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A cluster deposition method was used to produce films of loosely aggregated nanoclusters (NC) of Fe core-Fe3O4 shell or fully oxidized Fe3O4. Films of these NC on Si(100) or MgO(100)/Fe3O4(100) were irradiated to 10^16 Si2+/cm2 near room…

Ultrafast imaging of molecular chirality is a key step towards the dream of imaging and interpreting electronic dynamics in complex and biologically relevant molecules. Here, we propose a new ultrafast chiral phenomenon exploiting recent…

The model is constructed of the propagation of gamma-ray burst radiation through a dense molecular cloud. The main processes of the interaction of the radiation with the interstellar gas are taken into account in the simulations: the…

High Energy Astrophysical Phenomena · Physics 2024-05-20 Aleksandr Nesterenok

Semi-classical molecular dynamics simulations of small rare gas clusters in short laser pulses of 100 nm wavelength were performed. For comparison, the cluster response to 800 nm laser pulses was investigated as well. The inner ionization…

Atomic and Molecular Clusters · Physics 2009-11-10 D. Bauer

Photoionization of an atom $A$ by a strong laser field in the presence of a spatially well-separated neighboring atom $B$ is considered. The laser field frequency is assumed to lie below the ionization potential of atom $A$ and be resonant…

Atomic Physics · Physics 2018-10-03 J. Fedyk , A. B. Voitkiv , C. Müller

Sudden ionisation of a relatively large molecule can initiate a correlation-driven process dubbed charge migration, where the electron density distribution is expected to rapidly change. Capturing this few-femtosecond/attosecond charge…

Kinetic Boltzmann equations are used to model the ionization and expansion dynamics of xenon clusters irradiated with short intense VUV pulses. This unified model includes predominant interactions that contribute to the cluster dynamics…

Atomic and Molecular Clusters · Physics 2015-05-13 B. Ziaja , H. Wabnitz , F. Wang , E. Weckert , T. Moeller

We estimate rate coefficients for charge transfer between neutral hydrogen and helium and moderate to highly ionized heavy elements. Although charge transfer does not have much influence on hot collisionally ionized plasmas, its effects on…

Astrophysics · Physics 2009-10-30 G. J. Ferland , K. T. Korista , D. A. Verner , A. Dalgarno

Effects of ionization injection in low and high Z gas mixtures for the laser wake field acceleration of electrons are analyzed with the use of balance equations and particle-in-cell simulations via test probe particle trajectories in…

Plasma Physics · Physics 2020-03-04 A. Zhidkov , N. Pathak , J. Koga , K. Huang , M. Kando , T. Hosokai

It is known that rare-gas or metal clusters absorb incident laser energy very efficiently. However, due to the intricate dependencies on all the laser and cluster parameters it is difficult to predict under which circumstances ionization…

Plasma Physics · Physics 2009-11-13 M. Kundu , D. Bauer

Understanding the interaction of intense, femtosecond X-ray pulses with heavy atoms is crucial for gaining insights into the structure and dynamics of matter. One key aspect of nonlinear light-matter interaction was, so far, not studied…

Due to electronic many-body effects, the ionization of a molecule can trigger ultrafast electron dynamics appearing as a migration of the created hole charge throughout the system. Here we propose a scheme for control of the charge…

Chemical Physics · Physics 2015-06-11 Nikolay V. Golubev , Alexander I. Kuleff

We show that applying a few-femtosecond mid-infrared laser pulse parallel to the backbone of a halogenated, conjugated organic molecule induces localized ionization followed by long-lasting field-free charge migration (CM). Through…

Atomic Physics · Physics 2024-08-12 Kyle A. Hamer , Francois Mauger , Kenneth Lopata , Kenneth J. Schafer , Mette B. Gaarde

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

Atomic Physics · Physics 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

A detailed theoretical investigation of rare gas atom clusters under intense short laser pulses reveals that the mechanism of energy absorption is akin to {\it enhanced ionization} first discovered for diatomic molecules. The phenomenon is…

Atomic and Molecular Clusters · Physics 2009-11-07 Christian Siedschlag , Jan-Michael Rost

Interfacial ultrafast electron migration processes are simulated in finite cluster models of dye-sensitized solar cells within a single active electron approach. Initially, three different donor-acceptor $\pi$-conjugated dyes supported on…

Chemical Physics · Physics 2017-07-06 Gunter Hermann , Felix Witte , Jean Christophe Tremblay

We study transient charges formed in methane clusters following ionization by intense near-infrared laser pulses. Cluster ionization by 400 fs ($I=1 \times 10^{14}$ W/cm$^2$) pulses is highly efficient, resulting in the observation of a…

Atomic and Molecular Clusters · Physics 2017-08-02 Bernd Schütte , Marc J. J. Vrakking , Arnaud Rouzée

Laser-driven rescattering of electrons is the basis of many strong-field phenomena in atoms and molecules. Here, we will show how this mechanism operates in extended atomic systems, giving rise to effective energy absorption. Rescattering…

Atomic and Molecular Clusters · Physics 2008-04-07 Ulf Saalmann , Jan M. Rost

It is demonstrated that the ionization events in the vicinity of a small floating grain can increase the ion flux to its surface. In this respect the effect of electron impact ionization is fully analogous to that of the ion-neutral…

Plasma Physics · Physics 2012-03-13 Sergey A. Khrapak , Gregor E. Morfill

We have investigated multiphoton multiple ionization dynamics of argon and xenon atoms using a new x-ray free electron laser (XFEL) facility, SPring-8 Angstrom Compact free electron LAser (SACLA) in Japan, and identified that highly charged…