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High entropy oxides (HEO)s have garnered much interest due to their available high degree of tunability. Here, we study the local structure of (MgNiCuCoZn)0.167(MnCr)0.083O, a composition based on the parent HEO (MgNiCuCoZn)0.2O.We…

The comprehensive research of the electronic structure, thermodynamic and electrical transport properties reveals the existence of inhomogeneous superconductivity due to structural disorder in Ca$_3$Rh$_4$Sn$_{13}$ doped with La…

Superconductivity · Physics 2024-10-01 A. Slebarski , P. Zajdel , M. Fijalkowski , M. M. Maska , P. Witas , J. Goraus , Y. Fang , D. C. Arnold , M. B. Maple

Ferromagnetism and accompanying large negative magnetoresistance in Pb-substituted Bi-Sr-Co-O misfit-layer compound are investigated in detail. Recent structural analysis of (Bi,Pb)${}_2$Sr${}_{3}$Co${}_2$O${}_9$, which has been believed to…

Strongly Correlated Electrons · Physics 2009-10-31 I. Tsukada , T. Yamamoto , M. Takagi , T. Tsubone , S. Konno , K. Uchinokura

Correlated oxide heterostructures pose a challenging problem in condensed matter research due to their structural complexity interweaved with demanding electron states beyond the effective single-particle picture. By exploring the…

Materials Science · Physics 2018-04-05 Frank Lechermann

We studied the crystal and magnetic structure of the La$_{1-x}$Ca$_{x}$MnO$_{3}$ compound for $(0.11\leq x\leq 0.175)$ using stoichiometric samples. For $x<0.13$ the system's ground state is insulating canted antiferromagnetic. For $0.13\le…

Strongly Correlated Electrons · Physics 2009-11-11 M. Pissas , I. Margiolaki , G. Papavassiliou , D. Stamopoulos , D. Argyriou

Based on the first-principles calculations, we have investigated the geometry, binding properties, density of states and band structures of the novel superconductor LaFe1-xCoxAsO and its parent compounds with the ZrCuSiAs structure. We…

Superconductivity · Physics 2008-08-06 Haiming Li , Jiong Li , Shuo Zhang , Wangsheng Chu , Dongliang Chen , Ziyu Wu

The high pressure synthesis, structure and magnetic properties of Ca_25Co_22O_56(OH)_28 are reported. The compound has a misfit structure, consisting of double, square calcium oxide hydroxide rock-salt-like layers between hexagonal CoO_2…

Materials Science · Physics 2011-09-08 T. Klimczuk , H. W. Zandbergen , N. M. van der Pers , L. Viciu , V. L. Miller , M. -H. Lee , R. J. Cava

Double perovskite-based magnets wherein frustration and competition between emergent degrees of freedom are at play can lead to novel electronic and magnetic phenomena. Herein, we report the electronic structure and magnetic properties of…

Neutron diffraction studies have been carried out in the temperature(T) range between 10 K and 130 K on a single crystal of YBaCo4O7, which has the stacking of kagome and triangular lattices of CoO4 tetrahedra along the c-axis. Structural…

Strongly Correlated Electrons · Physics 2009-11-11 Minoru Soda , Yukio Yasui , Taketo Moyoshi , Masatoshi Sato , Naoki Igawa , Kazuhisa Kakurai

Oxygen vacancy ordering in perovskite-type transition-metal oxides plays an important role in the emergence of exotic electronic properties, as typified by superconducting cuprates. In this study, we predict the stability of…

Computational Physics · Physics 2020-04-15 Atsuto Seko , Shintaro Ishiwata

Properties of (BaTiO$_3$)$_1$/(BaZrO$_3$)$_n$ ferroelectric superlattices (SLs) with $n = {}$1--7 grown in the [001] direction are calculated from first principles within the density functional theory. It is revealed that the…

Materials Science · Physics 2013-06-20 Alexander I. Lebedev

By using solid-state reactions, we successfully synthesize new oxyselenides CsV$_2$Se$_{2-x}$O (x = 0, 0.5). These compounds containing V$_2$O planar layers with a square lattice crystallize in the CeCr$_2$Si$_2$C structure with the space…

Materials Science · Physics 2018-08-22 Hai Lin , Jin Si , Xiyu Zhu , Kehan Cai , Hao Li , Lu Kong , Xiaodong Yu , Hai-Hu Wen

We have investigated the structure of Co$_2$CO$_3$(OH)$_2$ using Density Functional Theory (DFT) simulations as well as Powder X-Ray Diffraction (PXRD) measurements on samples synthesized via deposition from aqueous solution. We consider…

Density-functional calculations of lattice dynamics and high-resolution synchrotron powder diffraction uncover antiferroelectric distortion in the kagome francisite Cu$_3$Bi(SeO$_3$)$_2$O$_2$Cl below 115K. Its Br-containing analogue is…

The temperature dependent local structure of TbMn2O5 was determined by x-ray absorption spectroscopy. An anomalous Tb-O distribution is found. At high temperature it is broad but resolves into two distinct peaks below approximately 180 K.…

Strongly Correlated Electrons · Physics 2009-11-13 T. A. Tyson , M. Deleon , S. Yoong , S. -W. Cheong

In this Thesis, a study of the electronic structure of two Ti-based oxide systems, TiO2 thin films and the ultra-thin LaAlO3-SrTiO3 (LAO-STO) heterojunctions, is given. A weak room-temperature ferromagnetism (FM) has been detected in…

Strongly Correlated Electrons · Physics 2012-10-31 Giovanni Drera

Bulk La_wCoO3 particles with w=1.1, 1.0, 0.9, 0.8, and 0.7 were synthesized using starting materials with varying molar ratios of La2O3 and Co3O4. The resulting particles are characterized as LaCoO3 crystals interfaced with a crystalline…

Strongly Correlated Electrons · Physics 2015-06-23 A. M. Durand , T. J. Hamil , D. P. Belanger , S. Chi , F. Ye , J. A. Fernandez-Baca , Y. Abdollahian , C. H. Booth

The structure of a new member of the AxCoO2 x nH2O family (A=Li,Na,K) was determined by high-resolution synchrotron X-ray powder diffraction. Layered lithium cobalt oxide hydrate LixCoO2 x 2H2O crystallizes in a disordered monoclinic…

Superconductivity · Physics 2016-08-31 Sangmoon Park , Yongjae Lee , Thomas Vogt

Measurements of electrical resistivity ($\rho$), DC magnetization ($M$) and specific heat ($C$) have been performed on layered oxide Li$_x$CoO$_2$ (0.25$\leq$$x$$\leq$0.99) using single crystal specimens. The $\rho$ versus temperature ($T$)…

Strongly Correlated Electrons · Physics 2015-05-19 K. Miyoshi , C. Iwai , H. Kondo , M. Miura , S. Nishigori , J. Takeuchi

The nonstoichiometric NaxCoO2 system exhibits extraordinary physical properties that correlate with temperature and Na concentration in its layered lattice without evident long-range structure modification when conventional crystallographic…

Strongly Correlated Electrons · Physics 2009-11-10 H. X. Yang , C. J. Nie , Y. G. Shi , H. C. Yu , S. Ding , Y. L. Liu , D. Wu , N. L. Wang , J. Q. Li