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Exchange correlation plays an important role in double-ionization of complex atoms by ultrashort laser pulse. In this work, we investigate two-photon double inner-shell electron ionization of neon induced by an attosecond extreme…

Atomic Physics · Physics 2019-06-05 Jianpeng Liu , Yongqiang Li , Jianmin Yuan

In X-ray photoelectron spectroscopy (XPS), the injected hole interacts with the electronic polarization cloud induced by the hole itself, ultimately resulting in a lower binding energy. Such polarization effect can shift the core-level…

Mesoscale and Nanoscale Physics · Physics 2023-06-23 Iskander Mukatayev , Gabriele D'Avino , Benoit Sklenard , Valerio Olevano , Jing Li

We investigate molecular dynamics of multiple ionization in N2 through multiple core-level photoabsorption and subsequent Auger decay processes induced by intense, short X-ray free electron laser pulses. The timing dynamics of the…

Serial femtosecond X-ray crystallography (SFX) captures the structure and dynamics of biological macromolecules at high spatial and temporal resolutions. The ultrashort pulse produced by an X-ray free electron laser (XFEL) 'outruns' much of…

Plasma Physics · Physics 2025-06-03 Spencer K. Passmore , Alaric L. Sanders , Andrew V. Martin , Harry M. Quiney

Strong-field ionization by counter-rotating two-color laser fields produces quantum interference between photoelectrons emitted on the leading and trailing edges of the laser field oscillations. We show that in chiral molecules, this…

External electric fields are highly attractive for dynamical manipulation of excitons in two-dimensional materials. Here, we theoretically study the ionization of excitons in monolayer transition metal dichalcogenides (TMDs) by intense…

Materials Science · Physics 2022-01-05 Høgni C. Kamban , Thomas G. Pedersen

We show, with an example of Na_92, that for jellium metal clusters the interference of fast electron-waves emitted from equivalent sites on the cluster edge produces monochromatic oscillations in all photoionization observables as a…

Atomic Physics · Physics 2007-05-23 Himadri S. Chakraborty , M. E. Madjet

The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectroscopy and diffraction imaging is a powerful approach to…

We examine correlated electron and doubly charged ion momentum spectra from strong field double ionization of Neon employing intense elliptically polarized laser pulses. An ellipticity-dependent asymmetry of correlated electron and ion…

Submicron-sized targets are found in intense laser-cluster interaction experiments and laser-based material processing. Here we investigate the internal field localization due to Mie scattering and its effect on ionization dynamics in…

Plasma Physics · Physics 2023-05-03 Xiaohui Gao

As a fundamental property of the electron, the spin plays a decisive role in the electronic structure of matter from solids to molecules and atoms, e.g. causing magnetism. Yet, despite its importance, the spin dynamics of electrons released…

We investigate the role of nuclear motion and strong-field-induced electronic couplings during the double ionization of deuterated water using momentum-resolved coincidence spectroscopy. By examining the three-body dicationic dissociation…

Laser-induced ionization is a fundamental tool for the frequency conversion of lasers into spectral regions so far inaccessible, including both extreme ultraviolet and terahertz. The low-frequency currents induced by laser-driven ionization…

We study the ionization dynamics of Ar clusters exposed to ultrashort near-infrared (NIR) laser pulses for intensities well below the threshold at which tunnel ionization ignites nanoplasma formation. We find that the emission of highly…

Atomic and Molecular Clusters · Physics 2016-01-27 Bernd Schütte , Mathias Arbeiter , Alexandre Mermillod-Blondin , Marc J. J. Vrakking , Arnaud Rouzée , Thomas Fennel

The interaction of intense laser fields with silver and argon clusters is investigated theoretically using a modified nanoplasma model. Single pulse and double pulse excitations are considered. The influence of the dense cluster environment…

Atomic and Molecular Clusters · Physics 2009-11-13 Paul Hilse , Max Moll , Manfred Schlanges , Thomas Bornath

We present combined experimental and theoretical results on strong-field ionization of oriented carbonyl-sulphide molecules by circularly-polarized laser pulses. The obtained molecular frame photoelectron angular distributions show…

The rapidly growing demand for compact, high-energy power sources has outpaced the capabilities of conventional electrochemical systems that rely on outer-shell redox reactions. In this work, we present a new energy platform that utilizes…

Atomic Physics · Physics 2026-01-27 Tianrui Li , Yi Jiang , Chen Zhao , Bingsheng Tu , Peining Chen , Jiajun Qin , Huisheng Peng

This paper concerns the theory of non-recollisional ionization or detachment of atoms or ions by intense few-cycle pulses. It is shown that in certain conditions of pulse duration, peak intensity and carrier-envelope phase, the ionization…

Atomic Physics · Physics 2014-09-04 C. C. Chirila , R. M. Potvliege

Metal ions play numerous important roles in biological systems being central to the function of biomolecules. In this letter we show that the absorption of X-rays by these ions leads to a complicated chain of ultrafast relaxation steps…

Chemical Physics · Physics 2016-03-23 Vasili Stumpf , Kirill Gokhberg , Lorenz S. Cederbaum

Inclusive electron scattering off few-nucleon systems is investigated at $x>1$ and high momentum transfer, including the contributions from quasi-elastic and deep inelastic scattering processes. It is shown that at $x>1$ the inclusive cross…

Nuclear Theory · Physics 2011-04-15 S. Simula