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The graphene-enhanced Raman scattering of Rhodamine 6G molecules on pristine, fluorinated and 4-nitrophenyl functionalized graphene substrates was studied. The uniformity of the Raman signal enhancement was studied by making large Raman…

A periodic arrangement of chains of gold discs shows pronounced plasmonic grating resonances. These have a clear impact on the Surface Enhanced Raman Scattering (SERS)-signal from 4-methylbenzenethiol molecules which form self-assembled…

A plasmonic nanostructure-based substrate, serving as a surface-enhanced Raman scattering (SERS) substrate, enhances the Raman scattering of molecules. By employing an electron beam lithography followed by our recently developed…

We develop a theory for micro-Raman scattering by single and coupled two-donor states in silicon. We find the Raman spectra to have significant dependence on the donor exchange splitting and the relative spatial positions of the two donor…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Belita Koiller , Xuedong Hu , H. D. Drew , S. Das Sarma

In this Letter we analyze theoretically how the emergence of collective strong coupling between vibrational excitations and confined cavity modes affects Raman scattering processes. This work is motivated by recent experiments [Shalabney et…

Mesoscale and Nanoscale Physics · Physics 2016-11-10 Javier del Pino , Johannes Feist , F. J. García-Vidal

Resonant excitation of atoms and ions in macroscopic cavities has lead to exceptional control over quanta of light. Translating these advantages into the solid state with emitters in microcavities promises revolutionary quantum technologies…

There is a growing consensus that the exceptional optoelectronic properties of metal halide perovskites (MHPs) are largely due to the peculiar interplay between the inorganic cage lattice, composed of a labile network of corner-sharing…

Materials Science · Physics 2026-05-21 Alejandro R. Goñi

Strong light-matter coupling gives rise to polaritons -- quasiparticles that combine both photonic and material characteristics. Here, we show that polar nanocrystals exhibit structure- and environment-dependent Raman scattering, enabled by…

Resonant metasurfaces have received extensive attention due to their sharp spectral feature and extraordinary field enhancement. In this work, by breaking the in-plane symmetry of silicon nanopillars, we achieve a sharp Fano resonance. The…

Optics · Physics 2020-04-06 Chaobiao Zhou , Shiyu Li , Cheng Gong , Yi Wang , Xiaojun Liu , Mingsheng Zhan

Localized surface plasmon resonances (LSPRs) have recently been identified in extremely diluted electron systems obtained by doping semiconductor quantum dots. Here we investigate the role that different surface effects, namely electronic…

Optics · Physics 2015-04-29 R. Carmina Monreal , Tomasz J. Antosiewicz , S. Peter Apell

Localized surface plasmon resonances have recently attracted considerable attention due to their ability to dramatically enhance near-field optical intensities and boost nanoscale light-matter interactions. Here we demonstrate unambiguously…

Optics · Physics 2013-01-30 Neda Ghofraniha , Pascal Andrè , Andrea Di falco , Claudio Conti

Localized surface plasmons in metal nanoparticles are widely used in nano-optics to confine and enhance optical fields. It has been previously shown that, if the nanoparticles are distributed periodically, an additional enhancement can be…

Optics · Physics 2024-06-04 Xiaorun Zang , Andriy Shevchenko

Vibrational mode frequencies and damping are calculated for an elastic sphere embedded in an infinite, homogeneous, isotropic elastic medium. Anisotropic elasticity of the sphere significantly shifts the frequencies in comparison to…

Materials Science · Physics 2007-05-23 Lucien Saviot , Daniel B Murray , Maria Del Carmen Marco De Lucas

Stimulated Raman scattering (SRS) in ultra-high-Q surface-tension-induced spherical and chip-based toroid microcavities is considered both theoretically and experimentally. These microcavities are fabricated from silica, exhibit small mode…

Optics · Physics 2007-05-23 Tobias J. Kippenberg , Sean M. Spillane , Bumki Min , Kerry J. Vahala

Presented here are studies of the impact of excitation angle on surface enhanced Raman and luminescence spectroscopy of dye immobilised on a plasmon active nanocavity array support. Results show that both Raman and luminescence intensities…

Optics · Physics 2015-05-20 Frances Lordan , James H Rice , Bincy Jose , Robert J Forster , Tia E Keyes

We explored the surface enhanced Raman scattering (SERS) activity of the InN nanostructures, possessing surface electron accumulation (SEA), using the Rhodamine 6G (R6G) molecules. SERS enhancement is observed for the InN nanostructures…

Materials Science · Physics 2018-08-14 Kishore K. Madapu , Sandip Dhara

We study the effects of chemical bonding on Raman scattering from benzenethiol chemisorbed on silver clusters using time-dependent density functional theory (TDDFT). Raman scattering cross sections are computed using a formalism that…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Semion K. Saikin , Roberto Olivares-Amaya , Dmitrij Rappoport , Michael Stopa , Alán Aspuru-Guzik

Here we show how surface-enhanced Raman spectroscopy (SERS) features can be fine-tuned in optically active substrates made of layered materials. To demonstrate this, we used DNA-assisted lithography (DALI) to create substrates with silver…

A theoretical study describing the coherence properties of near-field Raman scattering in two- and one-dimensional systems is presented. The model is applied to the Raman modes of pristine graphene and graphene edges. Our analysis is based…

Mesoscale and Nanoscale Physics · Physics 2014-03-31 Luiz Gustavo Cançado , Ryan Beams , Ado Jorio , Lukas Novotny

Nonlinear optics in photonic integrated circuits is usually limited to utilizing the nonlinearity of a single material. In this work, we demonstrate the use of hybrid optical nonlinearities that occur in two different materials. This…