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We study lead nanodroplets containing 147 to 1415 atoms at temperatures ranging from the bulk melting point up to the beginning of the evaporation regime. Molecular dynamics simulation and an embedded atom potential are used. The…

Materials Science · Physics 2009-10-30 G. Bilalbegovic , H. O. Lutz

We use density functional theory to quantify finite size and shape effects for gold nanoclusters. We concentrate on the computation of binding energy as a function of bond length for icosahedral and cuboctohedral clusters. We find that the…

Mesoscale and Nanoscale Physics · Physics 2009-12-31 Michael McGuigan , J. W. Davenport

There has long been a discrepancy between the size distributions of Ar$_n^+$ clusters measured by different groups regarding whether or not magic numbers appear at sizes corresponding to the closure of icosahedral (sub-)shells. We show that…

Atomic and Molecular Clusters · Physics 2019-12-04 Michael Gatchell , Paul Martini , Lorenz Kranabetter , Bilal Rasul , Paul Scheier

The properties of small clusters can differ dramatically from the bulk phases of the same constituents. In equilibrium, cluster assembly has been recently explored, whereas out of equilibrium, the physical principles of clustering remain…

Soft Condensed Matter · Physics 2019-03-22 Melody X. Lim , Anton Souslov , Vincenzo Vitelli , Heinrich M. Jaeger

We introduce a local order metric (LOM) that measures the degree of order in the neighborhood of an atomic or molecular site in a condensed medium. The LOM maximizes the overlap between the spatial distribution of sites belonging to that…

Computational Physics · Physics 2018-02-21 Fausto Martelli , Hsin-Yu Ko , Erdal C. Oguz , Roberto Car

We study the evolution of the ICM with a sample of 70 galaxy clusters spanning 0.18 < z < 1.24. We find that X-ray luminosity and ICM mass at a fixed temperature evolve with redshift in a manner inconsistent with the standard self-similar…

Astrophysics · Physics 2007-11-01 T. B. O'Hara , J. J. Mohr , A. J. R. Sanderson

Adsorption on a boundary line confining a monolayer of particles self-assembling into clusters is studied by MC simulations. We focus on a system of particles interacting via competing interaction potential in which effectively short-range…

Soft Condensed Matter · Physics 2020-01-22 E. Bildanau , J. Pȩkalski , V. Vikhrenko , A. Ciach

The yet virtually unexplored class of soft colloidal rods with small aspect ratio is investigated and shown to exhibit a very rich phase and dynamic behavior, spanning from liquid to nearly melt state. Instead of nematic order, these short…

Structural models of growing Ge hut clusters---pyramids and wedges---are proposed on the basis of data of recent STM investigations of nucleation and growth of Ge huts on the Si(001) surface in the process of molecular beam epitaxy. It is…

Materials Science · Physics 2013-09-13 Larisa V. Arapkina , Vladimir A. Yuryev

We study the three-dimensional structure formation when atoms are deposited onto a substrate with a decagonal quasicrystalline order. Molecular-dynamicscalculations show that the adsorbate layer consists of ordered nano-scale domains with…

Materials Science · Physics 2007-11-29 Muhittin Mungan , Yves Weisskopf , Mehmet Erbudak

Magic numbers in finite particle systems correspond to specific system sizes that allow configurations with low free energy, often exhibiting closed surface shells to maximize the number of nearest neighbors. Since their discovery in atomic…

Recently low-temperature structural transition has been reported for complex cubic compounds Cd6M (M=Ca, Yb, Y, rare earth) and it is believed that the transition is due to orientational ordering of an atomic shell in the icosahedral…

Materials Science · Physics 2009-11-13 Kazuki Nozawa , Yasushi Ishii

(shortened) The peculiar chemistry observed in the multiple populations of Galactic globular clusters is not generally found in other systems like dwarf galaxies and open clusters, and at the moment no model can fully explain its presence.…

Solar and Stellar Astrophysics · Physics 2018-06-20 E. Pancino

Metallic nanoclusters displaying electronic shell structure exhibit the special feature of a correlation between their geometry and the number of delocalized electrons . Their shape evolution can be described as a quantum oscillation…

Atomic and Molecular Clusters · Physics 2008-04-04 Vladimir Kresin

We consider the thermodynamically driven self-assembly of spheres onto the surface of a central sphere. This assembly process forms self-limiting, or terminal, anisotropic clusters (N-clusters) with well defined structures. We use Brownian…

Soft Condensed Matter · Physics 2015-06-03 Carolyn L. Phillips , Eric Jankowski , Michelle Marval , Sharon C. Glotzer

We present ab initio perturbed ion calculations on the structures and relative stabilities of doubly charged [(NaCl)_m(Na)_2]2+ cluster ions. The obtained stabilities show excellent agreement with experimental abundances obtained from mass…

Atomic and Molecular Clusters · Physics 2007-05-23 Andres Aguado

Motivated by contradicting reports in the literature, we have investigated the structural stability of tungsten nanoparticles using density functional theory calculations. The comparison of BCC, FCC, A15, disordered, and icosahedral…

Materials Science · Physics 2024-04-08 Laurent Pizzagalli , Sandrine Brochard , Julien Godet , Julien Durinck

Using the Embedded Atom Method as developed by Voter and Chen in combination with the {\it variable metric/quasi-Newton} and our own {\it Aufbau/Abbau} methods, we have identified the three most stable isomers of Au$_N$ clusters with $N$ up…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Denitsa Alamanova , Valeri G. Grigoryan , Michael Springborg

Bimetallic nanoparticles (often known as nanoalloys) with core-shell arrangement are of special interest in several applications, such as in optics, catalysis, magnetism and biomedicine. Despite wide interest in applications, the physical…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Davide Bochicchio , Riccardo Ferrando

Most stars do not form in isolation but as part of a cluster comprising anywhere between a few dozen to several million stars with stellar densities ranging from 0.01 to several 10$^5$ \Msun pc$^{-3}$. The majority of these clusters…

Astrophysics of Galaxies · Physics 2015-05-13 S. Pfalzner