English

All bound states of NO_2 (J=0)

Quantum Physics 2007-05-23 v3

Abstract

We calculated all 2967 even and odd bound states of the adiabatic ground state of NO_2, using a modification of the ab initio potential energy surface of Leonardi et al. [J. Chem. Phys. 105, 9051 (1996)]. The calculation was performed by harmonic inversion of the Chebyshev correlation function generated by a DVR Hamiltonian in Radau coordinates. The relative error for the computed eigenenergies is 10410^{-4} or better. Near the dissociation threshold the density of states is about 0.3cm1^{-1}. Statistical analysis of the states shows some interesting structure of the rigidity parameter Δ3\Delta_3 as a function of energy.

Keywords

Cite

@article{arxiv.quant-ph/9712024,
  title  = {All bound states of NO_2 (J=0)},
  author = {R. F. Salzgeber and V. Mandelshtam and Ch. Schlier and H. S. Taylor},
  journal= {arXiv preprint arXiv:quant-ph/9712024},
  year   = {2007}
}

Comments

18 pages of LaTeX including 4 figures. A Postscript of HTML version of this paper can be obtained via: http://phya3.physik.uni-freiburg.de/~rfs/rfs.html This paper was submitted to Journ. Chem. Phys