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Recent experiments have demonstrated strong light-matter coupling between electromagnetic nanoresonators and pristine sheets of two-dimensional semiconductors, and it has been speculated whether these systems can enter the quantum regime…

Quantum Physics · Physics 2022-02-23 E. V. Denning , M. Wubs , N. Stenger , J. Mork , P. T. Kristensen

We show that when following a simple cavity design metric, a quantum well exciton-microcavity photon coupling constant can be larger than the exciton binding energy in GaAs based optical microcavities. Such a very strong coupling…

Quantum Physics · Physics 2018-06-25 H. Zhang , N. Y. Kim , Y. Yamamoto , N. Na

We present detuning-dependent spectral and decay-rate measurements to study the difference between spectral and dynamical properties of single quantum dots embedded in micropillar and photonic-crystal cavities. For the micropillar cavity,…

Quantum Physics · Physics 2013-02-11 K. H. Madsen , P. Lodahl

Strong coupling of excitonic resonances with a cavity gives rise to exciton-polaritons which possess a modified energy landscape compared to the uncoupled emitter. However, due to the femtosecond lifetime of the so-called bright polariton…

Mesoscale and Nanoscale Physics · Physics 2022-05-19 Jan M. Lüttgens , Zhuoran Kuang , Nicolas F. Zorn , Tiago Buckup , Jana Zaumseil

We investigate the interband transitions in several ensembles of self-assembled InAs/GaAs quantum dots by using photoluminescence excitation spectroscopy under strong magnetic field. Well defined resonances are observed in the spectra. A…

Starting from a microscopic model, we investigate the optical spectra of molecules in strongly-coupled organic microcavities examining how they might self-consistently adapt their coupling to light. We consider both rotational and…

Mesoscale and Nanoscale Physics · Physics 2016-03-25 Justyna A. Cwik , Peter Kirton , Simone De Liberato , Jonathan Keeling

The quest to realise strongly interacting photons remains an outstanding challenge both for fundamental science and for applications. Here, we explore mediated photon-photon interactions in a highly imbalanced two-component mixture of…

Mesoscale and Nanoscale Physics · Physics 2021-01-13 A. Camacho-Guardian , M. Bastarrachea-Magnani , G. M. Bruun

Exciton-polaritons -- hybrid states of photons and excitons -- offer unique avenues for controlling electronic, optical, and chemical properties of materials. However, their modeling is mostly limited to formalisms that wash out atomistic…

Excitons, quasiparticles of electrons and holes bound by Coulombic attraction, are created transiently by light and play an important role in optoelectronics, photovoltaics and photosynthesis. While they are also predicted to form…

Strongly Correlated Electrons · Physics 2021-09-29 Keisuke Fukutani , Roland Stania , Chang Il Kwon , Jun Sung Kim , Ki Jeong Kong , Jaeyoung Kim , Han Woong Yeom

The optical spectra of CdSe nanocrystals up to 55 A in diameter are analyzed in a wide range of energies from the fine structure of the low-energy excitations to the so-called high-energy transitions. We apply a symmetry-based method in two…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Perez-Conde , A. K. Bhattacharjee

The coupling of excitons with atomic vibrations plays a pivotal role on the nonequilibrium optical properties of layered semiconductors. However, addressing the dynamical interaction between excitons and phonons represents a hard task both…

We investigate theoretically two-photon processes in a microcavity containing one quantum dot in the strong coupling regime. The cavity mode can be tuned to resonantly drive the two-photon transition between the ground and the biexciton…

Mesoscale and Nanoscale Physics · Physics 2010-01-08 Elena del Valle , Stefano Zippilli , Fabrice P. Laussy , Alejandro Gonzalez-Tudela , Giovanna Morigi , Carlos Tejedor

Quantum electrodynamics of excitons in a cavity is shown to be relevant to quantum operations. We present a theory of an integrable solid-state quantum controlled-phase gate for generating entanglement of two photons using a coupled…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Wang Yao , Renbao Liu , L. J. Sham

The concept of modifying molecular dynamics in strongly coupled exciton-polariton systems is an emerging topic in photonics due to its potential to produce customized chemical systems with tailored photophysical properties. However, before…

Materials Science · Physics 2020-10-09 Bin Liu , Vinod M. Menon , Matthew Y. Sfeir

We create exciton-polaritons in a zero-dimensional (0D) microcavity filled with organic ladder-type conjugated polymer in the strong light-matter interaction regime. Photonic confinement at wavelength scale is realized in the longitudinal…

Mesoscale and Nanoscale Physics · Physics 2019-01-23 Fabio Scafirimuto , Darius Urbonas , Ullrich Scherf , Rainer F. Mahrt , Thilo Stöferle

We study the interplay of electron-electron and electron-phonon interactions in the course of electron-hole bound state formation for gapped solid state systems. Adapting the essentially approximation-free diagrammatic Monte Carlo method…

Strongly Correlated Electrons · Physics 2018-01-31 A. S. Mishchenko , G. De Filippis , V. Cataudella , N. Nagaosa , H. Fehske

We demonstrate that electron-phonon interaction in quantum dots embedded in one-dimensional systems leads to pronounced, non-Markovian decoherence of optical transitions. The experiments we present focus on the lineshape of…

Mesoscale and Nanoscale Physics · Physics 2012-09-18 Christophe Galland , Alexander Högele , Hakan E. Türeci , Ataç Imamoğlu

We study cavity-mediated interactions that are generated in a two-dimensional two-band Hubbard model coupled to an optical cavity, when it is driven in-gap by a strong laser. Starting from a Floquet description of the driven system, we…

Quantum Physics · Physics 2024-03-19 Xiao Wang , Dieter Jaksch , Frank Schlawin

We study optical forces acting upon semiconductor quantum dots and the force driven motion of the dots in a colloid. In the spectral range of exciton transitions in uantum dots, when the photon energy is close to the exciton energy, the…

Mesoscale and Nanoscale Physics · Physics 2017-10-18 Vladimir N. Mantsevich , Sergey A. Tarasenko

We present a new methodology to calculate the strong light-matter coupling between photonic modes in microcavities and large molecular aggregates that consist of hundreds of molecular fragments. To this end, we combine our fragment…

Chemical Physics · Physics 2024-07-30 Richard Einsele , Luca Nils Philipp , Roland Mitrić