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The rate of spontaneous emission is known to depend on the environment of a light source, and the enhancement of one-photon emission in a resonant cavity is known as the Purcell effect. Here we develop a theory of spontaneous two-photon…
The Purcell effect is defined as the modification of spontaneous decay in the presence of a resonator, and in plasmonics it is usually associated with the large local-field enhancement in "hot spots" due to surface plasmon polaritons. Here…
A reliable photon source is required for many aspects of quantum technology. Organic molecules are attractive for this application because they can have high quantum yield and can be photostable, even at room temperature. To generate a…
Defect centers in GaN emerge as bright sources of single-photons which recently have been demonstrated to optically interface a localized spin. However, the structure and composition of these defects as well as their efficient excitation…
We investigate spontaneous emission from a quantum emitter located within the mode volume of a microring resonator that features chiral exceptional points. We show that this configuration offers enough degrees of freedom to exhibit a full…
Metastable qubits in atomic systems can enable large-scale quantum computing by simplifying hardware requirements and adding efficient erasure conversion to the pre-existing toolbox of high-fidelity laser-based control. For trapped atomic…
We demonstrate importance of molecular multiple excitons and higher-order plasmons for both enhancement and quenching of resonance Raman and fluorescence of single dye molecule located at plasmonic hotspot under strong coupling regime. The…
The inclusion of atomic inversion in Raman scattering can significantly alter field dynamics in plasmonic settings. Our calculations show that large local fields and femtosecond pulses combine to yield: (i) population inversion within hot…
The interaction between molecules is commonly ignored in surface-enhanced Raman scattering (SERS). Under this assumption, the total SERS signal is described as the sum of the individual contributions of each molecule treated independently.…
We study the role of strong electron confinement in surface-enhanced Raman scattering from molecules adsorbed on small noble-metal particles. We describe a new source of Raman signal enhancement which originates from different behavior of…
The development of many optical quantum technologies depends on the availability of solid-state single quantum emitters with near-perfect optical coherence. However, a standing issue that limits systematic improvement is the significant…
We study Raman scattering in active media placed in proximity of different types of metal nanostructures, at wavelengths that display either Fabry-Perot or plasmonic resonances, or a combination of both. We use a semi-classical approach to…
We demonstrate enhancements of Raman scattering from graphene on two-dimensional photonic crystals using double resonances, which originate from simultaneous enhancements by a localized guided mode and a cavity mode. By adjusting the…
Giant field enhancement and field singularities are a natural consequence of the commonly employed local-response framework. We show that a more general nonlocal treatment of the plasmonic response leads to new and possibly fundamental…
Stimulated photon-photon scattering is a predicted consequence of quantum electrodynamics that has yet to be measured directly. Measuring the cross-section for stimulated photon-photon scattering is the aim of a flagship experiment for NSF…
We present the first experimental evidence of stimulated Raman re-scattering of a laser in plasma: The scattered light produced by the Raman instability is intense enough to scatter again through the same instability. Although never…
Time-resolved spontaneous Raman spectroscopy serves as a probe for incoherent quasiparticle and collective excitation dynamics, and allows to distinguish symmetry changes across a photoinduced phase transition through the inelastic light…
We study theoretically the quantum optical properties of hybrid molecules composed of an individual quantum dot and a metallic nanoparticle. We calculate the resonance fluorescence of this hybrid system. Its incoherent part, the one arising…
A theoretical study describing the coherence properties of near-field Raman scattering in two- and one-dimensional systems is presented. The model is applied to the Raman modes of pristine graphene and graphene edges. Our analysis is based…
Quantum logic gates performed via two-photon stimulated-Raman transitions in ions and atoms are fundamentally limited by spontaneous scattering errors. Recent theoretical treatment of these scattering processes has predicted no lower bound…