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We treat resonant Raman scattering via the multiphonon exciton transitions in cylindrical quantum dots with a parabolic confinement in the lateral direction and with a finite rectangular interface-barrier confinement in the axial direction.…

Mesoscale and Nanoscale Physics · Physics 2012-05-09 S. N. Klimin , V. M. Fomin , J. T. Devreese , J. -P. Leburton

We demonstrate a Raman amplifier for matter-waves, where the amplified atoms and the gain medium are in two different hyperfine states. This amplifier is based on a novel form of superradiance that arises from self-stimulated Raman…

We demonstrate importance of molecular multiple excitons and higher-order plasmons for both enhancement and quenching of resonance Raman and fluorescence of single dye molecule located at plasmonic hotspot under strong coupling regime. The…

Optics · Physics 2019-02-28 Tamitake Itoh , Yuko S. Yamamoto

We investigate three-dimensional rolled-up metamaterials containing optically active quantum wells and metal gratings supporting surface plasmon polarition resonances. Finite-difference time-domain simulations show that by matching the…

Materials Science · Physics 2011-09-09 Andreas Rottler , Stephan Schwaiger , Anuen Koitmäe , Detlef Heitmann , Stefan Mendach

Many reports on stimulated Raman scattering in mixtures of Raman-active and noble gases indicate that the addition of a dispersive buffer gas increases the phase-mismatch to higher-order Stokes and antiStokes sidebands, resulting in…

Optical phonons in nanoparticles with the randomness of interatomic bonds are considered both analytically and numerically. For weak dilute disorder two qualitatively different regimes of separated and overlapped levels are observed,…

Mesoscale and Nanoscale Physics · Physics 2021-08-27 Oleg I. Utesov , Sergei V. Koniakhin , Andrey G. Yashenkin

The review is devoted to explanation of SERS in terms of the dipole and quadrupole light-molecule interactions arising in surface fields strongly varying in space in the region of the strongly irregular surface roughness. The main SERS…

Chemical Physics · Physics 2013-10-01 A. M. Polubotko

Raman spectra obtained by the inelastic scattering of light by crystalline solids contain contributions from first-order vibrational processes (e.g. the emission or absorption of one phonon, a quantum of vibration) as well as higher-order…

Materials Science · Physics 2017-08-22 Yannick Gillet , Stefan Kontur , Matteo Giantomassi , Claudia Draxl , Xavier Gonze

We report the observation of a novel nonlinear effect in the hard x-ray range. Upon illuminating Fe and Cu metal foils with intense x-ray pulses tuned near their respective K edges, photons at nearly twice the incoming photon energy are…

We report a detailed study of the strong near-field Raman scattering enhancement which takes place in tip-enhanced Raman scattering (TERS) in indium nitride. In addition to the well-known first-order optical phonons of indium nitride,…

A hyperbolic metamaterial (HM) resonator is analyzed as a nano-antenna for enhancing the radiative emission of quantum emitters in its vicinity. It has been shown that the spontaneous emission rate by an emitter near a hyperbolic…

Optics · Physics 2014-10-03 Caner Guclu , Ting Shan Luk , George T. Wang , Filippo Capolino

We analyse from a theoretical point of view the optical properties of arrays of carbon nanotubes filled with silver. Dependence of these properties on the different parameters involved is studied using a Transfer Matrix formalism able to…

Materials Science · Physics 2009-10-31 F. J. Garcia-Vidal , J. M. Pitarke , J. B. Pendry

Raman scattering signal can be enhanced through localization of incident field into sub-wavelength hot-spots through plasmonic nano-structures (Surface-enhanced Raman scattering-SERS). Recently, further enhancement of SERS signal via…

Semiconductor-based surface-enhanced Raman spectroscopy (SERS) substrates, as a new frontier in the field of SERS, are hindered by their poor electromagnetic field confinement, and weak light-matter interaction. Metasurfaces, a class of 2D…

The plasmon resonance has found important application in various systems, e.g., nanoantennas, solar panels, refractive index sensors. Unfortunately, a few analytical solutions for such systems are known. The work aims to find a solution for…

Optics · Physics 2022-12-13 Alex Verevkin , Alex Bereza , David Shapiro

Tip enhanced Raman scattering (TERS) amplifies the intensity of vibrational Raman scattering by employing the tip of a probe interacting, in ultra close proximity, with a surface. Although a general understanding of the TERS process is…

Recent Raman data on diamond and crystalline Si nanopowders are analyzed with the use of a microscopic theory of Raman scattering in ensembles of disordered nonpolar nanocrystals. The large width of the Raman peak in nanoparticles as…

Mesoscale and Nanoscale Physics · Physics 2021-09-20 Andrey G. Yashenkin , Oleg I. Utesov , Sergei V. Koniakhin

Raman scattering is the inelastic process where photons bounce off molecules, losing energy and becoming red-shifted. This weak effect is unique to each molecular species, making it an essential tool in e.g. spectroscopy and label-free…

Two-magnon Raman scattering provides important information about electronic correlations in the insulating parent compounds of high-$T_c$ materials. Recent experiments have shown a strong dependence of the Raman signal in $B_{1g}$ geometry…

Strongly Correlated Electrons · Physics 2009-10-30 Dirk K. Morr , Andrey V. Chubukov

In this article, we address the optomechanical effects in surface-enhanced resonant Raman scattering (SERRS) from a single molecule in a nano-particle on mirror (NPoM) nanocavity by developing a quantum master equation theory, which…