynamic properties of the adsorbate-substrate complex have been calculated. Calculations…

Materials Science · Physics 2009-11-10 M. Gajdos , J. Hafner

We study the electron dynamics at a monocrystalline Pd(111) surface with stepped vicinal nanostructures modeled in a simple Kronig-Penney scheme. The unoccupied bands of the surface are resonantly excited \textit{via} the resonant charge…

Atomic Physics · Physics 2021-06-08 John Shaw , David Monismith , Yixao Zhang , Yixao Zhang , Himadri S. Chakraborty

This paper presents two new adiabatic, global potential energy surfaces (PESs) for the two lowest $^3A'$ and $^3A''$ electronic states of the O($^3P$)+H$_2$ system. For each of these states, ab initio electronic energies were calculated for…

Atomic Physics · Physics 2019-10-02 Alexandre Zanchet , Marta Menéndez , Pablo G. Jambrina , F. Javier Aoiz

Using first-principles calculations, we systematically study the adsorption behaviors of molecular CO on the Be (0001) surface. By calculating the potential energy surfaces, we find that CO molecularly adsorbs on the Be surface with small…

Materials Science · Physics 2015-05-13 Shuang-Xi Wang , Yu Yang , Bo Sun , Rong-Wu Li , Shao-Jun Liu , Ping Zhang

Path optimization methods have been widely used and highly successful for the analysis of chemical reactions. Yet, they can fail to capture intrinsically multidimensional features of potential energy surfaces (PES). We introduce the nudged…

Statistical Mechanics · Physics 2026-04-23 Uday Sankar Manoj , Nicole Drew , Ismaila Dabo , Lukas Muechler

We study the vicinal surface with adsorption below the roughening temperature, using the restricted solid-on-solid model coupled with the Ising model. By the product-wavefunction renormalization group method, we calculate the surface…

Statistical Mechanics · Physics 2009-10-31 Noriko Akutsu , Yasuhiro Akutsu , Takao Yamamoto

We extend density matrix embedding theory to periodic systems, resulting in an electronic band structure method for solid-state materials. The electron correlation can be captured by means of a local impurity model using various choices of…

Strongly Correlated Electrons · Physics 2019-09-27 Hung Q. Pham , Matthew R. Hermes , Laura Gagliardi