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Related papers: Nonadiabatic corrections to rovibrational levels o…

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We present a program package for the simulation of ultrafast vibration-induced autoionization dynamics in molecular anions in the manifold of the adiabatic anionic states and the discretized ionization continuum. This program, called…

Chemical Physics · Physics 2023-07-14 Kevin Issler , Roland Mitrić , Jens Petersen

We calculated all 2967 even and odd bound states of the adiabatic ground state of NO_2, using a modification of the ab initio potential energy surface of Leonardi et al. [J. Chem. Phys. 105, 9051 (1996)]. The calculation was performed by…

Quantum Physics · Physics 2007-05-23 R. F. Salzgeber , V. Mandelshtam , Ch. Schlier , H. S. Taylor

We study strong field molecular ionization using few- (four to ten) cycle laser pulses. Employing a supercontinuum light source, we are able to tune the optical laser wavelength (photon energy) over a range of about $\sim$200 nm (500 meV).…

The rovibrational kinetic energy for an arbitrary number of rigid molecules is computed. The result has the same general form as the kinetic energy in the molecular rovibrational Hamiltonian, although certain quantities are augmented to…

Atomic and Molecular Clusters · Physics 2009-10-31 Kevin A. Mitchell , Robert G. Littlejohn

We derive an exact solution of an explicitly time-dependent multichannel model of quantum mechanical nonadiabatic transitions. Our model corresponds to the case of a single linear diabatic energy level interacting with a band of an…

Quantum Physics · Physics 2017-02-27 J Lin , N A Sinitsyn

We derive large-amplitude collective equations of motion from the variational principle for the time-dependent Schroedinger equation. These equations reduce to the well-known diabatic formulas for vibrational frequencies in the small…

Nuclear Theory · Physics 2008-11-26 G. F. Bertsch , H. Feldmeier

Second order Newton equations of motion for a radiating particle are presented. It is argued that the trajectories obeying them also satisfy the Abraham-Lorentz-Dirac (ALD) equations for general 3D motions in the non-relativistic and…

General Relativity and Quantum Cosmology · Physics 2013-09-13 Alejandro Cabo Montes de Oca , Nana Geraldine Cabo-Bizet

We review techniques for simulating fully quantum nonadiabatic dynamics using the frozen-width moving Gaussian basis functions to represent the nuclear wavefunction. A choice of these basis functions is primarily motivated by the idea of…

Chemical Physics · Physics 2018-09-05 Loïc Joubert-Doriol , Artur F. Izmaylov

Diabatization of the molecular Hamiltonian is a standard approach to removing the singularities of nonadiabatic couplings at conical intersections of adiabatic potential energy surfaces. In general, it is impossible to eliminate the…

Chemical Physics · Physics 2021-03-26 Seonghoon Choi , Jiří Vaníček

The Schr\"odinger equation for diatomic molecules in deSitter and anti-deSitter spaces is studied using the extended uncertainty principle formulation. The equations are solved by the Nikiforov-Uvarov method for both the Kratzer potential…

Mathematical Physics · Physics 2024-05-08 Meriem AbdelAziz , Mustafa Moumni , Mokhtar Falek

Quantum molecular dynamics requires an accurate representation of the molecular potential energy surface from a minimal number of electronic structure calculations, particularly for nonadiabatic dynamics where excited states are required.…

Chemical Physics · Physics 2016-08-24 Charles W. Heaps , David A. Mazziotti

It is proposed that the Schrodinger equation for a free point particle has non-linear corrections which depend on the mass of the particle. It is assumed that the corrections become extremely small when the mass is much smaller or much…

General Relativity and Quantum Cosmology · Physics 2007-05-23 T. P. Singh

An exactly solvable position-dependent mass Schr\"odinger equation in two dimensions, depicting a particle moving in a semi-infinite layer, is re-examined in the light of recent theories describing superintegrable two-dimensional systems…

Quantum Physics · Physics 2007-05-23 C. Quesne

An algorithm for the calculation of hyperfine structure and spectra of diatomic molecules based on the variational nuclear motion is presented. Hyperfine coupling terms considered are Fermi-contact, nuclear spin-electron spin dipole-dipole,…

Chemical Physics · Physics 2022-02-15 Qianwei Qu , Sergei N. Yurchenko , Jonathan Tennyson

The wobbling motion excited on triaxial superdeformed nuclei is studied in terms of the cranked shell model plus random phase approximation. Firstly, by calculating at a low rotational frequency the \gamma-dependence of the three moments of…

Nuclear Theory · Physics 2014-11-18 Masayuki Matsuzaki , Yoshifumi R. Shimizu , Kenichi Matsuyanagi

In this work, we present analytical solution of Schr\"odinger equation of confined pseudoharmonic potential in presence of a moving boundary condition, for an arbitrary angular momentum state. It turns out that an important quantity to…

Quantum Physics · Physics 2025-06-27 Akash Halder , Amlan K. Roy , Debraj Nath

The static and dynamic electric multipolar polarizabilities and second hyperpolarizabilities of the H$_2^+$, D$_2^+$, and HD$^+$ molecular ions in the ground and first excited states are calculated nonrelativistically using explicitly…

Atomic Physics · Physics 2014-09-23 Li-Yan Tang , Zong-Chao Yan , Ting-Yun Shi , James F. Babb

A general Hamiltonian theory for the adiabatic motion of relativistic charged particles confined by slowly-varying background electromagnetic fields is presented based on a unified Lie-transform perturbation analysis in extended phase space…

Plasma Physics · Physics 2009-11-13 Xin Tao , Anthony Chan , Alain Brizard

We investigate the transition of a quantum wave-packet through a one-dimensional avoided crossing of molecular energy levels when the energy levels at the crossing point are tilted. Using superadiabatic representations, and an approximation…

Mathematical Physics · Physics 2010-07-16 Volker Betz , Benjamin D. Goddard

After the study of the three body molecular system H$_2^+$ ({\it J. Phys. B: At. Mol. Opt. Phys.} {\bf 45} 065101), its isotopomer, the deuterium molecular ion D$_2^+$ is studied. The three-body Schr\"odinger equation is solved using the…

Atomic Physics · Physics 2015-06-15 Horacio Olivares Pilón